Toward Flexible Embodied Energy: Scale‐Inspired Overlapping Lithium‐Ion Batteries with High‐Energy‐Density and Variable Stiffness
High performance flexible batteries are essential ingredients for flexible devices. However, general isolated flexible batteries face critical challenges in developing multifunctional embodied energy systems, owing to the lack of integrative design. Herein, inspired by scales in creatures, overlappi...
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| Published in | Advanced functional materials Vol. 33; no. 37 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
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12.09.2023
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| Abstract | High performance flexible batteries are essential ingredients for flexible devices. However, general isolated flexible batteries face critical challenges in developing multifunctional embodied energy systems, owing to the lack of integrative design. Herein, inspired by scales in creatures, overlapping flexible lithium‐ion batteries (FLIBs) consisting of energy storage scales and connections using LiNi
0.5
Co
0.2
Mn
0.3
O
2
(NCM523) and graphite electrodes are presented. The scale‐dermis structure ensures a high energy density of 374.4 Wh L
−1
as well as a high capacity retention of 93.2% after 200 charge/discharge cycles and 40 000 bending times. A variable stiffness property is revealed that can be controlled by battery configurations and deformation modes. Furthermore, the overlapping FLIBs can be housed directly into the architecture of several flexible devices, such as robots and grippers, allowing to create multifunctionalities that go far beyond energy storage and include load‐bearing and variable flexibility. This study broadens the versatility of FLIBs toward energy storage structure engineering of flexible devices. |
|---|---|
| AbstractList | High performance flexible batteries are essential ingredients for flexible devices. However, general isolated flexible batteries face critical challenges in developing multifunctional embodied energy systems, owing to the lack of integrative design. Herein, inspired by scales in creatures, overlapping flexible lithium‐ion batteries (FLIBs) consisting of energy storage scales and connections using LiNi0.5Co0.2Mn0.3O2 (NCM523) and graphite electrodes are presented. The scale‐dermis structure ensures a high energy density of 374.4 Wh L−1 as well as a high capacity retention of 93.2% after 200 charge/discharge cycles and 40 000 bending times. A variable stiffness property is revealed that can be controlled by battery configurations and deformation modes. Furthermore, the overlapping FLIBs can be housed directly into the architecture of several flexible devices, such as robots and grippers, allowing to create multifunctionalities that go far beyond energy storage and include load‐bearing and variable flexibility. This study broadens the versatility of FLIBs toward energy storage structure engineering of flexible devices. High performance flexible batteries are essential ingredients for flexible devices. However, general isolated flexible batteries face critical challenges in developing multifunctional embodied energy systems, owing to the lack of integrative design. Herein, inspired by scales in creatures, overlapping flexible lithium‐ion batteries (FLIBs) consisting of energy storage scales and connections using LiNi 0.5 Co 0.2 Mn 0.3 O 2 (NCM523) and graphite electrodes are presented. The scale‐dermis structure ensures a high energy density of 374.4 Wh L −1 as well as a high capacity retention of 93.2% after 200 charge/discharge cycles and 40 000 bending times. A variable stiffness property is revealed that can be controlled by battery configurations and deformation modes. Furthermore, the overlapping FLIBs can be housed directly into the architecture of several flexible devices, such as robots and grippers, allowing to create multifunctionalities that go far beyond energy storage and include load‐bearing and variable flexibility. This study broadens the versatility of FLIBs toward energy storage structure engineering of flexible devices. |
| Author | Bao, Yinhua Zhao, Zeang Zhang, Xing‐Yu Liu, Haojie Liu, Guanzhong Ma, Xu Song, Wei‐Li |
| Author_xml | – sequence: 1 givenname: Yinhua orcidid: 0000-0003-2462-5219 surname: Bao fullname: Bao, Yinhua organization: Shanghai Institute of Applied Mathematics and Mechanics School of Mechanics and Engineering Science Shanghai Key Laboratory of Mechanics in Energy Engineering Shanghai University Shanghai 200444 China, Shanghai Frontier Science Center of Mechanoinformatics Shanghai 200444 China – sequence: 2 givenname: Haojie surname: Liu fullname: Liu, Haojie organization: Shanghai Institute of Applied Mathematics and Mechanics School of Mechanics and Engineering Science Shanghai Key Laboratory of Mechanics in Energy Engineering Shanghai University Shanghai 200444 China – sequence: 3 givenname: Zeang surname: Zhao fullname: Zhao, Zeang organization: Institute of Advanced Structure Technology Beijing Institute of Technology Beijing 100081 China – sequence: 4 givenname: Xu surname: Ma fullname: Ma, Xu organization: Shanghai Institute of Applied Mathematics and Mechanics School of Mechanics and Engineering Science Shanghai Key Laboratory of Mechanics in Energy Engineering Shanghai University Shanghai 200444 China – sequence: 5 givenname: Xing‐Yu surname: Zhang fullname: Zhang, Xing‐Yu organization: State Key Laboratory of Mechanics and Control for Aerospace Structures College of Aerospace Engineering Nanjing University of Aeronautics and Astronautics Nanjing 210016 China – sequence: 6 givenname: Guanzhong surname: Liu fullname: Liu, Guanzhong organization: Shanghai Institute of Applied Mathematics and Mechanics School of Mechanics and Engineering Science Shanghai Key Laboratory of Mechanics in Energy Engineering Shanghai University Shanghai 200444 China – sequence: 7 givenname: Wei‐Li surname: Song fullname: Song, Wei‐Li organization: Institute of Advanced Structure Technology Beijing Institute of Technology Beijing 100081 China |
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| Title | Toward Flexible Embodied Energy: Scale‐Inspired Overlapping Lithium‐Ion Batteries with High‐Energy‐Density and Variable Stiffness |
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