Iron‐Incorporated α‐Ni(OH)2 Hierarchical Nanosheet Arrays for Electrocatalytic Urea Oxidation
An iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single‐crystalline belt‐on‐sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni2+‐to‐Ni3+ pre...
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| Published in | Chemistry : a European journal Vol. 24; no. 69; pp. 18408 - 18412 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
10.12.2018
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| Abstract | An iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single‐crystalline belt‐on‐sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni2+‐to‐Ni3+ pre‐oxidation process to boost the generation of active high‐valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron‐incorporated α‐Ni(OH)2 hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future.
An iron belt: A hierarchical belt‐on‐sheet iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst was developed. This catalyst exhibits increased surface areas, improved charge‐transfer behavior, favorable reaction kinetics, and excellent structural stability for robust urea oxidation. |
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| AbstractList | An iron-incorporated α-Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single-crystalline belt-on-sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni2+ -to-Ni3+ pre-oxidation process to boost the generation of active high-valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron-incorporated α-Ni(OH)2 hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future.An iron-incorporated α-Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single-crystalline belt-on-sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni2+ -to-Ni3+ pre-oxidation process to boost the generation of active high-valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron-incorporated α-Ni(OH)2 hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future. An iron‐incorporated α‐Ni(OH) 2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single‐crystalline belt‐on‐sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni 2+ ‐to‐Ni 3+ pre‐oxidation process to boost the generation of active high‐valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron‐incorporated α‐Ni(OH) 2 hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future. An iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single‐crystalline belt‐on‐sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni2+‐to‐Ni3+ pre‐oxidation process to boost the generation of active high‐valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron‐incorporated α‐Ni(OH)2 hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future. An iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single‐crystalline belt‐on‐sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni2+‐to‐Ni3+ pre‐oxidation process to boost the generation of active high‐valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron‐incorporated α‐Ni(OH)2 hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future. An iron belt: A hierarchical belt‐on‐sheet iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst was developed. This catalyst exhibits increased surface areas, improved charge‐transfer behavior, favorable reaction kinetics, and excellent structural stability for robust urea oxidation. An iron-incorporated α-Ni(OH) nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The unique single-crystalline belt-on-sheet hierarchical nanostructure was identified and it endows more reactive edges for the Ni -to-Ni pre-oxidation process to boost the generation of active high-valence species for the urea oxidation reaction (UOR). Benefitting from the optimal Fe concentration, the UOR activity was further optimized owing to the favorable reaction kinetics. With the synergistic benefits of the increased surface areas, improved charge transfer behavior, favorable reaction kinetics and excellent structural stability, the iron-incorporated α-Ni(OH) hierarchical nanosheet array catalyst displays significantly improved UOR performance with both high activity and outstanding operational stability. This work could guide the design of advanced UOR catalysts for wastewater treatment and clean energy production in the future. |
| Author | Liu, Weiwei Xie, Junfeng Zhang, Xiaodong Tang, Bo Lei, Fengcai Gao, Li Qu, Haichao Hao, Pin Xie, Yi |
| Author_xml | – sequence: 1 givenname: Junfeng surname: Xie fullname: Xie, Junfeng email: xiejf@sdnu.edu.cn organization: University of Science and Technology of China – sequence: 2 givenname: Weiwei surname: Liu fullname: Liu, Weiwei organization: Shandong Normal University – sequence: 3 givenname: Fengcai surname: Lei fullname: Lei, Fengcai organization: University of Science and Technology of China – sequence: 4 givenname: Xiaodong surname: Zhang fullname: Zhang, Xiaodong organization: University of Science and Technology of China – sequence: 5 givenname: Haichao surname: Qu fullname: Qu, Haichao organization: Shandong Normal University – sequence: 6 givenname: Li surname: Gao fullname: Gao, Li organization: Shandong Normal University – sequence: 7 givenname: Pin surname: Hao fullname: Hao, Pin organization: Shandong Normal University – sequence: 8 givenname: Bo surname: Tang fullname: Tang, Bo email: tangb@sdnu.edu.cn organization: Shandong Normal University – sequence: 9 givenname: Yi orcidid: 0000-0002-1416-5557 surname: Xie fullname: Xie, Yi email: yxie@ustc.edu.cn organization: University of Science and Technology of China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30088303$$D View this record in MEDLINE/PubMed |
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| Copyright | 2018 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Keywords | oxidation element incorporation electrochemistry nanosheet hierarchical structure |
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| Snippet | An iron‐incorporated α‐Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The... An iron‐incorporated α‐Ni(OH) 2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported.... An iron-incorporated α-Ni(OH) nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The... An iron-incorporated α-Ni(OH)2 nanosheet array catalyst characterized by hierarchical surface nanobelts and robust urea oxidation performance are reported. The... |
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| SubjectTerms | Arrays Catalysis Catalysts Charge transfer Chemistry Clean energy electrochemistry element incorporation hierarchical structure Iron Kinetics nanosheet Nanosheets Nanostructure Nickel compounds Oxidation Oxidation process Reaction kinetics Structural stability Surface charge Urea Wastewater treatment |
| Title | Iron‐Incorporated α‐Ni(OH)2 Hierarchical Nanosheet Arrays for Electrocatalytic Urea Oxidation |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fchem.201803718 https://www.ncbi.nlm.nih.gov/pubmed/30088303 https://www.proquest.com/docview/2153562923 https://www.proquest.com/docview/2085663124 |
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