Anomalous temperature and symmetry-dependent electronic excitations in GdB6

•Unique electronic light scattering in rare-earth boride is observed.•Clear effects of electron-phonon interaction in the spectra temperature behavior.•Ab initio electron structure calculation doesn’t explain temperature effects.•Extra electron scattering is proposed to be coupled to spin disorder.•...

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Published inJournal of alloys and compounds Vol. 881; p. 160507
Main Authors Ponosov, Yu.S., Novoselov, D.Y.
Format Journal Article
LanguageEnglish
Published Lausanne Elsevier B.V 10.11.2021
Elsevier BV
Subjects
Electronic structure
Excitation
Excitation spectra
Inelastic scattering
Light scattering
Raman spectra
Single crystals
Symmetry
Temperature dependence
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Abstract •Unique electronic light scattering in rare-earth boride is observed.•Clear effects of electron-phonon interaction in the spectra temperature behavior.•Ab initio electron structure calculation doesn’t explain temperature effects.•Extra electron scattering is proposed to be coupled to spin disorder.•Chiral excitations found may confirm spin fluctuations existence. Electronic Raman scattering was studied on GdB6 single crystals in the temperature range 10–500 K. The shapes and energy positions of all electronic continua depend on the temperature and symmetry of the excitations. The experimental spectra were modeled using the ab initio DFT electronic structure calculations, taking into account electron-phonon scattering. The appearance of continua of the A1g and Eg symmetry in the spectra was identified with inelastic light scattering from electronic intraband excitations renormalized by the lattice and spin disorder scattering, which is confirmed by the performed calculations. Unexpected observation of T1g symmetry excitations whose profile, intensity and temperature dependence coincide with those for the T2g symmetry excitations suggests the existence of scattering by spin density fluctuations.
AbstractList Electronic Raman scattering was studied on GdB6 single crystals in the temperature range 10–500 K. The shapes and energy positions of all electronic continua depend on the temperature and symmetry of the excitations. The experimental spectra were modeled using the ab initio DFT electronic structure calculations, taking into account electron-phonon scattering. The appearance of continua of the A1g and Eg symmetry in the spectra was identified with inelastic light scattering from electronic intraband excitations renormalized by the lattice and spin disorder scattering, which is confirmed by the performed calculations. Unexpected observation of T1g symmetry excitations whose profile, intensity and temperature dependence coincide with those for the T2g symmetry excitations suggests the existence of scattering by spin density fluctuations.
•Unique electronic light scattering in rare-earth boride is observed.•Clear effects of electron-phonon interaction in the spectra temperature behavior.•Ab initio electron structure calculation doesn’t explain temperature effects.•Extra electron scattering is proposed to be coupled to spin disorder.•Chiral excitations found may confirm spin fluctuations existence. Electronic Raman scattering was studied on GdB6 single crystals in the temperature range 10–500 K. The shapes and energy positions of all electronic continua depend on the temperature and symmetry of the excitations. The experimental spectra were modeled using the ab initio DFT electronic structure calculations, taking into account electron-phonon scattering. The appearance of continua of the A1g and Eg symmetry in the spectra was identified with inelastic light scattering from electronic intraband excitations renormalized by the lattice and spin disorder scattering, which is confirmed by the performed calculations. Unexpected observation of T1g symmetry excitations whose profile, intensity and temperature dependence coincide with those for the T2g symmetry excitations suggests the existence of scattering by spin density fluctuations.
ArticleNumber 160507
Author Ponosov, Yu.S.
Novoselov, D.Y.
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SSID ssj0001931
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Snippet •Unique electronic light scattering in rare-earth boride is observed.•Clear effects of electron-phonon interaction in the spectra temperature behavior.•Ab...
Electronic Raman scattering was studied on GdB6 single crystals in the temperature range 10–500 K. The shapes and energy positions of all electronic continua...
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elsevier
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StartPage 160507
SubjectTerms Electronic structure
Excitation
Excitation spectra
Inelastic scattering
Light scattering
Raman spectra
Single crystals
Symmetry
Temperature dependence
Title Anomalous temperature and symmetry-dependent electronic excitations in GdB6
URI https://dx.doi.org/10.1016/j.jallcom.2021.160507
https://www.proquest.com/docview/2556881422
Volume 881
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