Quenching induced depolarization delay and structure evolution in (1-x)Na1/2Bi1/2TiO3-xBiFeO3 ceramics
As a relaxor, Na1/2Bi1/2TiO3 (NBT) presents limitations in high temperature application because of thermally induced depolarization. Stabilizing the polar ferroelectric phase is key for deferring the temperature dependent depolarization. In this work, a transition from relaxor to ferroelectric is in...
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| Published in | Scripta materialia Vol. 259; p. 116573 |
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| Format | Journal Article |
| Language | English |
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| Abstract | As a relaxor, Na1/2Bi1/2TiO3 (NBT) presents limitations in high temperature application because of thermally induced depolarization. Stabilizing the polar ferroelectric phase is key for deferring the temperature dependent depolarization. In this work, a transition from relaxor to ferroelectric is induced by incorporating BiFeO3 (BFO) in NBT. The transition is characterized by temperature dependent dielectric and piezoelectric properties, and supported by mechanical stress-strain tests and in-situ electric field dependent synchrotron XRD analysis. To improve the depolarization temperature (Td) further, 40NBT-60BFO (60BFO) is subject to a quenching treatment. Td of 60BFO increases from 300 °C to 520 °C upon quenching. The significant increase in Td is explained by analyzing the average and local structure changes. It is found that the ordered Bi and Na ions and the intensified Bi-O bonding upon quenching contribute to the increase in Td. This work clarifies the mechanism of quenching induced enhancement Td in NBT-BFO ceramics.
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| AbstractList | As a relaxor, Na1/2Bi1/2TiO3 (NBT) presents limitations in high temperature application because of thermally induced depolarization. Stabilizing the polar ferroelectric phase is key for deferring the temperature dependent depolarization. In this work, a transition from relaxor to ferroelectric is induced by incorporating BiFeO3 (BFO) in NBT. The transition is characterized by temperature dependent dielectric and piezoelectric properties, and supported by mechanical stress-strain tests and in-situ electric field dependent synchrotron XRD analysis. To improve the depolarization temperature (Td) further, 40NBT-60BFO (60BFO) is subject to a quenching treatment. Td of 60BFO increases from 300 °C to 520 °C upon quenching. The significant increase in Td is explained by analyzing the average and local structure changes. It is found that the ordered Bi and Na ions and the intensified Bi-O bonding upon quenching contribute to the increase in Td. This work clarifies the mechanism of quenching induced enhancement Td in NBT-BFO ceramics.
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| ArticleNumber | 116573 |
| Author | Zhang, Lixue Luo, Zhihong Liu, Laijun Zhang, Mao-Hua Ren, Pengrong Lin, Wenchao Long, Changbai |
| Author_xml | – sequence: 1 givenname: Pengrong surname: Ren fullname: Ren, Pengrong email: renpengrongxaut@126.com organization: Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an 710048, PR China – sequence: 2 givenname: Wenchao surname: Lin fullname: Lin, Wenchao organization: Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an 710048, PR China – sequence: 3 givenname: Zhihong surname: Luo fullname: Luo, Zhihong organization: Guangxi Key Lab of Optical and Electronic Functional Materials and Devices, Collaborative Innovation Center for Exploration of Nonferrous Metal Deposits and Efficient Utilization of Resources, College of Materials Science and Engineering, Guilin University of Technology, Guilin 541004, PR China – sequence: 4 givenname: Mao-Hua surname: Zhang fullname: Zhang, Mao-Hua organization: Wuzhen Laboratory, 314500, Jiaxing, PR China – sequence: 5 givenname: Laijun orcidid: 0000-0002-6889-2506 surname: Liu fullname: Liu, Laijun email: ljliu2@163.com organization: Guangxi Key Lab of Optical and Electronic Functional Materials and Devices, Collaborative Innovation Center for Exploration of Nonferrous Metal Deposits and Efficient Utilization of Resources, College of Materials Science and Engineering, Guilin University of Technology, Guilin 541004, PR China – sequence: 6 givenname: Changbai surname: Long fullname: Long, Changbai organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, PR China – sequence: 7 givenname: Lixue surname: Zhang fullname: Zhang, Lixue email: lxzhang@mail.xjtu.edu.cn organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, PR China |
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| Snippet | As a relaxor, Na1/2Bi1/2TiO3 (NBT) presents limitations in high temperature application because of thermally induced depolarization. Stabilizing the polar... |
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| SubjectTerms | BiFeO3, Depolarization behavior Na1/2Bi1/2TiO3 Quenching treatment |
| Title | Quenching induced depolarization delay and structure evolution in (1-x)Na1/2Bi1/2TiO3-xBiFeO3 ceramics |
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