Two-pronged strategy: Energizing bifunctional polyarylamine ketones in electrochromic supercapacitors
With the objective to actualize the lightweight and intelligent criteria in implementation and to extend the application range of high-performance polymers, a selection comprising polyarylamine ketone (PAAK) has been designed and synthesized as electrochromic materials. The remarkable photoelectric...
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| Published in | Journal of alloys and compounds Vol. 1013; p. 178526 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
31.01.2025
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| Subjects | |
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| Abstract | With the objective to actualize the lightweight and intelligent criteria in implementation and to extend the application range of high-performance polymers, a selection comprising polyarylamine ketone (PAAK) has been designed and synthesized as electrochromic materials. The remarkable photoelectric function of triphenylamine moieties and high-performance polymer characteristics were appropriately matched. And the synthesis method generalizability was confirmed through several attempts of side-chain substituent adjustment. The benefits of V2O5 nanowire ion storage layers in conjunction with the donor-acceptor (D-A) molecular engineering strategy deftly balanced electrochromic and energy storage features. Amongst them, devices employing PAAK-TPPA-OMe retained electrochromic performance subject to a 30,000-second switching. It was accessible to enhance the coloration efficiency to 331.19 cm2/C and reduce coloring time to 1.48 s after optimization. Likewise, PAAK-TPPA-OMe/V2O5 ECS yielded an area specific capacitance of 462.3 μF/cm2 and an energy density of 146.8 mWh/cm2 at a current density of 0.01 mA/cm2. It was convinced that such a conception could guide the intelligent integration of high-performance polymer functionalities.
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•Series of intelligent materials derived from PAAKs have been designed and synthesized.•The system features a highly adjustable D-A structure.•The rational device structure enables color change and energy storage integration.•The coloring time for PAAK-TPPA-OMe/V2O5 ECS after optimization is merely 1.48 s.•The PAAK-TPPA-OMe/V2O5 ECS can operate continuously for more than 30,000 s. |
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| AbstractList | With the objective to actualize the lightweight and intelligent criteria in implementation and to extend the application range of high-performance polymers, a selection comprising polyarylamine ketone (PAAK) has been designed and synthesized as electrochromic materials. The remarkable photoelectric function of triphenylamine moieties and high-performance polymer characteristics were appropriately matched. And the synthesis method generalizability was confirmed through several attempts of side-chain substituent adjustment. The benefits of V2O5 nanowire ion storage layers in conjunction with the donor-acceptor (D-A) molecular engineering strategy deftly balanced electrochromic and energy storage features. Amongst them, devices employing PAAK-TPPA-OMe retained electrochromic performance subject to a 30,000-second switching. It was accessible to enhance the coloration efficiency to 331.19 cm2/C and reduce coloring time to 1.48 s after optimization. Likewise, PAAK-TPPA-OMe/V2O5 ECS yielded an area specific capacitance of 462.3 μF/cm2 and an energy density of 146.8 mWh/cm2 at a current density of 0.01 mA/cm2. It was convinced that such a conception could guide the intelligent integration of high-performance polymer functionalities.
[Display omitted]
•Series of intelligent materials derived from PAAKs have been designed and synthesized.•The system features a highly adjustable D-A structure.•The rational device structure enables color change and energy storage integration.•The coloring time for PAAK-TPPA-OMe/V2O5 ECS after optimization is merely 1.48 s.•The PAAK-TPPA-OMe/V2O5 ECS can operate continuously for more than 30,000 s. |
| ArticleNumber | 178526 |
| Author | Jiang, Zhenhua Chen, Zheng Wang, Qilin Shen, Huilin Han, Yuntao Zheng, Zhibo |
| Author_xml | – sequence: 1 givenname: Qilin surname: Wang fullname: Wang, Qilin organization: Engineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, China – sequence: 2 givenname: Zhibo surname: Zheng fullname: Zheng, Zhibo organization: Department of Chemical Engineering and Applied Chemistry, College of Chemistry, Jilin University, Changchun 130012, China – sequence: 3 givenname: Huilin surname: Shen fullname: Shen, Huilin organization: Engineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, China – sequence: 4 givenname: Yuntao surname: Han fullname: Han, Yuntao email: hanyuntao@boe.com.cn organization: Engineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, China – sequence: 5 givenname: Zheng surname: Chen fullname: Chen, Zheng email: chenzheng2013@jlu.edu.cn organization: Engineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, China – sequence: 6 givenname: Zhenhua surname: Jiang fullname: Jiang, Zhenhua organization: Engineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Changchun 130012, China |
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