Radiation induced grafting of amphiphilic double poly(ionic liquid) copolymer onto silica surface for the removal of ReO4− as analogue of TcO4
Amphiphilic double poly(imidazole ionic liquid) grafted silica (SMIL-n) was prepared by radiation grafting of hydrophilic 1-vinyl-3-ethylimidazolium bromide and hydrophobic 1-vinyl-3-octylimidazolium bromide at different ratio onto silica. The adsorption behavior of SMIL-n was investigated. The adso...
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| Published in | Journal of radioanalytical and nuclear chemistry Vol. 332; no. 6; pp. 1869 - 1881 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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01.06.2023
Springer Nature B.V |
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| Abstract | Amphiphilic double poly(imidazole ionic liquid) grafted silica (SMIL-n) was prepared by radiation grafting of hydrophilic 1-vinyl-3-ethylimidazolium bromide and hydrophobic 1-vinyl-3-octylimidazolium bromide at different ratio onto silica. The adsorption behavior of SMIL-n was investigated. The adsorption equilibrium could reach less than 45 min, and their adsorption capacity were 152–171 mg/g obtained from Langmuir model. The selectivity of SMIL-n to ReO
4
−
increased with the increasing content of hydrophobic ionic liquid. SMIL-n displayed good reusability, excellent acid resistance and irradiation resistance. Particularly, SMIL-n showed promising for ReO
4
−
uptake from simulated contaminated Beishan groundwater and radioactive wastewater. |
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| AbstractList | Amphiphilic double poly(imidazole ionic liquid) grafted silica (SMIL-n) was prepared by radiation grafting of hydrophilic 1-vinyl-3-ethylimidazolium bromide and hydrophobic 1-vinyl-3-octylimidazolium bromide at different ratio onto silica. The adsorption behavior of SMIL-n was investigated. The adsorption equilibrium could reach less than 45 min, and their adsorption capacity were 152–171 mg/g obtained from Langmuir model. The selectivity of SMIL-n to ReO4− increased with the increasing content of hydrophobic ionic liquid. SMIL-n displayed good reusability, excellent acid resistance and irradiation resistance. Particularly, SMIL-n showed promising for ReO4− uptake from simulated contaminated Beishan groundwater and radioactive wastewater. Amphiphilic double poly(imidazole ionic liquid) grafted silica (SMIL-n) was prepared by radiation grafting of hydrophilic 1-vinyl-3-ethylimidazolium bromide and hydrophobic 1-vinyl-3-octylimidazolium bromide at different ratio onto silica. The adsorption behavior of SMIL-n was investigated. The adsorption equilibrium could reach less than 45 min, and their adsorption capacity were 152–171 mg/g obtained from Langmuir model. The selectivity of SMIL-n to ReO 4 − increased with the increasing content of hydrophobic ionic liquid. SMIL-n displayed good reusability, excellent acid resistance and irradiation resistance. Particularly, SMIL-n showed promising for ReO 4 − uptake from simulated contaminated Beishan groundwater and radioactive wastewater. |
| Author | Zhang, Manman Du, Jifu Zhang, Na Yang, Miao Bao, Qiburi Zhao, Long Dong, Zhen |
| Author_xml | – sequence: 1 givenname: Na surname: Zhang fullname: Zhang, Na organization: School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology – sequence: 2 givenname: Miao surname: Yang fullname: Yang, Miao organization: School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology – sequence: 3 givenname: Manman surname: Zhang fullname: Zhang, Manman organization: State Key Laboratory of Advanced Electromagnetic Engineering and Technology, School of Electrical and Electronic Engineering, Huazhong University of Science and Technology – sequence: 4 givenname: Jifu surname: Du fullname: Du, Jifu organization: School of Nuclear Technology and Chemistry & Biology, Hubei University of Science and Technology – sequence: 5 givenname: Qiburi surname: Bao fullname: Bao, Qiburi organization: School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology – sequence: 6 givenname: Long orcidid: 0000-0002-6126-2210 surname: Zhao fullname: Zhao, Long email: ryuuchou@hotmail.com, zhaolong@hust.edu.cn organization: State Key Laboratory of Advanced Electromagnetic Engineering and Technology, School of Electrical and Electronic Engineering, Huazhong University of Science and Technology – sequence: 7 givenname: Zhen surname: Dong fullname: Dong, Zhen email: bbcczhen@126.com organization: School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology |
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| Keywords | Removal Radiation grafting TcO Poly(ionic liquid) ReO Silica |
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| Snippet | Amphiphilic double poly(imidazole ionic liquid) grafted silica (SMIL-n) was prepared by radiation grafting of hydrophilic 1-vinyl-3-ethylimidazolium bromide... |
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| SubjectTerms | Acid resistance Adsorption Chemistry Chemistry and Materials Science Copolymers Diagnostic Radiology Graft copolymers Groundwater Hadrons Heavy Ions Hydrophobicity Imidazole Inorganic Chemistry Ionic liquids Nuclear Chemistry Nuclear Physics Physical Chemistry Radiation effects Silicon dioxide Wastewater |
| Title | Radiation induced grafting of amphiphilic double poly(ionic liquid) copolymer onto silica surface for the removal of ReO4− as analogue of TcO4 |
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