Sequentially photocatalytic degradation of mussel-inspired polydopamine: From nanoscale disassembly to effective mineralization

The photodegradation and deadhesion of mussel-inspired polydopamine was reported from nanoscale disassembly to effective mineralization. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. The patterned and gradient surfaces were prepared by the “top-down” m...

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Published inJournal of colloid and interface science Vol. 672; pp. 329 - 337
Main Authors Liu, Xinghuan, Li, Danya, Tabassum, Mehwish, Huang, Chao, Yi, Ke, Fang, Tianwen, Jia, Xin
Format Journal Article
LanguageEnglish
Published United States Elsevier Inc 15.10.2024
Subjects
Mineralization
Mussel-inspired polydopamine
Photocatalytic degradation
Surface patterning
Mussel-inspired polydopamine
Photocatalytic degradation
Surface patterning
Mineralization
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Abstract The photodegradation and deadhesion of mussel-inspired polydopamine was reported from nanoscale disassembly to effective mineralization. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. The patterned and gradient surfaces were prepared by the “top-down” method under the control of light scope and intensity, respectively. [Display omitted] Mussel-inspired polydopamine (PDA) coating has been utilized extensively as versatile deposition strategies that can functionalize surfaces of virtually all substrates. However, the strong adhesion, stability and intermolecular interaction of PDA make it inefficient in certain applications. Herein, a green and efficient photocatalytic method was reported to remove adhesion and degrade PDA by using TiO2-H2O2 as photocatalyst. The photodegradation process of the PDA spheres was first undergone nanoscale disassembly to form soluble PDA oligomers or well-dispersed nanoparticles. Most of the disassembled PDA can be photodegraded and finally mineralized to CO2 and H2O. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. Such process provides a practical strategy for constructing the patterned and gradient surfaces by the “top-down” method under the control of light scope and intensity. This sequential degradation strategy is beneficial to achieve the decomposition of highly crosslinked polymers.
AbstractList Mussel-inspired polydopamine (PDA) coating has been utilized extensively as versatile deposition strategies that can functionalize surfaces of virtually all substrates. However, the strong adhesion, stability and intermolecular interaction of PDA make it inefficient in certain applications. Herein, a green and efficient photocatalytic method was reported to remove adhesion and degrade PDA by using TiO -H O as photocatalyst. The photodegradation process of the PDA spheres was first undergone nanoscale disassembly to form soluble PDA oligomers or well-dispersed nanoparticles. Most of the disassembled PDA can be photodegraded and finally mineralized to CO and H O. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. Such process provides a practical strategy for constructing the patterned and gradient surfaces by the "top-down" method under the control of light scope and intensity. This sequential degradation strategy is beneficial to achieve the decomposition of highly crosslinked polymers.
Mussel-inspired polydopamine (PDA) coating has been utilized extensively as versatile deposition strategies that can functionalize surfaces of virtually all substrates. However, the strong adhesion, stability and intermolecular interaction of PDA make it inefficient in certain applications. Herein, a green and efficient photocatalytic method was reported to remove adhesion and degrade PDA by using TiO2-H2O2 as photocatalyst. The photodegradation process of the PDA spheres was first undergone nanoscale disassembly to form soluble PDA oligomers or well-dispersed nanoparticles. Most of the disassembled PDA can be photodegraded and finally mineralized to CO2 and H2O. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. Such process provides a practical strategy for constructing the patterned and gradient surfaces by the "top-down" method under the control of light scope and intensity. This sequential degradation strategy is beneficial to achieve the decomposition of highly crosslinked polymers.Mussel-inspired polydopamine (PDA) coating has been utilized extensively as versatile deposition strategies that can functionalize surfaces of virtually all substrates. However, the strong adhesion, stability and intermolecular interaction of PDA make it inefficient in certain applications. Herein, a green and efficient photocatalytic method was reported to remove adhesion and degrade PDA by using TiO2-H2O2 as photocatalyst. The photodegradation process of the PDA spheres was first undergone nanoscale disassembly to form soluble PDA oligomers or well-dispersed nanoparticles. Most of the disassembled PDA can be photodegraded and finally mineralized to CO2 and H2O. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. Such process provides a practical strategy for constructing the patterned and gradient surfaces by the "top-down" method under the control of light scope and intensity. This sequential degradation strategy is beneficial to achieve the decomposition of highly crosslinked polymers.
The photodegradation and deadhesion of mussel-inspired polydopamine was reported from nanoscale disassembly to effective mineralization. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. The patterned and gradient surfaces were prepared by the “top-down” method under the control of light scope and intensity, respectively. [Display omitted] Mussel-inspired polydopamine (PDA) coating has been utilized extensively as versatile deposition strategies that can functionalize surfaces of virtually all substrates. However, the strong adhesion, stability and intermolecular interaction of PDA make it inefficient in certain applications. Herein, a green and efficient photocatalytic method was reported to remove adhesion and degrade PDA by using TiO2-H2O2 as photocatalyst. The photodegradation process of the PDA spheres was first undergone nanoscale disassembly to form soluble PDA oligomers or well-dispersed nanoparticles. Most of the disassembled PDA can be photodegraded and finally mineralized to CO2 and H2O. Various PDA coated templates and PDA hollow structures can be photodegraded by this strategy. Such process provides a practical strategy for constructing the patterned and gradient surfaces by the “top-down” method under the control of light scope and intensity. This sequential degradation strategy is beneficial to achieve the decomposition of highly crosslinked polymers.
Author Jia, Xin
Yi, Ke
Fang, Tianwen
Huang, Chao
Liu, Xinghuan
Li, Danya
Tabassum, Mehwish
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  email: jiaxin@shzu.edu.cn
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Keywords Mussel-inspired polydopamine
Photocatalytic degradation
Surface patterning
Mineralization
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Snippet The photodegradation and deadhesion of mussel-inspired polydopamine was reported from nanoscale disassembly to effective mineralization. Various PDA coated...
Mussel-inspired polydopamine (PDA) coating has been utilized extensively as versatile deposition strategies that can functionalize surfaces of virtually all...
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StartPage 329
SubjectTerms Mineralization
Mussel-inspired polydopamine
Photocatalytic degradation
Surface patterning
Title Sequentially photocatalytic degradation of mussel-inspired polydopamine: From nanoscale disassembly to effective mineralization
URI https://dx.doi.org/10.1016/j.jcis.2024.06.008
https://www.ncbi.nlm.nih.gov/pubmed/38850860
https://www.proquest.com/docview/3065986537
Volume 672
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