Infrared spectrum of hydrogen in the condensed phase
A summary of experimental results in which the infrared spectra of solid and liquid hydrogen are obtained using a high resolution spectrometer with a resolution between 0.04 and 0.06/cm is given. Both normal and para-hydrogen samples are used in the experiments. An outline of the theoretical origin...
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Published in | Acta physica hungarica Vol. 55; no. 1-4; pp. 383 - 393 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
Published |
01.03.1984
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Abstract | A summary of experimental results in which the infrared spectra of solid and liquid hydrogen are obtained using a high resolution spectrometer with a resolution between 0.04 and 0.06/cm is given. Both normal and para-hydrogen samples are used in the experiments. An outline of the theoretical origin of zero phonon transitions which mark the spectrum in the condensed phase is given. Single and double transitions caused by the quadrupole-induced dipole moment dominate the infrared spectrum and include the Q and S lines and their combinations. Results obtained for a few of the double transitions which are more intense than the single transitions and prove the existence of rotational exciton bands in the solid, are presented and compared with the theory by Van Kranendonk (1960). Quadrupolar transitions in the liquid spectrum are also summarized. |
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AbstractList | A summary of experimental results in which the infrared spectra of solid and liquid hydrogen are obtained using a high resolution spectrometer with a resolution between 0.04 and 0.06/cm is given. Both normal and para-hydrogen samples are used in the experiments. An outline of the theoretical origin of zero phonon transitions which mark the spectrum in the condensed phase is given. Single and double transitions caused by the quadrupole-induced dipole moment dominate the infrared spectrum and include the Q and S lines and their combinations. Results obtained for a few of the double transitions which are more intense than the single transitions and prove the existence of rotational exciton bands in the solid, are presented and compared with the theory by Van Kranendonk (1960). Quadrupolar transitions in the liquid spectrum are also summarized. |
Author | D’Cunha, Romola Gaines, J. R. Rao, K. Narahari Balasubramanian, T. K. |
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CitedBy_id | crossref_primary_10_1016_0022_2852_92_90509_M crossref_primary_10_1177_0003702819861581 crossref_primary_10_1366_0003702011953946 crossref_primary_10_1103_PhysRevB_39_6514 crossref_primary_10_1103_PhysRevLett_73_2833 crossref_primary_10_1103_PhysRevB_55_10420 crossref_primary_10_1016_j_molstruc_2003_10_050 crossref_primary_10_1143_JPSJ_58_3406 crossref_primary_10_1016_j_molstruc_2003_11_043 crossref_primary_10_1063_1_4820528 |
Cites_doi | 10.1139/p64-090 10.1139/p69-264 10.1051/jphysrad:01961002203014900 10.1103/PhysRevLett.47.1277 10.1139/p72-276 10.1103/PhysRevLett.33.256 10.1139/p62-002 10.1139/p62-015 10.1103/RevModPhys.52.393 10.1063/1.441171 10.1139/p70-031 10.1063/1.1841160 10.1016/0031-8914(59)90027-8 10.1139/p60-024 10.1139/p65-192 10.1016/0022-2852(82)90083-2 10.1364/AO.6.001597 10.1103/RevModPhys.40.531 10.1063/1.1840870 10.1139/p60-020 10.1038/123160a0 10.1103/PhysRevA.17.1690 |
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References | H. P. Gush (BF03155950_CR16) 1961; 22 G. Karl (BF03155950_CR19) 1967; 46 BF03155950_CR25 BF03155950_CR24 E. J. Allin (BF03155950_CR2) 1967; 6 T. K. Balasubramanian (BF03155950_CR14) 1982; 92 M. Trefler (BF03155950_CR17) 1969; 47 V. F. Sears (BF03155950_CR21) 1964; 42 J. Van Kranendonk (BF03155950_CR9) 1968; 40 R. D. G. Prasad (BF03155950_CR23) 1978; 17 S. S. Bhatnagar (BF03155950_CR3) 1962; 40 M. J. Clouter (BF03155950_CR10) 1970; 48 J. C. McLennan (BF03155950_CR5) 1929; 123 W. Kolos (BF03155950_CR20) 1967; 46 K. P. Huber (BF03155950_CR26) 1979 BF03155950_CR15 T. K. Balasubramanian (BF03155950_CR13) 1981; 47 J. Van Kranendonk (BF03155950_CR7) 1960; 38 H. P. Gush (BF03155950_CR1) 1960; 38 J. Van Kranendonk (BF03155950_CR18) 1959; 25 W. Ivancic (BF03155950_CR12) 1981; 74 V. Soots (BF03155950_CR4) 1965; 43 I. F. Silvera (BF03155950_CR6) 1980; 52 J. D. Poll (BF03155950_CR8) 1962; 40 S. A. Boggs (BF03155950_CR11) 1972; 50 P. W. Gibbs (BF03155950_CR22) 1974; 33 |
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