Electrochemiluminescence sensor based on EuS nanocrystals for ultrasensitive detection of mercury ions in seafood
In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was dev...
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Published in | Sensors and actuators. B, Chemical Vol. 352; p. 131075 |
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Main Authors | , , , , , , , , |
Format | Journal Article |
Language | English |
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Lausanne
Elsevier B.V
01.02.2022
Elsevier Science Ltd |
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Abstract | In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was developed. A linear response between the ECL intensity and the concentration of Hg2+ was obtained in the range from 0.1 pM to 105 pM, achieving a detection limit of 0.028 pM. Moreover, this sensor was also successfully applied to the detection of Hg2+ in seafood with good recovery. The current study provides a green and feasible method for the detection of trace Hg2+ in seafood.
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•The electrochemiluminescence (ECL) of EuS nanocrystals was reported.•An intensive and stable cathode ECL emission at − 2.0 V was observed.•The ECL sensor with high selectivity and stability was achieved for detecting Hg2+.•This sensor was successfully applied for Hg2+ detection in seafood. |
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AbstractList | In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was developed. A linear response between the ECL intensity and the concentration of Hg2+ was obtained in the range from 0.1 pM to 105 pM, achieving a detection limit of 0.028 pM. Moreover, this sensor was also successfully applied to the detection of Hg2+ in seafood with good recovery. The current study provides a green and feasible method for the detection of trace Hg2+ in seafood.
[Display omitted]
•The electrochemiluminescence (ECL) of EuS nanocrystals was reported.•An intensive and stable cathode ECL emission at − 2.0 V was observed.•The ECL sensor with high selectivity and stability was achieved for detecting Hg2+.•This sensor was successfully applied for Hg2+ detection in seafood. In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective quenching of the ECL emission from EuS NCs by Hg2+, a novel label-free ECL sensor for the highly sensitive and selective detection of Hg2+ was developed. A linear response between the ECL intensity and the concentration of Hg2+ was obtained in the range from 0.1 pM to 105 pM, achieving a detection limit of 0.028 pM. Moreover, this sensor was also successfully applied to the detection of Hg2+ in seafood with good recovery. The current study provides a green and feasible method for the detection of trace Hg2+ in seafood. |
ArticleNumber | 131075 |
Author | Li, Min Zhuang, Xuming Sun, Wenjie Tian, Chunyuan Hua, Qing Gu, Xiaowen Wang, Xiaobin Tang, Feiyan Luan, Feng |
Author_xml | – sequence: 1 givenname: Qing surname: Hua fullname: Hua, Qing – sequence: 2 givenname: Feiyan surname: Tang fullname: Tang, Feiyan – sequence: 3 givenname: Xiaobin surname: Wang fullname: Wang, Xiaobin – sequence: 4 givenname: Min surname: Li fullname: Li, Min – sequence: 5 givenname: Xiaowen surname: Gu fullname: Gu, Xiaowen – sequence: 6 givenname: Wenjie surname: Sun fullname: Sun, Wenjie – sequence: 7 givenname: Feng surname: Luan fullname: Luan, Feng – sequence: 8 givenname: Chunyuan surname: Tian fullname: Tian, Chunyuan email: cytian@ytu.edu.cn – sequence: 9 givenname: Xuming surname: Zhuang fullname: Zhuang, Xuming email: xmzhuang@iccas.ac.cn |
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Snippet | In this work, the electrochemiluminescence (ECL) of europium sulfide nanocrystals (EuS NCs) in K2S2O8 cathode co-reagents was studied. Based on selective... |
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SubjectTerms | Electrochemiluminescence Emission analysis Europium Europium sulfide Mercury Mercury (metal) Nanocrystals Potassium persulfate Reagents Seafood Sensors |
Title | Electrochemiluminescence sensor based on EuS nanocrystals for ultrasensitive detection of mercury ions in seafood |
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