Preparation and luminescence properties of novel K2ZnP2O7: Mn2+ green phosphor
Novel green-emitting phosphors K 2 Zn 1 − x P 2 O 7 : x mol% Mn 2+ have been successfully prepared using classical solid-state reaction method in air atmosphere, doped by different Mn 2+ ion contents, namely x = 0.5, 1, 1.25 and 1.5 mol%. The samples were characterized by the thermogravimetric (ATD...
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Published in | Journal of materials science. Materials in electronics Vol. 32; no. 23; pp. 27475 - 27483 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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New York
Springer US
01.12.2021
Springer Nature B.V |
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Abstract | Novel green-emitting phosphors K
2
Zn
1 − x
P
2
O
7
: x mol% Mn
2+
have been successfully prepared using classical solid-state reaction method in air atmosphere, doped by different Mn
2+
ion contents, namely
x
= 0.5, 1, 1.25 and 1.5 mol%. The samples were characterized by the thermogravimetric (ATD/ATG/DSC), X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR), steady and time-resolved photoluminescence techniques. It was found that all K
2
Zn
1 − x
P
2
O
7
: x mol% Mn
2+
samples crystallize in the tetragonal phase with
P4
2
/mnm
space group. Upon 425 nm excitation, K
2
ZnP
2
O
7
: Mn
2+
exhibits an intense broad green asymmetric emission band peaking at 520 nm, owing to the
4
T
1
→
6
A
1
(
6
S) transition of Mn
2+
ion in K
2
ZnP
2
O
7
. In addition, it is suggested that Mn
2+
ions occupy more than one symmetry site in the host K
2
ZnP
2
O
7
. The optimal Mn
2+
ion concentration in K
2
ZnP
2
O
7
:Mn
2+
phosphor is 1 mol % and with the lifetime 9.81 ms. |
---|---|
AbstractList | Novel green-emitting phosphors K
2
Zn
1 − x
P
2
O
7
: x mol% Mn
2+
have been successfully prepared using classical solid-state reaction method in air atmosphere, doped by different Mn
2+
ion contents, namely
x
= 0.5, 1, 1.25 and 1.5 mol%. The samples were characterized by the thermogravimetric (ATD/ATG/DSC), X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR), steady and time-resolved photoluminescence techniques. It was found that all K
2
Zn
1 − x
P
2
O
7
: x mol% Mn
2+
samples crystallize in the tetragonal phase with
P4
2
/mnm
space group. Upon 425 nm excitation, K
2
ZnP
2
O
7
: Mn
2+
exhibits an intense broad green asymmetric emission band peaking at 520 nm, owing to the
4
T
1
→
6
A
1
(
6
S) transition of Mn
2+
ion in K
2
ZnP
2
O
7
. In addition, it is suggested that Mn
2+
ions occupy more than one symmetry site in the host K
2
ZnP
2
O
7
. The optimal Mn
2+
ion concentration in K
2
ZnP
2
O
7
:Mn
2+
phosphor is 1 mol % and with the lifetime 9.81 ms. Novel green-emitting phosphors K2Zn1 − xP2O7: x mol% Mn2+ have been successfully prepared using classical solid-state reaction method in air atmosphere, doped by different Mn2+ ion contents, namely x = 0.5, 1, 1.25 and 1.5 mol%. The samples were characterized by the thermogravimetric (ATD/ATG/DSC), X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR), steady and time-resolved photoluminescence techniques. It was found that all K2Zn1 − xP2O7: x mol% Mn2+ samples crystallize in the tetragonal phase with P42/mnm space group. Upon 425 nm excitation, K2ZnP2O7: Mn2+ exhibits an intense broad green asymmetric emission band peaking at 520 nm, owing to the 4T1→6A1(6 S) transition of Mn2+ ion in K2ZnP2O7. In addition, it is suggested that Mn2+ ions occupy more than one symmetry site in the host K2ZnP2O7. The optimal Mn2+ ion concentration in K2ZnP2O7:Mn2+ phosphor is 1 mol % and with the lifetime 9.81 ms. |
Author | Saidat, Boubakeur Bentria, Bachir Gacem, Lakhdar Soltani, Mohamed Toufik Guerbous, Lakhdar Belbal, Rim |
Author_xml | – sequence: 1 givenname: Rim surname: Belbal fullname: Belbal, Rim email: r.belbal@lagh-univ.dz organization: Materials Physics Laboratory, University Thelidji Amar – sequence: 2 givenname: Lakhdar surname: Gacem fullname: Gacem, Lakhdar organization: Materials Science and Informatics Laboratory, University of Ziane Achour Djelfa – sequence: 3 givenname: Bachir surname: Bentria fullname: Bentria, Bachir organization: Materials Physics Laboratory, University Thelidji Amar – sequence: 4 givenname: Boubakeur surname: Saidat fullname: Saidat, Boubakeur organization: Laboratory of Physical Chemistry of Materials (LPCM), Faculty of Sciences, University Thelidji Amar – sequence: 5 givenname: Mohamed Toufik surname: Soltani fullname: Soltani, Mohamed Toufik organization: Laboratory of Physics of Photonics and Multifunctional Nanomaterials, University of Biskra – sequence: 6 givenname: Lakhdar orcidid: 0000-0002-5371-5435 surname: Guerbous fullname: Guerbous, Lakhdar email: guerbous@yahoo.fr organization: Laser physics Department/Physics Division/Nuclear Research Center of Algiers |
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Snippet | Novel green-emitting phosphors K
2
Zn
1 − x
P
2
O
7
: x mol% Mn
2+
have been successfully prepared using classical solid-state reaction method in air... Novel green-emitting phosphors K2Zn1 − xP2O7: x mol% Mn2+ have been successfully prepared using classical solid-state reaction method in air atmosphere, doped... |
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StartPage | 27475 |
SubjectTerms | Characterization and Evaluation of Materials Chemistry and Materials Science Fourier transforms Infrared spectroscopy Ion concentration Luminescence Manganese ions Materials Science Optical and Electronic Materials Optical properties Original Research Phosphors Photoluminescence |
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Title | Preparation and luminescence properties of novel K2ZnP2O7: Mn2+ green phosphor |
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