Direct decomposition of NO into N2 and O2 on BaMnO3-based perovskite oxides

Effects of dopant in BaMnO3 perovskite oxide on the NO direct decomposition activity were investigated. NO direct decomposition activity was greatly elevated by doping La and Mg for Ba and Mn site in BaMnO3, respectively. The highest N2 yield was achieved on Ba0.8La0.2Mn0.8Mg0.2O3. The NO decomposit...

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Published inApplied catalysis. B, Environmental Vol. 74; no. 3-4; pp. 299 - 306
Main Authors Iwakuni, Hideharu, Shinmyou, Yusuke, Yano, Hiroshi, Matsumoto, Hiroshige, Ishihara, Tatsumi
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 31.07.2007
Elsevier
Subjects
BaMnO3
Catalysis
Chemistry
Dopant effects
Exact sciences and technology
General and physical chemistry
NO decomposition
Perovskite oxide
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
Dopant effects
Perovskite oxide
NO decomposition
BaMnO3
Heterogeneous catalysis
Perovskite type compound
Oxides
Decomposition
Environmental protection
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Abstract Effects of dopant in BaMnO3 perovskite oxide on the NO direct decomposition activity were investigated. NO direct decomposition activity was greatly elevated by doping La and Mg for Ba and Mn site in BaMnO3, respectively. The highest N2 yield was achieved on Ba0.8La0.2Mn0.8Mg0.2O3. The NO decomposition rate increased with increasing NO partial pressure with PNO1.19. Coexistence of oxygen lowered the N2 yield with PO2−0.18; however, N2 yield of 40% was sustained even under coexisting of 5% O2 at 1123K. Adsorption state of oxygen was also studied with temperature programmed desorption (TPD) method and the desorption temperature of oxygen was lowered by doping Mg for Mn site in BaMnO3.
AbstractList Effects of dopant in BaMnO3 perovskite oxide on the NO direct decomposition activity were investigated. NO direct decomposition activity was greatly elevated by doping La and Mg for Ba and Mn site in BaMnO3, respectively. The highest N2 yield was achieved on Ba0.8La0.2Mn0.8Mg0.2O3. The NO decomposition rate increased with increasing NO partial pressure with PNO1.19. Coexistence of oxygen lowered the N2 yield with PO2-0.18; however, N2 yield of 40% was sustained even under coexisting of 5% O2 at 1123K. Adsorption state of oxygen was also studied with temperature programmed desorption (TPD) method and the desorption temperature of oxygen was lowered by doping Mg for Mn site in BaMnO3.
Effects of dopant in BaMnO3 perovskite oxide on the NO direct decomposition activity were investigated. NO direct decomposition activity was greatly elevated by doping La and Mg for Ba and Mn site in BaMnO3, respectively. The highest N2 yield was achieved on Ba0.8La0.2Mn0.8Mg0.2O3. The NO decomposition rate increased with increasing NO partial pressure with PNO1.19. Coexistence of oxygen lowered the N2 yield with PO2−0.18; however, N2 yield of 40% was sustained even under coexisting of 5% O2 at 1123K. Adsorption state of oxygen was also studied with temperature programmed desorption (TPD) method and the desorption temperature of oxygen was lowered by doping Mg for Mn site in BaMnO3.
Author Matsumoto, Hiroshige
Yano, Hiroshi
Iwakuni, Hideharu
Ishihara, Tatsumi
Shinmyou, Yusuke
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  surname: Iwakuni
  fullname: Iwakuni, Hideharu
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  givenname: Yusuke
  surname: Shinmyou
  fullname: Shinmyou, Yusuke
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  givenname: Hiroshi
  surname: Yano
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  surname: Matsumoto
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  givenname: Tatsumi
  surname: Ishihara
  fullname: Ishihara, Tatsumi
  email: ishihara@cstf.kyushu-u.ac.jp
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Issue 3-4
Keywords Dopant effects
Perovskite oxide
NO decomposition
BaMnO3
Heterogeneous catalysis
Perovskite type compound
Oxides
Decomposition
Environmental protection
Language English
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Snippet Effects of dopant in BaMnO3 perovskite oxide on the NO direct decomposition activity were investigated. NO direct decomposition activity was greatly elevated...
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SubjectTerms BaMnO3
Catalysis
Chemistry
Dopant effects
Exact sciences and technology
General and physical chemistry
NO decomposition
Perovskite oxide
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
Title Direct decomposition of NO into N2 and O2 on BaMnO3-based perovskite oxides
URI https://dx.doi.org/10.1016/j.apcatb.2007.02.020
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