Systematic study on the impact of water on the performance and stability of perovskite solar cells
The effects of water on the photovoltaic performance of methylammonium lead iodide perovskite devices has recently become a topic of interest within the perovskite community. However, existing studies report contrasting and sometimes contradictory observations. In this work, small concentrations of...
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| Published in | RSC advances Vol. 6; no. 57; pp. 52448 - 52458 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2016
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| Online Access | Get full text |
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| Abstract | The effects of water on the photovoltaic performance of methylammonium lead iodide perovskite devices has recently become a topic of interest within the perovskite community. However, existing studies report contrasting and sometimes contradictory observations. In this work, small concentrations of water, consistent with those present in air-exposed DMF, were systematically incorporated directly into the PbI
2
precursor solution in order to investigate its effect on the performance of sequentially spin-coated, inverted perovskite solar cells. Increasing concentrations of water in the PbI
2
solution were found to have a negative impact on photovoltaic performance. The addition of water was observed to exaggerate the scan-rate and directional-dependent hysteresis and introduce new transient behaviours in comparison to the dry devices. Interestingly, the addition of water was also found to improve the long-term device stability in comparison with devices fabricated from dry precursors.
Sequentially spin-coated inverted perovskite solar cells were constructed with systematically varied concentrations of water in the PbI
2
precursor solution. Surprisingly, small concentrations of water improved long-term stability, although with lower initial efficiency. |
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| AbstractList | The effects of water on the photovoltaic performance of methylammonium lead iodide perovskite devices has recently become a topic of interest within the perovskite community. However, existing studies report contrasting and sometimes contradictory observations. In this work, small concentrations of water, consistent with those present in air-exposed DMF, were systematically incorporated directly into the PbI
2
precursor solution in order to investigate its effect on the performance of sequentially spin-coated, inverted perovskite solar cells. Increasing concentrations of water in the PbI
2
solution were found to have a negative impact on photovoltaic performance. The addition of water was observed to exaggerate the scan-rate and directional-dependent hysteresis and introduce new transient behaviours in comparison to the dry devices. Interestingly, the addition of water was also found to improve the long-term device stability in comparison with devices fabricated from dry precursors.
Sequentially spin-coated inverted perovskite solar cells were constructed with systematically varied concentrations of water in the PbI
2
precursor solution. Surprisingly, small concentrations of water improved long-term stability, although with lower initial efficiency. The effects of water on the photovoltaic performance of methylammonium lead iodide perovskite devices has recently become a topic of interest within the perovskite community. However, existing studies report contrasting and sometimes contradictory observations. In this work, small concentrations of water, consistent with those present in air-exposed DMF, were systematically incorporated directly into the PbI 2 precursor solution in order to investigate its effect on the performance of sequentially spin-coated, inverted perovskite solar cells. Increasing concentrations of water in the PbI 2 solution were found to have a negative impact on photovoltaic performance. The addition of water was observed to exaggerate the scan-rate and directional-dependent hysteresis and introduce new transient behaviours in comparison to the “dry” devices. Interestingly, the addition of water was also found to improve the long-term device stability in comparison with devices fabricated from “dry” precursors. |
| Author | Clegg, Charlotte Hill, Ian G |
| AuthorAffiliation | Dalhousie University Department of Physics and Atmospheric Science |
| AuthorAffiliation_xml | – sequence: 0 name: Dalhousie University – sequence: 0 name: Department of Physics and Atmospheric Science |
| Author_xml | – sequence: 1 givenname: Charlotte surname: Clegg fullname: Clegg, Charlotte – sequence: 2 givenname: Ian G surname: Hill fullname: Hill, Ian G |
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| Notes | O in the PbI 10.1039/c6ra11379f 2 film. See DOI Electronic supplementary information (ESI) available: Tables, statistical summaries of performance metrics, transient photocurrent fits and SEM images for devices/films fabricated with varying concentrations of H |
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| Snippet | The effects of water on the photovoltaic performance of methylammonium lead iodide perovskite devices has recently become a topic of interest within the... |
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| Title | Systematic study on the impact of water on the performance and stability of perovskite solar cells |
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