Constructing Pd/2D-C3N4 composites for efficient photocatalytic H2 evolution through nonplasmon-induced bound electrons
Pd/2D-C3N4 composites are prepared by a facile hydrothermal method, which exhibit enhanced light absorption through interband electronic transitions and show obvious enhanced photocatalytic H2 evolution rate (758.3 μmol/g/h). [Display omitted] •The Pd/2D-C3N4 composites can be synthesized via a faci...
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| Published in | Applied surface science Vol. 467-468; pp. 151 - 157 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2019
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Pd/2D-C3N4 composites are prepared by a facile hydrothermal method, which exhibit enhanced light absorption through interband electronic transitions and show obvious enhanced photocatalytic H2 evolution rate (758.3 μmol/g/h).
[Display omitted]
•The Pd/2D-C3N4 composites can be synthesized via a facile hydrothermal strategy.•Pd nanocubes have excellent trapping capability for electrons.•0.5% Pd/2D-C3N4 exhibits a stable and excellent H2 evolution activity.•The external quantum efficiency of 0.5% Pd/2D-C3N4 is up to 3.8% (λ = 420 nm).
As a kind of metal-free photocatalytic materials, carbon nitride has been widely applied in photocatalytic hydrogen (H2) evolution, but the solar to hydrogen conversion efficiency is still not ideal. In this work, Pd nanocubes are anchored on 2D-C3N4 through a facile hydrothermal strategy to obtain better charge separation/transfer efficiency, attributed to the excellent trapping capability for electrons and the energetic electrons via the interband transition of Pd nanocubes. The as-synthesized Pd/2D-C3N4 composites exhibit superior and stable photocatalytic H2 evolution performance, and 0.5% Pd/2D-C3N4 possesses the optimized activity with the H2 evolution rate of 1208.6 μmol g−1 h−1. In addition, the apparent quantum efficiency for photocatalytic H2 evolution is up to 3.8% at 420 nm. The increased photocatalytic activity may mainly benefit from the excellent charge separation/transfer efficiency caused by doping Pd nanocubes. |
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| AbstractList | Pd/2D-C3N4 composites are prepared by a facile hydrothermal method, which exhibit enhanced light absorption through interband electronic transitions and show obvious enhanced photocatalytic H2 evolution rate (758.3 μmol/g/h).
[Display omitted]
•The Pd/2D-C3N4 composites can be synthesized via a facile hydrothermal strategy.•Pd nanocubes have excellent trapping capability for electrons.•0.5% Pd/2D-C3N4 exhibits a stable and excellent H2 evolution activity.•The external quantum efficiency of 0.5% Pd/2D-C3N4 is up to 3.8% (λ = 420 nm).
As a kind of metal-free photocatalytic materials, carbon nitride has been widely applied in photocatalytic hydrogen (H2) evolution, but the solar to hydrogen conversion efficiency is still not ideal. In this work, Pd nanocubes are anchored on 2D-C3N4 through a facile hydrothermal strategy to obtain better charge separation/transfer efficiency, attributed to the excellent trapping capability for electrons and the energetic electrons via the interband transition of Pd nanocubes. The as-synthesized Pd/2D-C3N4 composites exhibit superior and stable photocatalytic H2 evolution performance, and 0.5% Pd/2D-C3N4 possesses the optimized activity with the H2 evolution rate of 1208.6 μmol g−1 h−1. In addition, the apparent quantum efficiency for photocatalytic H2 evolution is up to 3.8% at 420 nm. The increased photocatalytic activity may mainly benefit from the excellent charge separation/transfer efficiency caused by doping Pd nanocubes. |
| Author | Yan, Pengcheng Mo, Zhao Yi, Jianjian Zhu, Xingwang Li, Huaming Song, Yanhua Xu, Hui She, Xiaojie Lei, Yucheng Yuan, Shouqi |
| Author_xml | – sequence: 1 givenname: Zhao surname: Mo fullname: Mo, Zhao organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 2 givenname: Hui surname: Xu fullname: Xu, Hui email: xh@ujs.edu.cn organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 3 givenname: Xiaojie surname: She fullname: She, Xiaojie organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 4 givenname: Yanhua surname: Song fullname: Song, Yanhua organization: School of Environmental and Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, PR China – sequence: 5 givenname: Pengcheng surname: Yan fullname: Yan, Pengcheng organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 6 givenname: Jianjian surname: Yi fullname: Yi, Jianjian organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 7 givenname: Xingwang surname: Zhu fullname: Zhu, Xingwang organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 8 givenname: Yucheng surname: Lei fullname: Lei, Yucheng email: yclei@ujs.edu.cn organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 9 givenname: Shouqi surname: Yuan fullname: Yuan, Shouqi organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China – sequence: 10 givenname: Huaming surname: Li fullname: Li, Huaming organization: School of Materials Science & Engineering, Institute for Energy Research, Jiangsu University, Zhenjiang 212013, PR China |
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| SubjectTerms | 2D-C3N4 Nonplasmonic transition metals Pd nanocubes Photocatalytic H2 evolution |
| Title | Constructing Pd/2D-C3N4 composites for efficient photocatalytic H2 evolution through nonplasmon-induced bound electrons |
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