Hydrogen oxidation electrocatalysts for anion-exchange membrane fuel cells: activity descriptors, stability regulation, and perspectives

The burgeoning field of anion-exchange membrane fuel cells (AEMFCs) presents a promising avenue to circumvent the reliance on scarce and costly Pt-based catalysts, offering a zero-carbon emission alternative. Despite the success of numerous noble metal-free cathodic oxygen reduction reaction catalys...

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Published inEnergy & environmental science Vol. 17; no. 12; pp. 396 - 49
Main Authors Ren, Jin-Tao, Chen, Lei, Wang, Hao-Yu, Feng, Yi, Yuan, Zhong-Yong
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 18.06.2024
Subjects
Anion exchanging
Anodizing
Catalysts
Chemical reduction
Commercialization
Electrocatalysts
Electrolytes
Electrolytic cells
Emissions
Energy theory
Fuel cells
Fuel technology
Heterostructures
Hydrogen
Kinetics
Membranes
Noble metals
Oxidation
Oxygen reduction reactions
Reaction mechanisms
Stability
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Abstract The burgeoning field of anion-exchange membrane fuel cells (AEMFCs) presents a promising avenue to circumvent the reliance on scarce and costly Pt-based catalysts, offering a zero-carbon emission alternative. Despite the success of numerous noble metal-free cathodic oxygen reduction reaction catalysts in AEMFCs, the sluggish kinetics of the anodic hydrogen oxidation reaction (HOR) in alkaline media, necessitating a high Pt amount, poses a substantial impediment to AEMFC development. This review delves into the intricate landscape of the alkaline HOR, commencing with exploration of prevailing theories grounded in diverse activity descriptors, such as the hydrogen binding energy theory and bifunctional theory. The elucidation of sluggish kinetics and reaction mechanisms in alkaline electrolytes serves as the foundation for the analysis of noble and non-noble metal catalysts, encompassing considerations of morphology, composition, local structure, heterostructure, spillover effects, single atomic catalysts, and oxyphilic site engineering. Emphasis is placed on addressing pivotal but often overlooked challenges, including long-term stability, antioxidation ability, and CO tolerance of HOR catalysts. This review underscores the significance of theoretical investigations and in situ characterization technologies. Subsequently, recent strides in AEMFCs, leveraging various electrocatalysts for enhanced activity and durability, are meticulously summarized. The narrative concludes by spotlighting persisting controversies surrounding alkaline HOR mechanisms, along with an exposition of challenges and prospective research directions vital for the eventual commercialization of AEMFCs. The general principles in terms of reactivity and stability to design efficient electrocatalysts for the alkaline hydrogen oxidation reaction are reviewed. The performance of catalysts in anion-exchange membrane fuel cells is further discussed.
AbstractList The burgeoning field of anion-exchange membrane fuel cells (AEMFCs) presents a promising avenue to circumvent the reliance on scarce and costly Pt-based catalysts, offering a zero-carbon emission alternative. Despite the success of numerous noble metal-free cathodic oxygen reduction reaction catalysts in AEMFCs, the sluggish kinetics of the anodic hydrogen oxidation reaction (HOR) in alkaline media, necessitating a high Pt amount, poses a substantial impediment to AEMFC development. This review delves into the intricate landscape of the alkaline HOR, commencing with exploration of prevailing theories grounded in diverse activity descriptors, such as the hydrogen binding energy theory and bifunctional theory. The elucidation of sluggish kinetics and reaction mechanisms in alkaline electrolytes serves as the foundation for the analysis of noble and non-noble metal catalysts, encompassing considerations of morphology, composition, local structure, heterostructure, spillover effects, single atomic catalysts, and oxyphilic site engineering. Emphasis is placed on addressing pivotal but often overlooked challenges, including long-term stability, antioxidation ability, and CO tolerance of HOR catalysts. This review underscores the significance of theoretical investigations and in situ characterization technologies. Subsequently, recent strides in AEMFCs, leveraging various electrocatalysts for enhanced activity and durability, are meticulously summarized. The narrative concludes by spotlighting persisting controversies surrounding alkaline HOR mechanisms, along with an exposition of challenges and prospective research directions vital for the eventual commercialization of AEMFCs.
The burgeoning field of anion-exchange membrane fuel cells (AEMFCs) presents a promising avenue to circumvent the reliance on scarce and costly Pt-based catalysts, offering a zero-carbon emission alternative. Despite the success of numerous noble metal-free cathodic oxygen reduction reaction catalysts in AEMFCs, the sluggish kinetics of the anodic hydrogen oxidation reaction (HOR) in alkaline media, necessitating a high Pt amount, poses a substantial impediment to AEMFC development. This review delves into the intricate landscape of the alkaline HOR, commencing with exploration of prevailing theories grounded in diverse activity descriptors, such as the hydrogen binding energy theory and bifunctional theory. The elucidation of sluggish kinetics and reaction mechanisms in alkaline electrolytes serves as the foundation for the analysis of noble and non-noble metal catalysts, encompassing considerations of morphology, composition, local structure, heterostructure, spillover effects, single atomic catalysts, and oxyphilic site engineering. Emphasis is placed on addressing pivotal but often overlooked challenges, including long-term stability, antioxidation ability, and CO tolerance of HOR catalysts. This review underscores the significance of theoretical investigations and in situ characterization technologies. Subsequently, recent strides in AEMFCs, leveraging various electrocatalysts for enhanced activity and durability, are meticulously summarized. The narrative concludes by spotlighting persisting controversies surrounding alkaline HOR mechanisms, along with an exposition of challenges and prospective research directions vital for the eventual commercialization of AEMFCs. The general principles in terms of reactivity and stability to design efficient electrocatalysts for the alkaline hydrogen oxidation reaction are reviewed. The performance of catalysts in anion-exchange membrane fuel cells is further discussed.
The burgeoning field of anion-exchange membrane fuel cells (AEMFCs) presents a promising avenue to circumvent the reliance on scarce and costly Pt-based catalysts, offering a zero-carbon emission alternative. Despite the success of numerous noble metal-free cathodic oxygen reduction reaction catalysts in AEMFCs, the sluggish kinetics of the anodic hydrogen oxidation reaction (HOR) in alkaline media, necessitating a high Pt amount, poses a substantial impediment to AEMFC development. This review delves into the intricate landscape of the alkaline HOR, commencing with exploration of prevailing theories grounded in diverse activity descriptors, such as the hydrogen binding energy theory and bifunctional theory. The elucidation of sluggish kinetics and reaction mechanisms in alkaline electrolytes serves as the foundation for the analysis of noble and non-noble metal catalysts, encompassing considerations of morphology, composition, local structure, heterostructure, spillover effects, single atomic catalysts, and oxyphilic site engineering. Emphasis is placed on addressing pivotal but often overlooked challenges, including long-term stability, antioxidation ability, and CO tolerance of HOR catalysts. This review underscores the significance of theoretical investigations and in situ characterization technologies. Subsequently, recent strides in AEMFCs, leveraging various electrocatalysts for enhanced activity and durability, are meticulously summarized. The narrative concludes by spotlighting persisting controversies surrounding alkaline HOR mechanisms, along with an exposition of challenges and prospective research directions vital for the eventual commercialization of AEMFCs.
Author Feng, Yi
Wang, Hao-Yu
Ren, Jin-Tao
Chen, Lei
Yuan, Zhong-Yong
AuthorAffiliation Smart Sensing Interdisciplinary Science Center
School of Materials Science and Engineering
Nankai University
National Institute for Advanced Materials
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Notes Zhong-Yong Yuan received his PhD degree in Physical Chemistry from Nankai University in 1999. He worked as a postdoctoral fellow at the Institute of Physics, Chinese Academy of Sciences from 1999 to 2001. He then moved to Belgium, working as a research fellow at the University of Namur from 2001 to 2005, prior to joining Nankai University as a full professor. In 2016, he was elected as a fellow of the Royal Society of Chemistry (FRSC). His research interests are mainly in the self-assembly of hierarchically nanoporous and nanostructured materials for energy and environmental applications.
Jin-Tao Ren received his PhD degree from Nankai University in 2020 under the supervision of Prof. Zhong-Yong Yuan. He is currently a postdoctoral fellow at Nankai University. His research interests focus on advanced nanomaterials for applications in electrocatalysis, metal-air batteries, fuel cells, etc.
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Snippet The burgeoning field of anion-exchange membrane fuel cells (AEMFCs) presents a promising avenue to circumvent the reliance on scarce and costly Pt-based...
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SubjectTerms Anion exchanging
Anodizing
Catalysts
Chemical reduction
Commercialization
Electrocatalysts
Electrolytes
Electrolytic cells
Emissions
Energy theory
Fuel cells
Fuel technology
Heterostructures
Hydrogen
Kinetics
Membranes
Noble metals
Oxidation
Oxygen reduction reactions
Reaction mechanisms
Stability
Title Hydrogen oxidation electrocatalysts for anion-exchange membrane fuel cells: activity descriptors, stability regulation, and perspectives
URI https://www.proquest.com/docview/3069060803
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