Electrochemiluminescence sensor based on EuS nanocrystals for ultrasensitive detection of mercury ions in seafood

In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was dev...

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Published inSensors and actuators. B, Chemical Vol. 352; p. 131075
Main Authors Hua, Qing, Tang, Feiyan, Wang, Xiaobin, Li, Min, Gu, Xiaowen, Sun, Wenjie, Luan, Feng, Tian, Chunyuan, Zhuang, Xuming
Format Journal Article
LanguageEnglish
Published Lausanne Elsevier B.V 01.02.2022
Elsevier Science Ltd
Subjects
Electrochemiluminescence
Emission analysis
Europium
Europium sulfide
Mercury
Mercury (metal)
Nanocrystals
Potassium persulfate
Reagents
Seafood
Sensors
Seafood
Electrochemiluminescence
Europium sulfide
Mercury
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Abstract In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was developed. A linear response between the ECL intensity and the concentration of Hg2+ was obtained in the range from 0.1 pM to 105 pM, achieving a detection limit of 0.028 pM. Moreover, this sensor was also successfully applied to the detection of Hg2+ in seafood with good recovery. The current study provides a green and feasible method for the detection of trace Hg2+ in seafood. [Display omitted] •The electrochemiluminescence (ECL) of EuS nanocrystals was reported.•An intensive and stable cathode ECL emission at − 2.0 V was observed.•The ECL sensor with high selectivity and stability was achieved for detecting Hg2+.•This sensor was successfully applied for Hg2+ detection in seafood.
AbstractList In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was developed. A linear response between the ECL intensity and the concentration of Hg2+ was obtained in the range from 0.1 pM to 105 pM, achieving a detection limit of 0.028 pM. Moreover, this sensor was also successfully applied to the detection of Hg2+ in seafood with good recovery. The current study provides a green and feasible method for the detection of trace Hg2+ in seafood. [Display omitted] •The electrochemiluminescence (ECL) of EuS nanocrystals was reported.•An intensive and stable cathode ECL emission at − 2.0 V was observed.•The ECL sensor with high selectivity and stability was achieved for detecting Hg2+.•This sensor was successfully applied for Hg2+ detection in seafood.
In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was developed. A linear response between the ECL intensity and the concentration of Hg2+ was obtained in the range from 0.1 pM to 105 pM, achieving a detection limit of 0.028 pM. Moreover, this sensor was also successfully applied to the detection of Hg2+ in seafood with good recovery. The current study provides a green and feasible method for the detection of trace Hg2+ in seafood.
ArticleNumber 131075
Author Li, Min
Zhuang, Xuming
Sun, Wenjie
Tian, Chunyuan
Hua, Qing
Gu, Xiaowen
Wang, Xiaobin
Tang, Feiyan
Luan, Feng
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Electrochemiluminescence
Europium sulfide
Mercury
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Snippet In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective...
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StartPage 131075
SubjectTerms Electrochemiluminescence
Emission analysis
Europium
Europium sulfide
Mercury
Mercury (metal)
Nanocrystals
Potassium persulfate
Reagents
Seafood
Sensors
Title Electrochemiluminescence sensor based on EuS nanocrystals for ultrasensitive detection of mercury ions in seafood
URI https://dx.doi.org/10.1016/j.snb.2021.131075
https://www.proquest.com/docview/2623903564
Volume 352
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