A Molecularly Engineered Zwitterionic Hydrogel with Strengthened Anti‐Polyelectrolyte Effect: from High‐Rate Solar Desalination to Efficient Electricity Generation
Polyzwitterionic hydrogel is an emerging material for solar‐driven water evaporation in saline environment due to its special anti‐polyelectrolyte effect, which is a promising approach to co‐generation of freshwater and electricity. However, the molecular impact on anti‐polyelectrolyte effect remain...
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| Published in | Advanced functional materials Vol. 33; no. 43 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Hoboken
Wiley Subscription Services, Inc
18.10.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Polyzwitterionic hydrogel is an emerging material for solar‐driven water evaporation in saline environment due to its special anti‐polyelectrolyte effect, which is a promising approach to co‐generation of freshwater and electricity. However, the molecular impact on anti‐polyelectrolyte effect remains unclear, let alone to optimize the zwitterionic structure to promote water evaporation efficiency in high‐salinity brine. Herein, a molecularly engineered zwitterionic hydrogel is developed and the incorporated phenyl‐methylene‐imidazole motif greatly enhances the salt binding ability and strengthens anti‐polyelectrolyte effect, leading to boosted hydration, improved salt tolerance, ultra‐low evaporation enthalpy (almost half of traditional zwitterionic gel), and durable anti‐microbial ability in brine. Besides, gradient solar‐thermal network is penetrated to optimize water transport channel and heat confinement. The gel exhibits excellent evaporation rate of 3.17 kg m
−2
h
−1
in seawater, which is 1.6 times of that in water and such high efficiency could be maintained during 8 h continuous desalination, demonstrating outstanding salt tolerance. The high flux of ion stream can generate considerable voltage (321.3 mV) simultaneously. This work will bring new insights to the understanding of anti‐polyelectrolyte effect at molecular level and promote materials design for saline water evaporation. |
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| AbstractList | Polyzwitterionic hydrogel is an emerging material for solar‐driven water evaporation in saline environment due to its special anti‐polyelectrolyte effect, which is a promising approach to co‐generation of freshwater and electricity. However, the molecular impact on anti‐polyelectrolyte effect remains unclear, let alone to optimize the zwitterionic structure to promote water evaporation efficiency in high‐salinity brine. Herein, a molecularly engineered zwitterionic hydrogel is developed and the incorporated phenyl‐methylene‐imidazole motif greatly enhances the salt binding ability and strengthens anti‐polyelectrolyte effect, leading to boosted hydration, improved salt tolerance, ultra‐low evaporation enthalpy (almost half of traditional zwitterionic gel), and durable anti‐microbial ability in brine. Besides, gradient solar‐thermal network is penetrated to optimize water transport channel and heat confinement. The gel exhibits excellent evaporation rate of 3.17 kg m−2 h−1 in seawater, which is 1.6 times of that in water and such high efficiency could be maintained during 8 h continuous desalination, demonstrating outstanding salt tolerance. The high flux of ion stream can generate considerable voltage (321.3 mV) simultaneously. This work will bring new insights to the understanding of anti‐polyelectrolyte effect at molecular level and promote materials design for saline water evaporation. Polyzwitterionic hydrogel is an emerging material for solar‐driven water evaporation in saline environment due to its special anti‐polyelectrolyte effect, which is a promising approach to co‐generation of freshwater and electricity. However, the molecular impact on anti‐polyelectrolyte effect remains unclear, let alone to optimize the zwitterionic structure to promote water evaporation efficiency in high‐salinity brine. Herein, a molecularly engineered zwitterionic hydrogel is developed and the incorporated phenyl‐methylene‐imidazole motif greatly enhances the salt binding ability and strengthens anti‐polyelectrolyte effect, leading to boosted hydration, improved salt tolerance, ultra‐low evaporation enthalpy (almost half of traditional zwitterionic gel), and durable anti‐microbial ability in brine. Besides, gradient solar‐thermal network is penetrated to optimize water transport channel and heat confinement. The gel exhibits excellent evaporation rate of 3.17 kg m −2 h −1 in seawater, which is 1.6 times of that in water and such high efficiency could be maintained during 8 h continuous desalination, demonstrating outstanding salt tolerance. The high flux of ion stream can generate considerable voltage (321.3 mV) simultaneously. This work will bring new insights to the understanding of anti‐polyelectrolyte effect at molecular level and promote materials design for saline water evaporation. |
| Author | Zhou, Jiahui Fu, Jimin Zhang, Dong Zheng, Si Yu Zhu, Fengbo Yang, Jintao Wang, Shuaibing Lin, Ji Si, Mengjie |
| Author_xml | – sequence: 1 givenname: Si Yu orcidid: 0000-0001-7602-6731 surname: Zheng fullname: Zheng, Si Yu organization: Zhejiang Key Laboratory of Plastic Modification and Processing Technology College of Materials Science & Engineering Zhejiang University of Technology Hangzhou 310014 P. R. China – sequence: 2 givenname: Jiahui surname: Zhou fullname: Zhou, Jiahui organization: Zhejiang Key Laboratory of Plastic Modification and Processing Technology College of Materials Science & Engineering Zhejiang University of Technology Hangzhou 310014 P. R. China – sequence: 3 givenname: Mengjie surname: Si fullname: Si, Mengjie organization: Zhejiang Key Laboratory of Plastic Modification and Processing Technology College of Materials Science & Engineering Zhejiang University of Technology Hangzhou 310014 P. R. China – sequence: 4 givenname: Shuaibing surname: Wang fullname: Wang, Shuaibing organization: Zhejiang Key Laboratory of Plastic Modification and Processing Technology College of Materials Science & Engineering Zhejiang University of Technology Hangzhou 310014 P. R. China – sequence: 5 givenname: Fengbo surname: Zhu fullname: Zhu, Fengbo organization: College of Materials Science & Engineering Taiyuan University of Technology Taiyuan 030024 P. R. China – sequence: 6 givenname: Ji surname: Lin fullname: Lin, Ji organization: School of Mechanical Engineering & Mechanics Ningbo University Ningbo 315211 P. R. China – sequence: 7 givenname: Jimin orcidid: 0000-0003-2591-9198 surname: Fu fullname: Fu, Jimin organization: Research Institute for Intelligent Wearable Systems School of Fashion and Textiles Hong Kong Polytechnic University Hong Kong SAR 999077 P. R. China – sequence: 8 givenname: Dong orcidid: 0000-0001-7002-7661 surname: Zhang fullname: Zhang, Dong organization: The Wallace H. Coulter Department of Biomedical Engineering Georgia Institute of Technology and Emory University Atlanta GA 30332 USA – sequence: 9 givenname: Jintao orcidid: 0000-0002-3133-1246 surname: Yang fullname: Yang, Jintao organization: Zhejiang Key Laboratory of Plastic Modification and Processing Technology College of Materials Science & Engineering Zhejiang University of Technology Hangzhou 310014 P. R. China |
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| Snippet | Polyzwitterionic hydrogel is an emerging material for solar‐driven water evaporation in saline environment due to its special anti‐polyelectrolyte effect,... |
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| SubjectTerms | Brines Desalination Electricity Enthalpy Evaporation rate Hydrogels Imidazole Materials science Microorganisms Polyelectrolytes Saline environments Saline water Seawater Zwitterions |
| Title | A Molecularly Engineered Zwitterionic Hydrogel with Strengthened Anti‐Polyelectrolyte Effect: from High‐Rate Solar Desalination to Efficient Electricity Generation |
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