Preparation and properties of K2NiF4-type perovskite oxides La2NiO4 catalysts for steam reforming of ethanol

The performance of La2NiO4 perovskite catalysts, prepared using a citric acid complexation method, for the steam reforming of ethanol was studied. The catalysts were characterized by X-ray diffractometry （XRD）, specific surface area measurements （BET）, thermogravimetric analysis （TGA） and scanning e...

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Published inTransactions of Nonferrous Metals Society of China Vol. 19; no. 6; pp. 1444 - 1449
Main Author 张利峰 王一平 黄群武
Format Journal Article
LanguageEnglish
Published 01.12.2009
Subjects
K2NiF4型
La2NiO4
扫描电子显微镜
重整催化剂
钙钛矿氧化物
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ISSN1003-6326
DOI10.1016/S1003-6326(09)60048-0

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Abstract The performance of La2NiO4 perovskite catalysts, prepared using a citric acid complexation method, for the steam reforming of ethanol was studied. The catalysts were characterized by X-ray diffractometry （XRD）, specific surface area measurements （BET）, thermogravimetric analysis （TGA） and scanning electron microscopy （SEM）. The experimental results show that the calcination temperature and thc amount of citric acid （CA） have a significant influence on the characteristics of the catalysts and their catalytic activity. Among the catalysts tested, the La2NiO4 catalyst calcined at 700 ℃ with n（La）：n（Ni）：n（CA） of 2：1：3 exhibits the best activity and excellent stability as well as very low coke formation.
AbstractList The performance of La2NiO4 perovskite catalysts, prepared using a citric acid complexation method, for the steam reforming of ethanol was studied. The catalysts were characterized by X-ray diffractometry （XRD）, specific surface area measurements （BET）, thermogravimetric analysis （TGA） and scanning electron microscopy （SEM）. The experimental results show that the calcination temperature and thc amount of citric acid （CA） have a significant influence on the characteristics of the catalysts and their catalytic activity. Among the catalysts tested, the La2NiO4 catalyst calcined at 700 ℃ with n（La）：n（Ni）：n（CA） of 2：1：3 exhibits the best activity and excellent stability as well as very low coke formation.
Author 张利峰 王一平 黄群武
AuthorAffiliation School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
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Notes hydrogen; ethanol; perovskite-like oxides; La2NiO4
43-1239/TG
perovskite-like oxides
La2NiO4
O614.338
hydrogen
ethanol
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Snippet The performance of La2NiO4 perovskite catalysts, prepared using a citric acid complexation method, for the steam reforming of ethanol was studied. The...
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SubjectTerms K2NiF4型
La2NiO4
扫描电子显微镜
重整催化剂
钙钛矿氧化物
Title Preparation and properties of K2NiF4-type perovskite oxides La2NiO4 catalysts for steam reforming of ethanol
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