Nitrogen-rich covalent phosphazene-based framework for efficient removal of lead() ions
Covalent organic frameworks (COFs), as a new type of porous crystalline material, are suitable for selective adsorption and separation of various heavy metal ions due to their stable framework structure, abundant surface functional groups, adjustable pore structure and large adsorption capacity. Her...
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Published in | New journal of chemistry Vol. 47; no. 13; pp. 695 - 611 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
Cambridge
Royal Society of Chemistry
27.03.2023
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Abstract | Covalent organic frameworks (COFs), as a new type of porous crystalline material, are suitable for selective adsorption and separation of various heavy metal ions due to their stable framework structure, abundant surface functional groups, adjustable pore structure and large adsorption capacity. Herein, a nitrogen-rich phosphazene-based covalent organic framework was synthesized for efficient Pb
2+
removal from aqueous solution. Adsorption equilibrium of the adsorbent could be achieved within 30 min, and the as-synthesized N-CPF exhibits an exceedingly high Pb
2+
uptake capacity of 816 mg g
−1
, surpassing those of most previously reported materials. The kinetics and adsorption isotherms were better fitted by the pseudo-second-order model and the Langmuir model, respectively. Furthermore, N-CPF exhibited high adsorption selectivity for Pb
2+
compared to other heavy metals.
Nitrogen-rich phosphazene-based covalent organic framework was synthesized for efficient Pb
2+
removal from aqueous solution. The N-CPF exhibits an exceedingly high Pb
2+
uptake capacity of 816 mg g
−1
and a fast adsorption rate. |
---|---|
AbstractList | Covalent organic frameworks (COFs), as a new type of porous crystalline material, are suitable for selective adsorption and separation of various heavy metal ions due to their stable framework structure, abundant surface functional groups, adjustable pore structure and large adsorption capacity. Herein, a nitrogen-rich phosphazene-based covalent organic framework was synthesized for efficient Pb
2+
removal from aqueous solution. Adsorption equilibrium of the adsorbent could be achieved within 30 min, and the as-synthesized N-CPF exhibits an exceedingly high Pb
2+
uptake capacity of 816 mg g
−1
, surpassing those of most previously reported materials. The kinetics and adsorption isotherms were better fitted by the pseudo-second-order model and the Langmuir model, respectively. Furthermore, N-CPF exhibited high adsorption selectivity for Pb
2+
compared to other heavy metals.
Nitrogen-rich phosphazene-based covalent organic framework was synthesized for efficient Pb
2+
removal from aqueous solution. The N-CPF exhibits an exceedingly high Pb
2+
uptake capacity of 816 mg g
−1
and a fast adsorption rate. Covalent organic frameworks (COFs), as a new type of porous crystalline material, are suitable for selective adsorption and separation of various heavy metal ions due to their stable framework structure, abundant surface functional groups, adjustable pore structure and large adsorption capacity. Herein, a nitrogen-rich phosphazene-based covalent organic framework was synthesized for efficient Pb2+ removal from aqueous solution. Adsorption equilibrium of the adsorbent could be achieved within 30 min, and the as-synthesized N-CPF exhibits an exceedingly high Pb2+ uptake capacity of 816 mg g−1, surpassing those of most previously reported materials. The kinetics and adsorption isotherms were better fitted by the pseudo-second-order model and the Langmuir model, respectively. Furthermore, N-CPF exhibited high adsorption selectivity for Pb2+ compared to other heavy metals. Covalent organic frameworks (COFs), as a new type of porous crystalline material, are suitable for selective adsorption and separation of various heavy metal ions due to their stable framework structure, abundant surface functional groups, adjustable pore structure and large adsorption capacity. Herein, a nitrogen-rich phosphazene-based covalent organic framework was synthesized for efficient Pb 2+ removal from aqueous solution. Adsorption equilibrium of the adsorbent could be achieved within 30 min, and the as-synthesized N-CPF exhibits an exceedingly high Pb 2+ uptake capacity of 816 mg g −1 , surpassing those of most previously reported materials. The kinetics and adsorption isotherms were better fitted by the pseudo-second-order model and the Langmuir model, respectively. Furthermore, N-CPF exhibited high adsorption selectivity for Pb 2+ compared to other heavy metals. |
Author | Xie, Jun Liu, Yu Tang, Ke-Wen Peng, Lin-ling Zhou, Cong-Shan Xu, Wei-Feng Zhou, Wei-Fang |
AuthorAffiliation | Department of Chemistry and Chemical Engineering Hunan Institute of Science and Technology |
AuthorAffiliation_xml | – name: Hunan Institute of Science and Technology – name: Department of Chemistry and Chemical Engineering |
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SubjectTerms | Aqueous solutions Covalence Functional groups Heavy metals Lead Nitrogen Phosphazene Porous materials Selective adsorption Synthesis |
Title | Nitrogen-rich covalent phosphazene-based framework for efficient removal of lead() ions |
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