Laminated Flow-Cell Detector with Granulated Scintillator for the Detection of Tritiated Water

Nuclear sites require regular measurements of the air, soil, and groundwater to ensure the safety of the surrounding environment from potentially hazardous levels of contamination. Although high-energy beta and gamma emitters can often be detected instantly using fixed dosimeters, the detection of l...

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Published inRadiation (Multidisciplinary Digital Publishing Institute) Vol. 3; no. 4; pp. 211 - 225
Main Authors Dixon, Nile E. J., Monk, Stephen D., Graham, James, Cheneler, David
Format Journal Article
LanguageEnglish
Published Munich MDPI AG 01.12.2023
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Abstract Nuclear sites require regular measurements of the air, soil, and groundwater to ensure the safety of the surrounding environment from potentially hazardous levels of contamination. Although high-energy beta and gamma emitters can often be detected instantly using fixed dosimeters, the detection of low-energy beta emitters is a difficult challenge, especially in groundwater, as its radiation is easily self-absorbed by the surrounding medium. Therefore, it is common practice to sample groundwater and transfer it to a laboratory for analysis using Liquid Scintillation Counting. This work demonstrates a new detector design for the real-time monitoring of tritiated water, a weak beta emitter. This design utilizes a flow cell filled with a granulated scintillator to maximize the surface area of the sample. The cavity is made from plastic sheets, which allow rapid manufacture using readily available lamination sheets. A column of SiPMs in coincidence counting mode has been implemented to reduce noise and allow future extensions to the flow cell for greater detection rates while allowing the detector to fit within limited spaces such as groundwater monitoring boreholes. Using multiple concentrations of tritiated water, this detector has been validated and calibrated, obtaining a minimum detection activity of 26.356 ± 0.889 Bq/mL for a 1-day counting period.
AbstractList Simple SummaryTritium, a radioactive isotope of hydrogen, is incredibly difficult to detect at a distance, making conventional monitoring equipment like Geiger Müller detectors unsuitable. This is partly because tritium only emits low-energy beta radiation, which is easily absorbed by surrounding matter, including the mica window of a Geiger Müller tube, which typically can only measure higher energy radiation emitted from heavier isotopes (the limit is Carbon-14, which emits 156 keV beta). Scintillators are an alternative radiation-monitoring approach and are used to detect radiation by interacting with these betas, producing light that itself can be detected using high-sensitivity light sensors. This work tests a granulated scintillator that can be mixed directly with water-containing tritium and kept contained within a flow cell formed using heat lamination. Results show a relationship between powder fineness and detection rate, as well as an increased count rate when tritium is added to a manufactured laminated flow cell containing a granulated scintillator.AbstractNuclear sites require regular measurements of the air, soil, and groundwater to ensure the safety of the surrounding environment from potentially hazardous levels of contamination. Although high-energy beta and gamma emitters can often be detected instantly using fixed dosimeters, the detection of low-energy beta emitters is a difficult challenge, especially in groundwater, as its radiation is easily self-absorbed by the surrounding medium. Therefore, it is common practice to sample groundwater and transfer it to a laboratory for analysis using Liquid Scintillation Counting. This work demonstrates a new detector design for the real-time monitoring of tritiated water, a weak beta emitter. This design utilizes a flow cell filled with a granulated scintillator to maximize the surface area of the sample. The cavity is made from plastic sheets, which allow rapid manufacture using readily available lamination sheets. A column of SiPMs in coincidence counting mode has been implemented to reduce noise and allow future extensions to the flow cell for greater detection rates while allowing the detector to fit within limited spaces such as groundwater monitoring boreholes. Using multiple concentrations of tritiated water, this detector has been validated and calibrated, obtaining a minimum detection activity of 26.356 ± 0.889 Bq/mL for a 1-day counting period.
Nuclear sites require regular measurements of the air, soil, and groundwater to ensure the safety of the surrounding environment from potentially hazardous levels of contamination. Although high-energy beta and gamma emitters can often be detected instantly using fixed dosimeters, the detection of low-energy beta emitters is a difficult challenge, especially in groundwater, as its radiation is easily self-absorbed by the surrounding medium. Therefore, it is common practice to sample groundwater and transfer it to a laboratory for analysis using Liquid Scintillation Counting. This work demonstrates a new detector design for the real-time monitoring of tritiated water, a weak beta emitter. This design utilizes a flow cell filled with a granulated scintillator to maximize the surface area of the sample. The cavity is made from plastic sheets, which allow rapid manufacture using readily available lamination sheets. A column of SiPMs in coincidence counting mode has been implemented to reduce noise and allow future extensions to the flow cell for greater detection rates while allowing the detector to fit within limited spaces such as groundwater monitoring boreholes. Using multiple concentrations of tritiated water, this detector has been validated and calibrated, obtaining a minimum detection activity of 26.356 ± 0.889 Bq/mL for a 1-day counting period.
Author Dixon, Nile E. J.
Cheneler, David
Monk, Stephen D.
Graham, James
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Simple SummaryTritium, a radioactive isotope of hydrogen, is incredibly difficult to detect at a distance, making conventional monitoring equipment like Geiger...
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SubjectTerms Cosmic rays
Drinking water
Efficiency
Energy
flow-cell detector
granulated scintillator
Particle size
Radiation
Sensors
tritiated water
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Title Laminated Flow-Cell Detector with Granulated Scintillator for the Detection of Tritiated Water
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