Non-isothermal and isothermal co-pyrolysis characteristics of coal gangue/coal slime and pine sawdust: Thermogravimetric analyzer and fixed bed pyrolysis reactor study
The generation and accumulation of coal gangue (CG) and coal slime (CS) are a serious cause of environmental pollution. The co-pyrolysis of CG/CS and pine sawdust (PS) is an effective method to reduce pollution and waste generation. In this work, the co-pyrolysis characteristics of CG/CS and PS were...
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Published in | International journal of hydrogen energy Vol. 59; pp. 1230 - 1243 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
Published |
Elsevier Ltd
15.03.2024
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Abstract | The generation and accumulation of coal gangue (CG) and coal slime (CS) are a serious cause of environmental pollution. The co-pyrolysis of CG/CS and pine sawdust (PS) is an effective method to reduce pollution and waste generation. In this work, the co-pyrolysis characteristics of CG/CS and PS were analyzed by the thermogravimetric analyzer and fixed bed pyrolysis reactor. The kinetics analysis showed that the activation energies decreased with the PS mixing ratio increased for CG/PS blends and CS/PS blends in the second pyrolysis stage. The synergistic effect on yield is quantified by comparing the results of the co-pyrolysis of CG/CS and PS blends with weighted results from the pyrolysis of CG, CS and PS individually. The results revealed that when the mixing ratio of CG:PS was 1:1, the difference between the experimental and calculated yields (2.9 %) and the H2 yield (320 ml/g) were maximum. Among the CS/PS blends, these values are maximum when the mixing ratio of CS:PS is 3:1 (2.5 % and 450 ml/g). Furthermore, the alkali and alkaline earth metals K and Ca in the co-pyrolysis char catalyze the decomposition of the –OH functional group.
•CG/CS and PS co-pyrolysis was studied by non-isothermal and isothermal conditions.•The alkali and alkaline earth metals in the co-pyrolysis char had a catalytic effect.•CG/PS1-1 and CS/PS3-1 mixing ratio had the highest hydrogen yield. |
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AbstractList | The generation and accumulation of coal gangue (CG) and coal slime (CS) are a serious cause of environmental pollution. The co-pyrolysis of CG/CS and pine sawdust (PS) is an effective method to reduce pollution and waste generation. In this work, the co-pyrolysis characteristics of CG/CS and PS were analyzed by the thermogravimetric analyzer and fixed bed pyrolysis reactor. The kinetics analysis showed that the activation energies decreased with the PS mixing ratio increased for CG/PS blends and CS/PS blends in the second pyrolysis stage. The synergistic effect on yield is quantified by comparing the results of the co-pyrolysis of CG/CS and PS blends with weighted results from the pyrolysis of CG, CS and PS individually. The results revealed that when the mixing ratio of CG:PS was 1:1, the difference between the experimental and calculated yields (2.9 %) and the H2 yield (320 ml/g) were maximum. Among the CS/PS blends, these values are maximum when the mixing ratio of CS:PS is 3:1 (2.5 % and 450 ml/g). Furthermore, the alkali and alkaline earth metals K and Ca in the co-pyrolysis char catalyze the decomposition of the –OH functional group.
•CG/CS and PS co-pyrolysis was studied by non-isothermal and isothermal conditions.•The alkali and alkaline earth metals in the co-pyrolysis char had a catalytic effect.•CG/PS1-1 and CS/PS3-1 mixing ratio had the highest hydrogen yield. |
Author | Han, Fengtao Han, Shuang Niu, Yonghong Hu, Yuyang Yang, Man |
Author_xml | – sequence: 1 givenname: Yonghong orcidid: 0000-0001-7599-401X surname: Niu fullname: Niu, Yonghong email: niuyonghong@imust.cn organization: Inner Mongolia University of Science and Technology, China – sequence: 2 givenname: Shuang surname: Han fullname: Han, Shuang organization: Inner Mongolia University of Science and Technology, China – sequence: 3 givenname: Yuyang surname: Hu fullname: Hu, Yuyang organization: North China Electric Power University, China – sequence: 4 givenname: Man surname: Yang fullname: Yang, Man organization: Inner Mongolia University of Science and Technology, China – sequence: 5 givenname: Fengtao surname: Han fullname: Han, Fengtao organization: Wenzhou University of Technology, China |
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Snippet | The generation and accumulation of coal gangue (CG) and coal slime (CS) are a serious cause of environmental pollution. The co-pyrolysis of CG/CS and pine... |
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SubjectTerms | Biomass Co-pyrolysis characteristics Coal gangue Coal slime Kinetics |
Title | Non-isothermal and isothermal co-pyrolysis characteristics of coal gangue/coal slime and pine sawdust: Thermogravimetric analyzer and fixed bed pyrolysis reactor study |
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