Development and performance of graphene oxide reinforced LDPE nanocomposite polymers for 3D printing
Abstract This study evaluated the mechanical properties and the chemical and thermal characteristics of low-density polyethylene (LDPE) nanocomposites reinforced with graphene oxide for manufacturing via 3D printing. LDPE nanocomposites with different graphene oxide (GO) loadings (0.5% and 1.5%) wer...
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| Published in | REM - International Engineering Journal Vol. 77; no. 2 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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2024
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| Abstract | Abstract This study evaluated the mechanical properties and the chemical and thermal characteristics of low-density polyethylene (LDPE) nanocomposites reinforced with graphene oxide for manufacturing via 3D printing. LDPE nanocomposites with different graphene oxide (GO) loadings (0.5% and 1.5%) were processed by a single-screw extruder. To characterize the pre-injected material, Fourier transform infrared spectroscopy (FTIR) and thermal characterization with thermogravimetry (TGA) were used. The injected material was also characterized with mechanical impact and traction tests. The results showed that incorporating GO into the polymeric matrix added hydroxyl groups to the matrix structure, with a 39.13% increase in Young's modulus for LDPE-1.5%wtGO samples. Mechanical tests of 3D printed samples showed that, with an increase in the amount of GO in the polymer matrix, the composite loses ductility, enabling its use in 3D printing technologies and thus encouraging new studies on printed materials for various applications. |
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| AbstractList | Abstract This study evaluated the mechanical properties and the chemical and thermal characteristics of low-density polyethylene (LDPE) nanocomposites reinforced with graphene oxide for manufacturing via 3D printing. LDPE nanocomposites with different graphene oxide (GO) loadings (0.5% and 1.5%) were processed by a single-screw extruder. To characterize the pre-injected material, Fourier transform infrared spectroscopy (FTIR) and thermal characterization with thermogravimetry (TGA) were used. The injected material was also characterized with mechanical impact and traction tests. The results showed that incorporating GO into the polymeric matrix added hydroxyl groups to the matrix structure, with a 39.13% increase in Young's modulus for LDPE-1.5%wtGO samples. Mechanical tests of 3D printed samples showed that, with an increase in the amount of GO in the polymer matrix, the composite loses ductility, enabling its use in 3D printing technologies and thus encouraging new studies on printed materials for various applications. |
| Author | Gonçalves, Rodolfo Luiz Prazeres Tegon, Caroline C. Massi, Marcos Oliveira, Andressa A. Soares, Marcelo M. Silva, Bryan M. M. Couto, Antonio Augusto |
| AuthorAffiliation | Universidade Presbiteriana Mackenzie |
| AuthorAffiliation_xml | – name: Universidade Presbiteriana Mackenzie |
| Author_xml | – sequence: 1 givenname: Bryan M. M. orcidid: 0000-0002-7815-569X surname: Silva fullname: Silva, Bryan M. M. organization: Universidade Presbiteriana Mackenzie, Brasil – sequence: 2 givenname: Caroline C. orcidid: 0000-0001-5155-2698 surname: Tegon fullname: Tegon, Caroline C. organization: Universidade Presbiteriana Mackenzie, Brasil – sequence: 3 givenname: Marcelo M. orcidid: 0000-0001-7143-2255 surname: Soares fullname: Soares, Marcelo M. organization: Universidade Presbiteriana Mackenzie, Brasil – sequence: 4 givenname: Rodolfo Luiz Prazeres orcidid: 0000-0001-5183-4636 surname: Gonçalves fullname: Gonçalves, Rodolfo Luiz Prazeres organization: Universidade Presbiteriana Mackenzie, Brasil – sequence: 5 givenname: Andressa A. orcidid: 0000-0002-0362-9918 surname: Oliveira fullname: Oliveira, Andressa A. organization: Universidade Presbiteriana Mackenzie, Brasil – sequence: 6 givenname: Antonio Augusto orcidid: 0000-0003-1503-1582 surname: Couto fullname: Couto, Antonio Augusto organization: Universidade Presbiteriana Mackenzie, Brasil – sequence: 7 givenname: Marcos orcidid: 0000-0002-7117-8039 surname: Massi fullname: Massi, Marcos organization: Universidade Presbiteriana Mackenzie, Brasil |
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| Cites_doi | 10.1016/j.compositesb.2008.01.002 10.4322/2176-1523.1593 10.3390/ma11020323 10.1242/jcs.91.2.269 10.1016/j.compositesa.2017.02.023 10.1016/j.carbon.2016.05.020 10.3390/ma12162520 10.1016/j.synthmet.2019.06.015 10.1016/0261-3069(91)90101-9 10.1021/nn201717a 10.1039/c2nr31164j 10.1016/j.compscitech.2006.06.015 10.1021/nn9010472 10.1016/j.matdes.2020.108831 10.1016/j.compositesa.2017.04.019 10.1177/0021998316683782 10.1016/j.ijom.2017.06.001 10.1016/j.ijom.2012.12.013 10.1021/acs.jafc.9b04442 |
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| Keywords | low-density polyethylene (LDPE) 3D printing graphene oxide (GO) |
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S. – volume: 39 start-page: 933 issue: 6 year: 2008 end-page: 961 article-title: Effects of particle size, particle/matrix interface adhesion and particle loading on mechanical properties of particulate-polymer composites publication-title: Composites Part B: Engineering contributor: fullname: FU, S.-Y.; FENG, X.-Q.; LAUKE, B.; MAI, Y.-W. – year: 2019 article-title: Graphene based polymer electrolyte membranes for electro-chemical energy applications publication-title: International Journal of Hydrogen Energy contributor: fullname: GAHLOT, S.; KULSHRESTHA, V. – volume: 67 start-page: 11464 issue: 41 year: 2019 end-page: 11473 article-title: Methionine and its hydroxyl analogs improve stem cell activity to eliminate deoxynivalenol-induced intestinal injury by reactivating wnt/β-catenin signaling publication-title: Journal of Agricultural and Food Chemistry contributor: fullname: ZHOU, J.; WANG, Z.; ZHANG, S.; LIN, H.; GAO, C; ZHAO, J.; WANG, X. – volume: 100 start-page: 31 year: 2017 end-page: 39 article-title: Influence of the chemical functionalization of graphene on the properties of polypropylene--based nanocomposites publication-title: Composites Part A: Applied Science and Manufacturing contributor: fullname: QUILES-DÍAZ, S.; ENRIQUE-JIMENEZ, P.; PAPAGEORGIOU, D. G.; ANIA, F.; FLORES, A.; KINLOCH, I. A.; SALAVAGIONE, H. J. – start-page: 108831 year: 2020 end-page: 108831 article-title: Spray deposition of graphene nano-platelets for modifying interleaves in carbon fiber reinforced polymer laminates publication-title: Materials & Design contributor: fullname: NAGI, C. S.; OGIN, S. L.; MOHAGHEGHIAN, I.; CREAN, C.; FOREMAN, A. D. – volume: 254 start-page: 141 year: 2019 end-page: 152 article-title: Electrochemical molecularly imprinted polymer based on zinc oxide/graphene/poly(o-phenylenediamine) for 4-chlorophenoldetection publication-title: Synthetic Metals contributor: fullname: AL-AMMARI, R. H..; GANASH, A. A..; SALAM, M. A. – year: 2006 publication-title: Estudos de compósitos de partículas de madeira e PEBD reciclado na presença de agentes compatibilizantes contributor: fullname: REDIGHIERI, K. I. – volume: 11 issue: 2 year: 2018 article-title: The preparation, characterization, mechanical and antibacterial properties of GO-ZnO nanocomposites with a poly(L-lactide)- modified surface publication-title: Materials contributor: fullname: YUAN, M.; XIONG, C.; JIANG, L.; LI, H; YUAN, M. – volume: 67 start-page: 1709 issue: 7-8 year: 2007 end-page: 1718 article-title: A review of the fabrication and properties of vapor-grown carbon nanofiber/polymer composites publication-title: Composites Science and Technology contributor: fullname: TIBBETTS, G.; LAKE, M.; STRONG, K.; RICE, B. – volume: 3 start-page: 3884 issue: 12 year: 2009 end-page: 3890 article-title: Enhanced mechanical properties of nanocomposites at low graphene content publication-title: ACS Nano contributor: fullname: RAFIEE, M. A.; RAFIEE, J.; WANG, Z.; SONG, H.; YU, Z.-Z.; KORATKAR, N. – volume: 240 start-page: 124486 year: 2022 end-page: 124486 article-title: Graphene and its application in thermoplastic polymers as nano-filler publication-title: A Review. contributor: fullname: TRIVEDI, D. N.; RACHCHH, N. V. – volume: 4 start-page: 5910 issue: 19 year: 2012 article-title: Mechanical properties of graphene oxides publication-title: Nanoscale contributor: fullname: LIU, L.; ZHANG, J.; ZHAO, J.; LIU, F. – volume: 5 start-page: 5920 issue: 7 year: 2011 end-page: 5927 article-title: Compatibilization of immiscible polymer blends using graphene oxide sheets publication-title: ACS Nano contributor: fullname: CAO, Y..; ZHANG, J..; FENG, J..; WU, P. – volume: 1205 article-title: Development of graphene oxide/ Polyethylene to enhance mechanical properties through melt mixing technique. IOP Conference Series publication-title: Earth and Environmental Science contributor: fullname: YUSOF, M. A.; NOR RAHMAN, N. H.; IZIRWAN, I.; MAT DESA, M. S. Z.; AB GHANI, N. F. |
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| Title | Development and performance of graphene oxide reinforced LDPE nanocomposite polymers for 3D printing |
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