Nano Copper Sulfide-Doped nanofiber surface on polylactic acid substrate for advanced photothermal membrane distillation
[Display omitted] •An asymmetric construction for efficient PMD was proposed;•The PAPHF membrane maintained desalination efficiency with an daily flux of 1.86 kg·m−2·h−1;•CuS NPs decreased water-evaporation enthalpy in PMD process; The phase change process was simulated using CFD. Photothermal membr...
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| Published in | Separation and purification technology Vol. 370; p. 133306 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
18.10.2025
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| Subjects | |
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| Abstract | [Display omitted]
•An asymmetric construction for efficient PMD was proposed;•The PAPHF membrane maintained desalination efficiency with an daily flux of 1.86 kg·m−2·h−1;•CuS NPs decreased water-evaporation enthalpy in PMD process; The phase change process was simulated using CFD.
Photothermal membrane distillation has been recognized as an attractive technology for freshwater generation. However, its widespread application still depends on substantial development to increase membrane flux and decrease energy consumption. Herein, we designed a electrospinning poly(vinylidene fluoride)–co-hexafluoropropylene (PVDF-HFP) nanofiber with photothermal CuS NPs as the top layer, while agglutinating the bottom hydrophilic polylactic acid layer by polydopamine, yielding a novel photothermal asymmetric PVDF-HFP fibrous (PAPHF) membrane. Compared to tradtional filtration method for material doped, such regulatable structure gives competitive advantage in the light utilization, water evaporation and transport. Electrospun photothermal nanofibers, which possesses a 81 %-90 % light-to-heat conversion efficiency, combined with the hydrophobic pores, can efficiently convert liquid water to vapor water and prevent heat diffusion outside the phase change inerface, meanwhile, enable effective vapor transport due to hydrophilic bottom layer with macropores. The PAPHF membrane demonstrated an excellent daily flux of 1.86 kg·m−2·h−1 with 1 sun irradiation as the only energy input. Computational fluid dynamics exhibited phase change processes acrosss the membrane. This study offers prospects for optimizing material combinations to improve performance, emphasizing scalable manufacturing implementation for broader applications. |
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| AbstractList | [Display omitted]
•An asymmetric construction for efficient PMD was proposed;•The PAPHF membrane maintained desalination efficiency with an daily flux of 1.86 kg·m−2·h−1;•CuS NPs decreased water-evaporation enthalpy in PMD process; The phase change process was simulated using CFD.
Photothermal membrane distillation has been recognized as an attractive technology for freshwater generation. However, its widespread application still depends on substantial development to increase membrane flux and decrease energy consumption. Herein, we designed a electrospinning poly(vinylidene fluoride)–co-hexafluoropropylene (PVDF-HFP) nanofiber with photothermal CuS NPs as the top layer, while agglutinating the bottom hydrophilic polylactic acid layer by polydopamine, yielding a novel photothermal asymmetric PVDF-HFP fibrous (PAPHF) membrane. Compared to tradtional filtration method for material doped, such regulatable structure gives competitive advantage in the light utilization, water evaporation and transport. Electrospun photothermal nanofibers, which possesses a 81 %-90 % light-to-heat conversion efficiency, combined with the hydrophobic pores, can efficiently convert liquid water to vapor water and prevent heat diffusion outside the phase change inerface, meanwhile, enable effective vapor transport due to hydrophilic bottom layer with macropores. The PAPHF membrane demonstrated an excellent daily flux of 1.86 kg·m−2·h−1 with 1 sun irradiation as the only energy input. Computational fluid dynamics exhibited phase change processes acrosss the membrane. This study offers prospects for optimizing material combinations to improve performance, emphasizing scalable manufacturing implementation for broader applications. |
| ArticleNumber | 133306 |
| Author | Wang, Ao Tao, Hui Lin, Tao Ding, Mingmei Xu, Hang Ma, Jun Wang, Jingjun Hu, Tianlong |
| Author_xml | – sequence: 1 givenname: Ao surname: Wang fullname: Wang, Ao organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 2 givenname: Hang surname: Xu fullname: Xu, Hang email: xuhang810826@hhu.edu.com organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 3 givenname: Jun surname: Ma fullname: Ma, Jun organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 4 givenname: Tianlong surname: Hu fullname: Hu, Tianlong organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 5 givenname: Jingjun surname: Wang fullname: Wang, Jingjun organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 6 givenname: Tao surname: Lin fullname: Lin, Tao organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 7 givenname: Hui surname: Tao fullname: Tao, Hui organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China – sequence: 8 givenname: Mingmei surname: Ding fullname: Ding, Mingmei email: dingmm2021@163.com organization: Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes, Ministry of Education, College of Environment, Hohai University, No.1 Xikang Road, Nanjing 210098, China |
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| SubjectTerms | Desalination Electrospinning Evaporation Membrane distillation Photothermal Membrane distillation |
| Title | Nano Copper Sulfide-Doped nanofiber surface on polylactic acid substrate for advanced photothermal membrane distillation |
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