Performance, limitation, and opportunities of acid-resistant nanofiltration membranes for industrial wastewater treatment

Various industrial activities generate highly acidic wastewaters, posing a particular concern due to their large volume, environmental impact, and limited disposal options. Nanofiltration (NF) has the potential to provide energy-, cost-, and space-effective solutions for wastewater treatment at indu...

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Published inJournal of membrane science Vol. 666; p. 121142
Main Authors Lee, Jaewon, Shin, Yeojin, Boo, Chanhee, Hong, Seungkwan
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.01.2023
Subjects
acid tolerance
Acid-resistant
environmental impact
hydrolysis
industrial wastewater treatment
Industrial wastewaters
Nanofiltration
polyamides
Reverse osmosis
surveys
wastewater
Industrial wastewaters
Nanofiltration
Reverse osmosis
Acid-resistant
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Abstract Various industrial activities generate highly acidic wastewaters, posing a particular concern due to their large volume, environmental impact, and limited disposal options. Nanofiltration (NF) has the potential to provide energy-, cost-, and space-effective solutions for wastewater treatment at industrial sites. However, conventional thin-film composite NF membranes degrade under acid exposures, largely limiting their applications in industrial wastewater treatment. Development of chemically robust NF membranes that are stable during operation with highly acidic feed streams has been a subject of active research and industrial interest. In this critical review, we first provide a comprehensive survey for the broad spectrum of industrial processes that yield acidic wastewaters. We then conduct in-depth analyses for short- and long-term rejection performances and stabilities of commercial NF membranes, especially under low solution pH conditions. Several key mechanisms responsible for the degradation of semi-aromatic polyamide networks by acid-catalyzed hydrolysis are discussed to highlight the limitation of commercially available NF membranes. Finally, we describe a wide variety of technical strategies to fabricate acid-resistant NF membranes, focusing on the key mechanism to enhance acid stability. We conclude by providing useful insights to guide the future directions for academic studies as well as industrial applications of acid-resistant NF membranes. [Display omitted] •Performances of NF/RO membranes under acidic conditions were analyzed.•Fundamental mechanisms of acid-catalyzed degradation were described.•Recent fabrication strategies for acid-resistance NF membranes were discussed.•Future directions for acid-resistance NF membrane applications were proposed.
AbstractList Various industrial activities generate highly acidic wastewaters, posing a particular concern due to their large volume, environmental impact, and limited disposal options. Nanofiltration (NF) has the potential to provide energy-, cost-, and space-effective solutions for wastewater treatment at industrial sites. However, conventional thin-film composite NF membranes degrade under acid exposures, largely limiting their applications in industrial wastewater treatment. Development of chemically robust NF membranes that are stable during operation with highly acidic feed streams has been a subject of active research and industrial interest. In this critical review, we first provide a comprehensive survey for the broad spectrum of industrial processes that yield acidic wastewaters. We then conduct in-depth analyses for short- and long-term rejection performances and stabilities of commercial NF membranes, especially under low solution pH conditions. Several key mechanisms responsible for the degradation of semi-aromatic polyamide networks by acid-catalyzed hydrolysis are discussed to highlight the limitation of commercially available NF membranes. Finally, we describe a wide variety of technical strategies to fabricate acid-resistant NF membranes, focusing on the key mechanism to enhance acid stability. We conclude by providing useful insights to guide the future directions for academic studies as well as industrial applications of acid-resistant NF membranes.
Various industrial activities generate highly acidic wastewaters, posing a particular concern due to their large volume, environmental impact, and limited disposal options. Nanofiltration (NF) has the potential to provide energy-, cost-, and space-effective solutions for wastewater treatment at industrial sites. However, conventional thin-film composite NF membranes degrade under acid exposures, largely limiting their applications in industrial wastewater treatment. Development of chemically robust NF membranes that are stable during operation with highly acidic feed streams has been a subject of active research and industrial interest. In this critical review, we first provide a comprehensive survey for the broad spectrum of industrial processes that yield acidic wastewaters. We then conduct in-depth analyses for short- and long-term rejection performances and stabilities of commercial NF membranes, especially under low solution pH conditions. Several key mechanisms responsible for the degradation of semi-aromatic polyamide networks by acid-catalyzed hydrolysis are discussed to highlight the limitation of commercially available NF membranes. Finally, we describe a wide variety of technical strategies to fabricate acid-resistant NF membranes, focusing on the key mechanism to enhance acid stability. We conclude by providing useful insights to guide the future directions for academic studies as well as industrial applications of acid-resistant NF membranes. [Display omitted] •Performances of NF/RO membranes under acidic conditions were analyzed.•Fundamental mechanisms of acid-catalyzed degradation were described.•Recent fabrication strategies for acid-resistance NF membranes were discussed.•Future directions for acid-resistance NF membrane applications were proposed.
ArticleNumber 121142
Author Boo, Chanhee
Shin, Yeojin
Lee, Jaewon
Hong, Seungkwan
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  orcidid: 0000-0001-8920-8964
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  organization: Center for Water Cycle Research, Climate and Environmental Research Institute, Korea Institute of Science and Technology (KIST), Seoul, 02792, Republic of Korea
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  organization: School of Civil, Environmental and Architectural Engineering, Korea University, 145 Anam-ro, Seongbuk-gu, Seoul, 02841, Republic of Korea
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Snippet Various industrial activities generate highly acidic wastewaters, posing a particular concern due to their large volume, environmental impact, and limited...
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elsevier
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StartPage 121142
SubjectTerms acid tolerance
Acid-resistant
environmental impact
hydrolysis
industrial wastewater treatment
Industrial wastewaters
Nanofiltration
polyamides
Reverse osmosis
surveys
wastewater
Title Performance, limitation, and opportunities of acid-resistant nanofiltration membranes for industrial wastewater treatment
URI https://dx.doi.org/10.1016/j.memsci.2022.121142
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