Aggregation-induced emission type non-traditional intrinsic luminescent polymers with improved thermal property via one-pot Barbier polymerization-induced emission
Developing simple methods to prepare non-traditional intrinsic luminescent (NTIL) polymers with enhanced thermal property are very urgent, interesting and important. Here, we demonstrate a one-pot method to design NTIL polymer with improved thermal property by introducing phenyl ether group into the...
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| Published in | Journal of luminescence Vol. 269; p. 120516 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.05.2024
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Developing simple methods to prepare non-traditional intrinsic luminescent (NTIL) polymers with enhanced thermal property are very urgent, interesting and important. Here, we demonstrate a one-pot method to design NTIL polymer with improved thermal property by introducing phenyl ether group into the molecular design of triphenylmethanol-containing polymers via Barbier polymerization-induced emission (PIE). Through Barbier polymerization of 4,4′-dibromodiphenyl ether and peroxyesters in tetrahydrofuran at 80 °C, a series of phenyl ether containing polymers have been prepared, including poly (phenylether-triphenylmethanol) (PPTPM), poly (phenylether para-methyl-triphenylmethanol) (PPMTPM), poly (phenylether para-methoxy-triphenylmethanol) (PPMeOTPM). Interestingly, these polymers exhibit aggregation-induced emission (AIE) type NTIL characteristics. By introducing functional phenyl ether group into polymer design, the thermal property of these polymers gets improved, where the decomposition temperature at 5% weight loss (T5) increases from 196 to 288 °C, in comparison with that without phenyl ether group. This work therefore opens a simple and one-pot avenue for the preparation of AIE type NTIL polymers with improved thermal property, which might cause inspirations to different fields such as polymerization, NTIL and AIE.
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•A series of non-traditional intrinsic luminescent (NTIL) polymers were prepared via Barbier polymerization-induced emission (PIE).•These NTIL polymers exhibit aggregation-induced emission (AIE) type NTIL.•NTIL polymers have improved thermal property by introducing phenyl ether group. |
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| AbstractList | Developing simple methods to prepare non-traditional intrinsic luminescent (NTIL) polymers with enhanced thermal property are very urgent, interesting and important. Here, we demonstrate a one-pot method to design NTIL polymer with improved thermal property by introducing phenyl ether group into the molecular design of triphenylmethanol-containing polymers via Barbier polymerization-induced emission (PIE). Through Barbier polymerization of 4,4′-dibromodiphenyl ether and peroxyesters in tetrahydrofuran at 80 °C, a series of phenyl ether containing polymers have been prepared, including poly (phenylether-triphenylmethanol) (PPTPM), poly (phenylether para-methyl-triphenylmethanol) (PPMTPM), poly (phenylether para-methoxy-triphenylmethanol) (PPMeOTPM). Interestingly, these polymers exhibit aggregation-induced emission (AIE) type NTIL characteristics. By introducing functional phenyl ether group into polymer design, the thermal property of these polymers gets improved, where the decomposition temperature at 5% weight loss (T5) increases from 196 to 288 °C, in comparison with that without phenyl ether group. This work therefore opens a simple and one-pot avenue for the preparation of AIE type NTIL polymers with improved thermal property, which might cause inspirations to different fields such as polymerization, NTIL and AIE.
[Display omitted]
•A series of non-traditional intrinsic luminescent (NTIL) polymers were prepared via Barbier polymerization-induced emission (PIE).•These NTIL polymers exhibit aggregation-induced emission (AIE) type NTIL.•NTIL polymers have improved thermal property by introducing phenyl ether group. |
| ArticleNumber | 120516 |
| Author | Li, Qian Wan, Wen-Ming Xiao, Hang Shi, Quan-Xi Cai, Hua-Wen Bao, Hongli Zheng, Xing-Ying |
| Author_xml | – sequence: 1 givenname: Qian surname: Li fullname: Li, Qian organization: Key Laboratory of Coal to Ethylene Glycol and Its Related Technology, State Key Laboratory of Structural Chemistry, Center for Excellence in Molecular Synthesis, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, PR China – sequence: 2 givenname: Hang surname: Xiao fullname: Xiao, Hang organization: College of Environmental and Resource Sciences, Engineering Research Center of Polymer Green Recycling of Ministry of Education, Fujian Key Laboratory of Pollution Control &Resource Reuse, Fujian Normal University, Fuzhou, 350007, PR China – sequence: 3 givenname: Quan-Xi surname: Shi fullname: Shi, Quan-Xi organization: Key Laboratory of Coal to Ethylene Glycol and Its Related Technology, State Key Laboratory of Structural Chemistry, Center for Excellence in Molecular Synthesis, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, PR China – sequence: 4 givenname: Xing-Ying surname: Zheng fullname: Zheng, Xing-Ying organization: College of Environmental and Resource Sciences, Engineering Research Center of Polymer Green Recycling of Ministry of Education, Fujian Key Laboratory of Pollution Control &Resource Reuse, Fujian Normal University, Fuzhou, 350007, PR China – sequence: 5 givenname: Hua-Wen surname: Cai fullname: Cai, Hua-Wen organization: College of Environmental and Resource Sciences, Engineering Research Center of Polymer Green Recycling of Ministry of Education, Fujian Key Laboratory of Pollution Control &Resource Reuse, Fujian Normal University, Fuzhou, 350007, PR China – sequence: 6 givenname: Wen-Ming orcidid: 0000-0002-3692-4454 surname: Wan fullname: Wan, Wen-Ming email: wanwenming@fjnu.edu.cn organization: Key Laboratory of Coal to Ethylene Glycol and Its Related Technology, State Key Laboratory of Structural Chemistry, Center for Excellence in Molecular Synthesis, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, PR China – sequence: 7 givenname: Hongli surname: Bao fullname: Bao, Hongli email: hlbao@fjirsm.ac.cn organization: Key Laboratory of Coal to Ethylene Glycol and Its Related Technology, State Key Laboratory of Structural Chemistry, Center for Excellence in Molecular Synthesis, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, PR China |
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| Keywords | One-pot Barbier polymerization Polymerization-induced emission Aggregation-induced emission Non-traditional intrinsic luminescence |
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