Tailoring performance of Bi(Ni0.50Ti0.50)O3–BiFeO3–Pb(Zr0.50Ti0.50)O3 ceramics via composition designing and sintering process improvement

Via composition designing and sintering condition tailoring, high-density pure perovskite structure x Bi(Ni 0.50 Ti 0.50 )O 3 –0.05BiFeO 3 –(0.95− x )Pb(Zr 0.50 Ti 0.50 )O 3 [ x BNT–0.05BF–(0.95− x )PZT, x = 0.19, 0.20, 0.21, 0.22, 0.23] ceramics were prepared by solid-state sintering method with ad...

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Published in	Bulletin of materials science Vol. 47; no. 2; p. 107
Main Authors	Wang, Shihao, Fang, Bijun, Chen, Zhihui, Lu, Xiaolong, Zhang, Shuai, Ding, Jianning
Format	Journal Article
Language	English
Published	Bangalore Indian Academy of Sciences 23.05.2024 Springer Nature B.V
Subjects	Ceramics Chemistry and Materials Science Composition Crystal structure Engineering High temperature Lead zirconate titanates Materials Science Perovskite structure Perovskites Phase transitions Piezoelectricity Point defects Raman spectroscopy Sintering Sintering aids Temperature Japan electrical performance Ti Pb(Zr BiFeO tolerance factor sintering aid Bi(Ni O
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Abstract	Via composition designing and sintering condition tailoring, high-density pure perovskite structure x Bi(Ni 0.50 Ti 0.50 )O 3 –0.05BiFeO 3 –(0.95− x )Pb(Zr 0.50 Ti 0.50 )O 3 [ x BNT–0.05BF–(0.95− x )PZT, x = 0.19, 0.20, 0.21, 0.22, 0.23] ceramics were prepared by solid-state sintering method with adding additional 0.5 wt% LiBO 2 sintering aid, whose sintering temperature was lower than that reported in literature. The x BNT–0.05BF–(0.95− x )PZT ceramics have mainly tetragonal structure confirmed by X-ray diffraction measurement and Raman spectroscopy, which is affected by composition and sintering condition. Broad dielectric peaks appear in all samples, and diffusive phase transition and dielectric frequency dispersion are obvious as well. The 0.20BNT–0.05BF–0.75PZT ceramics exhibit large piezoelectricity d 33 = 386 pC/N combined with rather high dielectric constant maximum temperature T m = 264°C, presenting enormous application potential in the high-temperature piezoelectric-related field.
AbstractList	Via composition designing and sintering condition tailoring, high-density pure perovskite structure x Bi(Ni 0.50 Ti 0.50 )O 3 –0.05BiFeO 3 –(0.95− x )Pb(Zr 0.50 Ti 0.50 )O 3 [ x BNT–0.05BF–(0.95− x )PZT, x = 0.19, 0.20, 0.21, 0.22, 0.23] ceramics were prepared by solid-state sintering method with adding additional 0.5 wt% LiBO 2 sintering aid, whose sintering temperature was lower than that reported in literature. The x BNT–0.05BF–(0.95− x )PZT ceramics have mainly tetragonal structure confirmed by X-ray diffraction measurement and Raman spectroscopy, which is affected by composition and sintering condition. Broad dielectric peaks appear in all samples, and diffusive phase transition and dielectric frequency dispersion are obvious as well. The 0.20BNT–0.05BF–0.75PZT ceramics exhibit large piezoelectricity d 33 = 386 pC/N combined with rather high dielectric constant maximum temperature T m = 264°C, presenting enormous application potential in the high-temperature piezoelectric-related field. Via composition designing and sintering condition tailoring, high-density pure perovskite structure xBi(Ni0.50Ti0.50)O3–0.05BiFeO3–(0.95−x)Pb(Zr0.50Ti0.50)O3 [xBNT–0.05BF–(0.95−x)PZT, x = 0.19, 0.20, 0.21, 0.22, 0.23] ceramics were prepared by solid-state sintering method with adding additional 0.5 wt% LiBO2 sintering aid, whose sintering temperature was lower than that reported in literature. The xBNT–0.05BF–(0.95−x)PZT ceramics have mainly tetragonal structure confirmed by X-ray diffraction measurement and Raman spectroscopy, which is affected by composition and sintering condition. Broad dielectric peaks appear in all samples, and diffusive phase transition and dielectric frequency dispersion are obvious as well. The 0.20BNT–0.05BF–0.75PZT ceramics exhibit large piezoelectricity d33 = 386 pC/N combined with rather high dielectric constant maximum temperature Tm = 264°C, presenting enormous application potential in the high-temperature piezoelectric-related field.
ArticleNumber	107
Author	Ding, Jianning Chen, Zhihui Zhang, Shuai Lu, Xiaolong Fang, Bijun Wang, Shihao
Author_xml	– sequence: 1 givenname: Shihao surname: Wang fullname: Wang, Shihao organization: School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Jiangsu Province Cultivation Base for State Key Laboratory of Photovoltaic Science and Technology, National Experimental Demonstration Center for Materials Science and Engineering, Changzhou University – sequence: 2 givenname: Bijun orcidid: 0000-0002-9510-9433 surname: Fang fullname: Fang, Bijun email: fangbj@cczu.edu.cn organization: School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Jiangsu Province Cultivation Base for State Key Laboratory of Photovoltaic Science and Technology, National Experimental Demonstration Center for Materials Science and Engineering, Changzhou University – sequence: 3 givenname: Zhihui surname: Chen fullname: Chen, Zhihui organization: School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Jiangsu Province Cultivation Base for State Key Laboratory of Photovoltaic Science and Technology, National Experimental Demonstration Center for Materials Science and Engineering, Changzhou University – sequence: 4 givenname: Xiaolong surname: Lu fullname: Lu, Xiaolong organization: School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Jiangsu Province Cultivation Base for State Key Laboratory of Photovoltaic Science and Technology, National Experimental Demonstration Center for Materials Science and Engineering, Changzhou University – sequence: 5 givenname: Shuai surname: Zhang fullname: Zhang, Shuai organization: School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Jiangsu Province Cultivation Base for State Key Laboratory of Photovoltaic Science and Technology, National Experimental Demonstration Center for Materials Science and Engineering, Changzhou University – sequence: 6 givenname: Jianning surname: Ding fullname: Ding, Jianning organization: School of Materials Science and Engineering, Jiangsu Collaborative Innovation Center of Photovolatic Science and Engineering, Jiangsu Province Cultivation Base for State Key Laboratory of Photovoltaic Science and Technology, National Experimental Demonstration Center for Materials Science and Engineering, Changzhou University, School of Mechanical Engineering, Yangzhou University
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Snippet	Via composition designing and sintering condition tailoring, high-density pure perovskite structure x Bi(Ni 0.50 Ti 0.50 )O 3 –0.05BiFeO 3 –(0.95− x )Pb(Zr... Via composition designing and sintering condition tailoring, high-density pure perovskite structure xBi(Ni0.50Ti0.50)O3–0.05BiFeO3–(0.95−x)Pb(Zr0.50Ti0.50)O3...
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SubjectTerms	Ceramics Chemistry and Materials Science Composition Crystal structure Engineering High temperature Lead zirconate titanates Materials Science Perovskite structure Perovskites Phase transitions Piezoelectricity Point defects Raman spectroscopy Sintering Sintering aids Temperature
Title	Tailoring performance of Bi(Ni0.50Ti0.50)O3–BiFeO3–Pb(Zr0.50Ti0.50)O3 ceramics via composition designing and sintering process improvement
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