Advanced design strategies for Fe-based metal-organic framework-derived electrocatalysts toward high-performance Zn-air batteries

Zinc-air batteries (ZABs) are considered as one of the most promising energy systems due to their environmentally friendly and high energy density characteristics. Nevertheless, the kinetics of oxygen reaction at the air electrode of ZABs are slow, resulting in poor energy efficiency and cycling pro...

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Published inEnergy & environmental science Vol. 17; no. 5; pp. 1725 - 1755
Main Authors Guo, Ya-Fei, Zhao, Shan, Zhang, Nan, Liu, Zong-Lin, Wang, Peng-Fei, Zhang, Jun-Hong, Xie, Ying, Yi, Ting-Feng
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 05.03.2024
Subjects
Catalysts
Chemical reduction
Cycles
Electrocatalysts
Energy efficiency
Heavy metals
Iron
Metal air batteries
Metal-organic frameworks
Metals
Noble metals
Oxygen
Oxygen evolution reactions
Oxygen reduction reactions
Porosity
Precious metals
Pyrolysis
Storage capacity
Structural stability
Transition metals
Zinc-oxygen batteries
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Abstract Zinc-air batteries (ZABs) are considered as one of the most promising energy systems due to their environmentally friendly and high energy density characteristics. Nevertheless, the kinetics of oxygen reaction at the air electrode of ZABs are slow, resulting in poor energy efficiency and cycling properties of ZABs. How to improve the overall performance and long-term cycling stability of ZABs is the key to their development. So far, precious metals and their alloys have been considered the most ideal oxygen reduction reaction/oxygen evolution reaction catalysts. Nevertheless, the high cost and low storage capacity of these precious metals limit their application. Transition metal catalysts have received widespread attention because of their high electrocatalytic activity, structural stability, abundant reserves, and low prices. Among them, Fe-based catalysts are regarded as one of the most hopeful candidates due to their lowest price and ease of performance improvement. Metal-organic frameworks (MOFs) have advantages such as structural diversity, high specific surface area (SSA), and porosity. Especially as precursors of transition metal catalysts, organic ligands in MOFs are combined with bridged metal nodes to provide the necessary metals, carbon, and heteroatoms for electrocatalysts. However, MOFs may experience structural collapse, atomic aggregation, and reduced active sites during pyrolysis, which limits their commercial applications. Therefore, nano-design is extremely significant in improving catalytic capability. This review summarizes the morphology, composition, and structural control strategies of Fe-based MOF-derived electrocatalysts. In addition, the active sites, catalytic mechanism, and corresponding characteristics of electrocatalysts are introduced. Finally, the challenges and development prospects of optimized oxygen electrocatalysts in ZABs are discussed. This review provides insights into the targeted optimization of Fe-based MOF derived oxygen electrocatalysts and is expected to promote the future development of high-performance ZABs. This article summarizes the regulation strategies of Fe-based MOFs-derived electrocatalysts for ZABs, and provides a prospect for their future development.
AbstractList Zinc-air batteries (ZABs) are considered as one of the most promising energy systems due to their environmentally friendly and high energy density characteristics. Nevertheless, the kinetics of oxygen reaction at the air electrode of ZABs are slow, resulting in poor energy efficiency and cycling properties of ZABs. How to improve the overall performance and long-term cycling stability of ZABs is the key to their development. So far, precious metals and their alloys have been considered the most ideal oxygen reduction reaction/oxygen evolution reaction catalysts. Nevertheless, the high cost and low storage capacity of these precious metals limit their application. Transition metal catalysts have received widespread attention because of their high electrocatalytic activity, structural stability, abundant reserves, and low prices. Among them, Fe-based catalysts are regarded as one of the most hopeful candidates due to their lowest price and ease of performance improvement. Metal-organic frameworks (MOFs) have advantages such as structural diversity, high specific surface area (SSA), and porosity. Especially as precursors of transition metal catalysts, organic ligands in MOFs are combined with bridged metal nodes to provide the necessary metals, carbon, and heteroatoms for electrocatalysts. However, MOFs may experience structural collapse, atomic aggregation, and reduced active sites during pyrolysis, which limits their commercial applications. Therefore, nano-design is extremely significant in improving catalytic capability. This review summarizes the morphology, composition, and structural control strategies of Fe-based MOF-derived electrocatalysts. In addition, the active sites, catalytic mechanism, and corresponding characteristics of electrocatalysts are introduced. Finally, the challenges and development prospects of optimized oxygen electrocatalysts in ZABs are discussed. This review provides insights into the targeted optimization of Fe-based MOF derived oxygen electrocatalysts and is expected to promote the future development of high-performance ZABs. This article summarizes the regulation strategies of Fe-based MOFs-derived electrocatalysts for ZABs, and provides a prospect for their future development.
Zinc–air batteries (ZABs) are considered as one of the most promising energy systems due to their environmentally friendly and high energy density characteristics. Nevertheless, the kinetics of oxygen reaction at the air electrode of ZABs are slow, resulting in poor energy efficiency and cycling properties of ZABs. How to improve the overall performance and long-term cycling stability of ZABs is the key to their development. So far, precious metals and their alloys have been considered the most ideal oxygen reduction reaction/oxygen evolution reaction catalysts. Nevertheless, the high cost and low storage capacity of these precious metals limit their application. Transition metal catalysts have received widespread attention because of their high electrocatalytic activity, structural stability, abundant reserves, and low prices. Among them, Fe-based catalysts are regarded as one of the most hopeful candidates due to their lowest price and ease of performance improvement. Metal–organic frameworks (MOFs) have advantages such as structural diversity, high specific surface area (SSA), and porosity. Especially as precursors of transition metal catalysts, organic ligands in MOFs are combined with bridged metal nodes to provide the necessary metals, carbon, and heteroatoms for electrocatalysts. However, MOFs may experience structural collapse, atomic aggregation, and reduced active sites during pyrolysis, which limits their commercial applications. Therefore, nano-design is extremely significant in improving catalytic capability. This review summarizes the morphology, composition, and structural control strategies of Fe-based MOF-derived electrocatalysts. In addition, the active sites, catalytic mechanism, and corresponding characteristics of electrocatalysts are introduced. Finally, the challenges and development prospects of optimized oxygen electrocatalysts in ZABs are discussed. This review provides insights into the targeted optimization of Fe-based MOF derived oxygen electrocatalysts and is expected to promote the future development of high-performance ZABs.
Author Zhang, Jun-Hong
Yi, Ting-Feng
Zhao, Shan
Zhang, Nan
Wang, Peng-Fei
Liu, Zong-Lin
Xie, Ying
Guo, Ya-Fei
AuthorAffiliation Ministry of Education
School of Resources and Materials
School of Materials Science and Engineering
Key Laboratory of Functional Inorganic Material Chemistry
School of Chemistry and Materials Science
Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology
College of Chemistry and Chemical Engineering
Heilongjiang University
Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province
Northeastern University
Liaocheng University
Northeastern University at Qinhuangdao
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Notes Prof. Ting-Feng Yi is currently a full professor at the School of Materials Science and Engineering, Northeastern University, Shenyang, China. He received his MSc degree in Applied Chemistry in 2004 and PhD degree in Chemical Engineering and Technology from the Harbin Institute of Technology in 2007. His research interests include the synthesis of functional materials and their application in batteries and supercapacitors.
Nan Zhang is currently a master's student at the School of Materials Science and Engineering of Northeastern University. Her main research interests are energy storage and conversion devices, especially Zn-air batteries and solid-state batteries.
Dr Zonglin Liu is currently a lecturer at the School of Resources and Materials, Northeastern University at Qinhuangdao, Qinhuangdao, China. She received her BSc and MSc from Northeast Forestry University and Ocean University of China, respectively. Then, she obtained her PhD degree in 2023 from Harbin Institute of Technology. Her research focuses on catalysts for electrocatalytic reactions, mainly for hydrogen evolution reaction, oxygen evolution reaction, water splitting, and zinc-air batteries.
Ya-Fei Guo is currently a master's student at the School of Materials Science and Engineering of Northeastern University. Her current research focuses on aqueous zinc metal-based batteries.
Dr Peng-Fei Wang is currently a lecturer at Northeastern University at Qinhuangdao, China. He received his PhD degree from Nanjing University in 2021. His major research interests focus on Li-sulfur battery, solid-state battery and photothermal battery.
Prof. Junhong Zhang is currently a professor at the College of Chemistry and Chemical Engineering, Liaocheng University, Liaocheng, China. She received her BSc and MSc from Liaocheng University. Then, she obtained her PhD degree in 2011 from the Ocean University of China. Her research focuses on electrochemistry.
Shan Zhao is currently a master's student at the School of Materials Science and Engineering of Northeastern University. Her main research interests are metal-air batteries and water electrolysis.
Prof. Ying Xie is currently a full professor at the School of Chemistry and Materials Science, Heilongjiang University, Harbin, China. He received his MSc degree in Applied Chemistry in 2004 and PhD degree in Chemical Engineering and Technology from the Harbin Institute of Technology in 2008. His research interests mainly focus on the applications of theoretical methods to explore the structure-property relationships of some energy storage and conversion materials.
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Snippet Zinc-air batteries (ZABs) are considered as one of the most promising energy systems due to their environmentally friendly and high energy density...
Zinc–air batteries (ZABs) are considered as one of the most promising energy systems due to their environmentally friendly and high energy density...
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SubjectTerms Catalysts
Chemical reduction
Cycles
Electrocatalysts
Energy efficiency
Heavy metals
Iron
Metal air batteries
Metal-organic frameworks
Metals
Noble metals
Oxygen
Oxygen evolution reactions
Oxygen reduction reactions
Porosity
Precious metals
Pyrolysis
Storage capacity
Structural stability
Transition metals
Zinc-oxygen batteries
Title Advanced design strategies for Fe-based metal-organic framework-derived electrocatalysts toward high-performance Zn-air batteries
URI https://www.proquest.com/docview/2937271095
Volume 17
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