Chemical lattice strain in nonstoichiometric oxides: an overview

Strong coupling between the chemical composition and crystal lattice dimensions resulting in the contraction or expansion of a material upon change of its chemical composition is known as chemical expansion or chemical strain. This phenomenon significantly influences the performance of oxide materia...

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Published inJournal of materials chemistry. A, Materials for energy and sustainability Vol. 1; no. 12; pp. 6351 - 6375
Main Authors Tsvetkov, Dmitry S, Sereda, Vladimir V, Malyshkin, Dmitry A, Ivanov, Ivan L, Zuev, Andrey Yu
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 22.03.2022
Subjects
Chemical composition
Computer applications
Coupling
Crystal lattices
Electrochemistry
Energy conversion
Energy storage
Fuel technology
High temperature
Lattice strain
Mechanical properties
Reviews
Solid oxide fuel cells
State-of-the-art reviews
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Abstract Strong coupling between the chemical composition and crystal lattice dimensions resulting in the contraction or expansion of a material upon change of its chemical composition is known as chemical expansion or chemical strain. This phenomenon significantly influences the performance of oxide materials in different energy conversion and storage devices. In many such applications, e.g. , in oxygen-permeating membranes or solid oxide fuel cells (SOFCs), the materials are subject to significant in situ variation of their chemical composition, which is accompanied by large volume changes. This may often be detrimental to the operation of the electrochemical device. Not only is chemo-mechanical coupling crucial for various practical applications, but also, when measured accurately and discussed appropriately, the chemical strain of an oxide material allows better understanding of its local electronic and defect structure. Chemical strain is also strongly correlated with diffusion phenomena in high-temperature electrochemical devices - the subject that for many years has been of particular scientific interest for John Kilner and where he holds a lot of pioneering achievements. This article reviews the state of the art in the field of chemical strain of various oxide materials, primarily those intended to operate at elevated temperatures, and aims at summarizing the available experimental, theoretical and computational insights into its origins, factors impacting its magnitude, and the available means for its a priori quantitative estimation. This article reviews the state of the art - from the experimental and computational data available to the models, origins and possible uses - in the field of chemical strain of oxide materials (primarily those for elevated-temperature applications).
AbstractList Strong coupling between the chemical composition and crystal lattice dimensions resulting in the contraction or expansion of a material upon change of its chemical composition is known as chemical expansion or chemical strain. This phenomenon significantly influences the performance of oxide materials in different energy conversion and storage devices. In many such applications, e.g. , in oxygen-permeating membranes or solid oxide fuel cells (SOFCs), the materials are subject to significant in situ variation of their chemical composition, which is accompanied by large volume changes. This may often be detrimental to the operation of the electrochemical device. Not only is chemo-mechanical coupling crucial for various practical applications, but also, when measured accurately and discussed appropriately, the chemical strain of an oxide material allows better understanding of its local electronic and defect structure. Chemical strain is also strongly correlated with diffusion phenomena in high-temperature electrochemical devices – the subject that for many years has been of particular scientific interest for John Kilner and where he holds a lot of pioneering achievements. This article reviews the state of the art in the field of chemical strain of various oxide materials, primarily those intended to operate at elevated temperatures, and aims at summarizing the available experimental, theoretical and computational insights into its origins, factors impacting its magnitude, and the available means for its a priori quantitative estimation.
Strong coupling between the chemical composition and crystal lattice dimensions resulting in the contraction or expansion of a material upon change of its chemical composition is known as chemical expansion or chemical strain. This phenomenon significantly influences the performance of oxide materials in different energy conversion and storage devices. In many such applications, e.g., in oxygen-permeating membranes or solid oxide fuel cells (SOFCs), the materials are subject to significant in situ variation of their chemical composition, which is accompanied by large volume changes. This may often be detrimental to the operation of the electrochemical device. Not only is chemo-mechanical coupling crucial for various practical applications, but also, when measured accurately and discussed appropriately, the chemical strain of an oxide material allows better understanding of its local electronic and defect structure. Chemical strain is also strongly correlated with diffusion phenomena in high-temperature electrochemical devices – the subject that for many years has been of particular scientific interest for John Kilner and where he holds a lot of pioneering achievements. This article reviews the state of the art in the field of chemical strain of various oxide materials, primarily those intended to operate at elevated temperatures, and aims at summarizing the available experimental, theoretical and computational insights into its origins, factors impacting its magnitude, and the available means for its a priori quantitative estimation.
Strong coupling between the chemical composition and crystal lattice dimensions resulting in the contraction or expansion of a material upon change of its chemical composition is known as chemical expansion or chemical strain. This phenomenon significantly influences the performance of oxide materials in different energy conversion and storage devices. In many such applications, e.g. , in oxygen-permeating membranes or solid oxide fuel cells (SOFCs), the materials are subject to significant in situ variation of their chemical composition, which is accompanied by large volume changes. This may often be detrimental to the operation of the electrochemical device. Not only is chemo-mechanical coupling crucial for various practical applications, but also, when measured accurately and discussed appropriately, the chemical strain of an oxide material allows better understanding of its local electronic and defect structure. Chemical strain is also strongly correlated with diffusion phenomena in high-temperature electrochemical devices - the subject that for many years has been of particular scientific interest for John Kilner and where he holds a lot of pioneering achievements. This article reviews the state of the art in the field of chemical strain of various oxide materials, primarily those intended to operate at elevated temperatures, and aims at summarizing the available experimental, theoretical and computational insights into its origins, factors impacting its magnitude, and the available means for its a priori quantitative estimation. This article reviews the state of the art - from the experimental and computational data available to the models, origins and possible uses - in the field of chemical strain of oxide materials (primarily those for elevated-temperature applications).
Author Malyshkin, Dmitry A
Tsvetkov, Dmitry S
Zuev, Andrey Yu
Sereda, Vladimir V
Ivanov, Ivan L
AuthorAffiliation Ural Federal University
Institute of Natural Sciences and Mathematics
Laboratory of Hydrogen Energy
AuthorAffiliation_xml – name: Laboratory of Hydrogen Energy
– name: Ural Federal University
– name: Institute of Natural Sciences and Mathematics
Author_xml – sequence: 1
  givenname: Dmitry S
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  surname: Zuev
  fullname: Zuev, Andrey Yu
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SSID ssj0000800699
Score 2.529729
Snippet Strong coupling between the chemical composition and crystal lattice dimensions resulting in the contraction or expansion of a material upon change of its...
SourceID proquest
crossref
rsc
SourceType Aggregation Database
Publisher
StartPage 6351
SubjectTerms Chemical composition
Computer applications
Coupling
Crystal lattices
Electrochemistry
Energy conversion
Energy storage
Fuel technology
High temperature
Lattice strain
Mechanical properties
Reviews
Solid oxide fuel cells
State-of-the-art reviews
Title Chemical lattice strain in nonstoichiometric oxides: an overview
URI https://www.proquest.com/docview/2641404657
Volume 1
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