3D hierarchical microspheres constructed by ultrathin MoS2-C nanosheets as high-performance anode material for sodium-ion batteries
MoS2/C composites are considered to have great application potential in sodium-ion batteries (SIBs). It is a challenging and meaningful subject that developing high-performance anode materials via combining MoS2 and carbon effectively to give free rein to their advantages in sodium ion storage. In t...
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| Published in | Journal of energy chemistry Vol. 49; pp. 307 - 315 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.10.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | MoS2/C composites are considered to have great application potential in sodium-ion batteries (SIBs). It is a challenging and meaningful subject that developing high-performance anode materials via combining MoS2 and carbon effectively to give free rein to their advantages in sodium ion storage. In this work, a novel MoS2-C material was designed by using cellulose nanocrystals (CNCs) as low-cost and green carbon source. 3D hierarchical microspheres (200–250 nm) constructed by ultrathin MoS2-C nanosheets were synthesized by synchronizing the pre-carbonization of CNCs with the formation of MoS2 in hydrothermal reaction and subsequent pyrolysis process. It is found that the ultrathin MoS2-C nanosheets were composed of CNCs-derived short-range ordered carbon and few-layered MoS2. Benefiting from the unique structure and robust combination of MoS2 and CNCs-derived carbon, the ultrathin MoS2-C nanosheets composite was proved to have excellent cycling stability and superior rate performance in sodium-ion half-cell test and have high first reversible specific capacity of 397.9 mAh/g in full-cell test. This work provides a significant and effective pathway to prepare MoS2-C materials with excellent electrochemical performance for the application in large-scale energy storage systems.
Three-dimensional MoS2-C microspheres composed of biomass cellulose nanocrystals (CNCs) derived carbon and few-layered MoS2 nanosheets were constructed, which have excellent cycling stability and superior rate performance in sodium-ion half/full batteries. [Display omitted] |
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| AbstractList | MoS2/C composites are considered to have great application potential in sodium-ion batteries (SIBs). It is a challenging and meaningful subject that developing high-performance anode materials via combining MoS2 and carbon effectively to give free rein to their advantages in sodium ion storage. In this work, a novel MoS2-C material was designed by using cellulose nanocrystals (CNCs) as low-cost and green carbon source. 3D hierarchical microspheres (200–250 nm) constructed by ultrathin MoS2-C nanosheets were synthesized by synchronizing the pre-carbonization of CNCs with the formation of MoS2 in hydrothermal reaction and subsequent pyrolysis process. It is found that the ultrathin MoS2-C nanosheets were composed of CNCs-derived short-range ordered carbon and few-layered MoS2. Benefiting from the unique structure and robust combination of MoS2 and CNCs-derived carbon, the ultrathin MoS2-C nanosheets composite was proved to have excellent cycling stability and superior rate performance in sodium-ion half-cell test and have high first reversible specific capacity of 397.9 mAh/g in full-cell test. This work provides a significant and effective pathway to prepare MoS2-C materials with excellent electrochemical performance for the application in large-scale energy storage systems.
Three-dimensional MoS2-C microspheres composed of biomass cellulose nanocrystals (CNCs) derived carbon and few-layered MoS2 nanosheets were constructed, which have excellent cycling stability and superior rate performance in sodium-ion half/full batteries. [Display omitted] |
| Author | Li, Songlin Huang, Zhongyuan Hou, Teng Kuang, Yafei Zhang, Wenlong Wang, Chuqing Li, Huanxin Yan, Zhanheng Zhou, Haihui |
| Author_xml | – sequence: 1 givenname: Wenlong surname: Zhang fullname: Zhang, Wenlong organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 2 givenname: Haihui surname: Zhou fullname: Zhou, Haihui email: haihuizh@163.com organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 3 givenname: Zhongyuan surname: Huang fullname: Huang, Zhongyuan email: zhongyhuang@hnu.edu.cn organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 4 givenname: Songlin surname: Li fullname: Li, Songlin email: lisl@csu.edu.cn organization: State Key Laboratory of Powder Metallurgy, Central South University, Changsha 410083, Hunan, China – sequence: 5 givenname: Chuqing surname: Wang fullname: Wang, Chuqing organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 6 givenname: Huanxin surname: Li fullname: Li, Huanxin organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 7 givenname: Zhanheng surname: Yan fullname: Yan, Zhanheng organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 8 givenname: Teng surname: Hou fullname: Hou, Teng organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China – sequence: 9 givenname: Yafei surname: Kuang fullname: Kuang, Yafei email: yafeik@163.com organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, Hunan, China |
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| Keywords | Anode material MoS2-C nanosheets Cellulose nanocrystals Sodium-ion batteries Hierarchical microspheres |
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| Snippet | MoS2/C composites are considered to have great application potential in sodium-ion batteries (SIBs). It is a challenging and meaningful subject that developing... |
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| SubjectTerms | Anode material Cellulose nanocrystals Hierarchical microspheres MoS2-C nanosheets Sodium-ion batteries |
| Title | 3D hierarchical microspheres constructed by ultrathin MoS2-C nanosheets as high-performance anode material for sodium-ion batteries |
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