Preparation of metal-organic framework-derived Fe-CoZnCN-T nanocomposites and their microwave absorption performance
•When the Fe-CoZnCN-T composites are mixed in solid paraffin with 30 wt% filler content, Fe-CoZnCN-700 exhibits good impedance matching ability and microwave loss ability due to the appropriate permittivity and permeability, thus exhibiting excellent microwave absorption performance.•The RLmin reach...
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| Published in | Materials research bulletin Vol. 190; p. 113517 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.10.2025
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| Abstract | •When the Fe-CoZnCN-T composites are mixed in solid paraffin with 30 wt% filler content, Fe-CoZnCN-700 exhibits good impedance matching ability and microwave loss ability due to the appropriate permittivity and permeability, thus exhibiting excellent microwave absorption performance.•The RLmin reaches −61.95 dB at the frequency of 15.20 GHz, the effective absorption bandwidth is greater than 5.42 GHz, and the matching thickness is only 2 mm.
With advancing technology, electromagnetic wave applications are expanding, yet associated radiation increasingly threatens precision instruments and human health, necessitating high-performance absorption materials. Metal-organic frameworks (MOFs) emerge as promising candidates due to their lightweight design, structural tunability, and porosity. This study synthesized three Fe-CoZnCN-T composites through Fc-ZIF-8@CoZn-ZIF pyrolysis at 700 °C, 800 °C, and 900 °C. Structural characterization via TEM/XRD/VSM/Raman revealed optimized dielectric/magnetic properties in Fe-CoZnCN-700. When blended with paraffin (30 wt%), this composite demonstrated exceptional impedance matching and wave dissipation. At 2 mm thickness, Fe-CoZnCN-700 achieved a minimum reflection loss of -61.95 dB at 15.20 GHz with >5.42 GHz effective bandwidth, outperforming counterparts processed at higher temperatures. The balanced permittivity-permeability synergy in 700 °C-derived material underscores its potential for ultrathin microwave absorbers in GHz-range applications.
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| AbstractList | •When the Fe-CoZnCN-T composites are mixed in solid paraffin with 30 wt% filler content, Fe-CoZnCN-700 exhibits good impedance matching ability and microwave loss ability due to the appropriate permittivity and permeability, thus exhibiting excellent microwave absorption performance.•The RLmin reaches −61.95 dB at the frequency of 15.20 GHz, the effective absorption bandwidth is greater than 5.42 GHz, and the matching thickness is only 2 mm.
With advancing technology, electromagnetic wave applications are expanding, yet associated radiation increasingly threatens precision instruments and human health, necessitating high-performance absorption materials. Metal-organic frameworks (MOFs) emerge as promising candidates due to their lightweight design, structural tunability, and porosity. This study synthesized three Fe-CoZnCN-T composites through Fc-ZIF-8@CoZn-ZIF pyrolysis at 700 °C, 800 °C, and 900 °C. Structural characterization via TEM/XRD/VSM/Raman revealed optimized dielectric/magnetic properties in Fe-CoZnCN-700. When blended with paraffin (30 wt%), this composite demonstrated exceptional impedance matching and wave dissipation. At 2 mm thickness, Fe-CoZnCN-700 achieved a minimum reflection loss of -61.95 dB at 15.20 GHz with >5.42 GHz effective bandwidth, outperforming counterparts processed at higher temperatures. The balanced permittivity-permeability synergy in 700 °C-derived material underscores its potential for ultrathin microwave absorbers in GHz-range applications.
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| ArticleNumber | 113517 |
| Author | Lian, Aizhen Ju, Pengfei Yu, Haojie Zang, Xusheng Wang, Li Liang, Hongyu Nan, Bohua Ren, Shuning |
| Author_xml | – sequence: 1 givenname: Shuning surname: Ren fullname: Ren, Shuning organization: State Key Laboratory of Chemical Engineering and Low-Carbon Technology, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310058, PR China – sequence: 2 givenname: Pengfei surname: Ju fullname: Ju, Pengfei organization: Shanghai Aerospace Equipment manufacturer Co., Ltd., Shanghai 200240, PR China – sequence: 3 givenname: Haojie orcidid: 0000-0002-7405-7881 surname: Yu fullname: Yu, Haojie email: hjyu@zju.edu.cn organization: State Key Laboratory of Chemical Engineering and Low-Carbon Technology, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310058, PR China – sequence: 4 givenname: Bohua surname: Nan fullname: Nan, Bohua email: nanbohua5@163.com organization: Shanghai Aerospace Equipment manufacturer Co., Ltd., Shanghai 200240, PR China – sequence: 5 givenname: Li surname: Wang fullname: Wang, Li organization: State Key Laboratory of Chemical Engineering and Low-Carbon Technology, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310058, PR China – sequence: 6 givenname: Aizhen surname: Lian fullname: Lian, Aizhen organization: Shanghai Aerospace Equipment manufacturer Co., Ltd., Shanghai 200240, PR China – sequence: 7 givenname: Xusheng surname: Zang fullname: Zang, Xusheng organization: Shanghai Aerospace Equipment manufacturer Co., Ltd., Shanghai 200240, PR China – sequence: 8 givenname: Hongyu surname: Liang fullname: Liang, Hongyu organization: Shanghai Aerospace Equipment manufacturer Co., Ltd., Shanghai 200240, PR China |
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| SubjectTerms | Ferrocene Metal-organic framework Microwave absorption performance |
| Title | Preparation of metal-organic framework-derived Fe-CoZnCN-T nanocomposites and their microwave absorption performance |
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