Preparation of porous carbon electrodes from semen cassiae for high-performance electric double-layer capacitors
A series of sponge-like hierarchical porous carbons are prepared using semen cassiae as the precursor and potassium oxalate monohydrate as the activation agent. These sponge-like carbon materials have high surface areas, wide distributions of pore size, and the appropriate forms of nitrogen/oxygen d...
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| Published in | New journal of chemistry Vol. 42; no. 9; pp. 6763 - 6769 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
2018
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| Subjects | |
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| Abstract | A series of sponge-like hierarchical porous carbons are prepared using semen cassiae as the precursor and potassium oxalate monohydrate as the activation agent. These sponge-like carbon materials have high surface areas, wide distributions of pore size, and the appropriate forms of nitrogen/oxygen derivatives. All these advantages in structures and surface states contribute to the outstanding performances of such materials as electrodes for high performance electric double-layer capacitors, which include high specific capacitance, high cycling stability, and high energy density. For example, the optimal sample exhibits a high specific capacitance of 401 F g
−1
, excellent cycling stability (94.5% retention after 10 000 cycles), high energy density (12.01 W h kg
−1
) and a high power density (10 200 W kg
−1
) in 1 M H
2
SO
4
solution. |
|---|---|
| AbstractList | A series of sponge-like hierarchical porous carbons are prepared using semen cassiae as the precursor and potassium oxalate monohydrate as the activation agent. These sponge-like carbon materials have high surface areas, wide distributions of pore size, and the appropriate forms of nitrogen/oxygen derivatives. All these advantages in structures and surface states contribute to the outstanding performances of such materials as electrodes for high performance electric double-layer capacitors, which include high specific capacitance, high cycling stability, and high energy density. For example, the optimal sample exhibits a high specific capacitance of 401 F g−1, excellent cycling stability (94.5% retention after 10 000 cycles), high energy density (12.01 W h kg−1) and a high power density (10 200 W kg−1) in 1 M H2SO4 solution. A series of sponge-like hierarchical porous carbons are prepared using semen cassiae as the precursor and potassium oxalate monohydrate as the activation agent. These sponge-like carbon materials have high surface areas, wide distributions of pore size, and the appropriate forms of nitrogen/oxygen derivatives. All these advantages in structures and surface states contribute to the outstanding performances of such materials as electrodes for high performance electric double-layer capacitors, which include high specific capacitance, high cycling stability, and high energy density. For example, the optimal sample exhibits a high specific capacitance of 401 F g −1 , excellent cycling stability (94.5% retention after 10 000 cycles), high energy density (12.01 W h kg −1 ) and a high power density (10 200 W kg −1 ) in 1 M H 2 SO 4 solution. |
| Author | Zhang, Peng Xiong, Huan-Ming Gao, Shuyan Wei, Ji-Shi Wan, Suige Chen, Xiao-Bo Wei, Xianjun Ding, Hui |
| Author_xml | – sequence: 1 givenname: Ji-Shi orcidid: 0000-0002-0605-040X surname: Wei fullname: Wei, Ji-Shi organization: Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433, P. R. China – sequence: 2 givenname: Suige surname: Wan fullname: Wan, Suige organization: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education) and School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang Henan 453007, P. R. China – sequence: 3 givenname: Peng surname: Zhang fullname: Zhang, Peng organization: Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433, P. R. China – sequence: 4 givenname: Hui orcidid: 0000-0002-7568-182X surname: Ding fullname: Ding, Hui organization: College of Chemical Engineering, China University of Mining and Technology, Xuzhou Jiangsu 221008, P. R. China – sequence: 5 givenname: Xiao-Bo surname: Chen fullname: Chen, Xiao-Bo organization: School of Engineering, RMIT University, Carlton, Australia – sequence: 6 givenname: Huan-Ming surname: Xiong fullname: Xiong, Huan-Ming organization: Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai 200433, P. R. China – sequence: 7 givenname: Shuyan surname: Gao fullname: Gao, Shuyan organization: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education) and School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang Henan 453007, P. R. China – sequence: 8 givenname: Xianjun surname: Wei fullname: Wei, Xianjun organization: Key Laboratory of Green Chemical Media and Reactions (Ministry of Education) and School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang Henan 453007, P. R. China |
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| SubjectTerms | Capacitance Capacitors Carbon Cycles Density Electrodes Flux density Pore size Porosity Potassium oxalate monohydrate Semen Stability Sulfuric acid |
| Title | Preparation of porous carbon electrodes from semen cassiae for high-performance electric double-layer capacitors |
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