Navigating the intricacies: A critical review of numerical modeling in battery research and design

The intricate interplay of multi-scale and multi-physics phenomena within battery systems poses a substantial challenge in harmonizing microscopic electrochemical processes. This complexity impedes the advancement of innovative designs for large-scale transportation and energy storage applications,...

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Published inJournal of power sources Vol. 628; p. 235902
Main Authors Wen, Jian, Wang, Li, He, Xiangming
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.02.2025
Subjects
Battery operations
Electrochemical processes
Multi-physics interactions
Multi-scale phenomena
Numerical modeling
Thermal management
Numerical modeling
Multi-scale phenomena
Multi-physics interactions
Thermal management
Battery operations
Electrochemical processes
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Abstract The intricate interplay of multi-scale and multi-physics phenomena within battery systems poses a substantial challenge in harmonizing microscopic electrochemical processes. This complexity impedes the advancement of innovative designs for large-scale transportation and energy storage applications, frequently culminating in prohibitively high costs. Anticipating the real-world impact of laboratory-developed batteries on industrial devices remains largely an elusive endeavor. Nonetheless, physics-based numerical inquiries have emerged as a promising approach to illuminating the interactions across various battery domains and scales, ranging from the individual cell to the system level. Physical models, grounded in a set of assumptions, may result in critical inaccuracies when based on ill-informed predictions, a particular risk within the nuanced sphere of battery design, which is fraught with complex physical and chemical interactions. This paper endeavors to clarify the subtleties of numerical models utilized in battery research and design. It seeks to demystify the development of battery models by drawing on physical expressions from scholarly works to map the interconnections among diverse models. This paper provides an insight into the subject, delineating the essential electrochemical governing equations, equivalent circuit models, degradation mechanisms, and methodologies for multi-physics integration, thereby establishing a robust framework for the exploration and creation of cutting-edge battery technologies. •Multi-scale challenges in battery operations hinder alignment with systems.•Complexity in battery design impacts large-scale energy storage innovation.•Numerical study in physics based models offer insight into battery all scales.•Battery model evolution clarified through literature-based interconnections.•Explores electrochemistry, degradation, and multi-physics couplings in models.
AbstractList The intricate interplay of multi-scale and multi-physics phenomena within battery systems poses a substantial challenge in harmonizing microscopic electrochemical processes. This complexity impedes the advancement of innovative designs for large-scale transportation and energy storage applications, frequently culminating in prohibitively high costs. Anticipating the real-world impact of laboratory-developed batteries on industrial devices remains largely an elusive endeavor. Nonetheless, physics-based numerical inquiries have emerged as a promising approach to illuminating the interactions across various battery domains and scales, ranging from the individual cell to the system level. Physical models, grounded in a set of assumptions, may result in critical inaccuracies when based on ill-informed predictions, a particular risk within the nuanced sphere of battery design, which is fraught with complex physical and chemical interactions. This paper endeavors to clarify the subtleties of numerical models utilized in battery research and design. It seeks to demystify the development of battery models by drawing on physical expressions from scholarly works to map the interconnections among diverse models. This paper provides an insight into the subject, delineating the essential electrochemical governing equations, equivalent circuit models, degradation mechanisms, and methodologies for multi-physics integration, thereby establishing a robust framework for the exploration and creation of cutting-edge battery technologies. •Multi-scale challenges in battery operations hinder alignment with systems.•Complexity in battery design impacts large-scale energy storage innovation.•Numerical study in physics based models offer insight into battery all scales.•Battery model evolution clarified through literature-based interconnections.•Explores electrochemistry, degradation, and multi-physics couplings in models.
ArticleNumber 235902
Author Wen, Jian
Wang, Li
He, Xiangming
Author_xml – sequence: 1
  givenname: Jian
  surname: Wen
  fullname: Wen, Jian
  organization: Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, China
– sequence: 2
  givenname: Li
  surname: Wang
  fullname: Wang, Li
  organization: Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, China
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  givenname: Xiangming
  orcidid: 0000-0001-7146-4097
  surname: He
  fullname: He, Xiangming
  email: hexm@tsinghua.edu.cn, hexiangming@tsinghua.org.cn, he-xm@tsinghua.edu.cn
  organization: Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, China
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Snippet The intricate interplay of multi-scale and multi-physics phenomena within battery systems poses a substantial challenge in harmonizing microscopic...
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SubjectTerms Battery operations
Electrochemical processes
Multi-physics interactions
Multi-scale phenomena
Numerical modeling
Thermal management
Title Navigating the intricacies: A critical review of numerical modeling in battery research and design
URI https://dx.doi.org/10.1016/j.jpowsour.2024.235902
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