K2YF5:Tb3+ single crystal: An in-depth study of spectroscopic properties, energy transfer and quantum cutting

Tb3+ doped K2YF5 single crystal was synthesized by the hydrothermal technique. Structure of material was analyzed by X-ray diffraction pattern and Raman spectra. The optical properties were studied through absorption, luminescence spectra and decay curves. Absorption spectra were used to calculate t...

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Published inOptical materials Vol. 106; p. 109939
Main Authors Tuyen, Vu Phi, Quang, Vu Xuan, Khaidukov, Nicholas M., Thanh, Luong Duy, Ca, Nguyen Xuan, Van Hao, Nguyen, Van Nghia, Nguyen, Van Do, Phan
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.08.2020
Subjects
Judd-ofelt theory
K2YF5 single Crystal
Quantum cutting
K2YF5 single Crystal
Quantum cutting
Judd-ofelt theory
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Abstract Tb3+ doped K2YF5 single crystal was synthesized by the hydrothermal technique. Structure of material was analyzed by X-ray diffraction pattern and Raman spectra. The optical properties were studied through absorption, luminescence spectra and decay curves. Absorption spectra were used to calculate the bonding parameter (δ) and Judd-Ofelt intensity parameters (Ω2,4,6). The JO parameters and emission spectra have been used to estimate radiative properties such as transition probability (AR), branching ratios (βcal, βexp), lifetime (τcal) stimulated emission cross-sections (σλp, 10−22 cm2) and optical gain (σλp × τcal, 10−25 cm2 s) for 5D3→7FJ and 5D4→7FJ (J = 0 ÷ 6) transitions. The dominant interaction mechanism and energy transfer parameters between Tb3+ ions have been found by fitting the decay curves of 5D3 level to the Inokuti-Hirayama model. In addition, the quantum cutting process based on energy transfer between Tb3+ ions has also been studied for K2YF5:Tb3+ crystal. •Quantum cutting luminescence in K2YF2:Tb3+ occurs under excitation at 245 nm.•Spectroscopic properties of K2YF2:Tb3+ crystal is analyzed by Judd-Ofelt theory.•Luminescence from 5D4 level is enhanced with the increase of Tb3+ concentration.•The 5D4.→7F5 transition has application ability for laser and optical amplifier.•Energy transfer between Tb3+ ions is studied through Inokuti-Hirayama model.
AbstractList Tb3+ doped K2YF5 single crystal was synthesized by the hydrothermal technique. Structure of material was analyzed by X-ray diffraction pattern and Raman spectra. The optical properties were studied through absorption, luminescence spectra and decay curves. Absorption spectra were used to calculate the bonding parameter (δ) and Judd-Ofelt intensity parameters (Ω2,4,6). The JO parameters and emission spectra have been used to estimate radiative properties such as transition probability (AR), branching ratios (βcal, βexp), lifetime (τcal) stimulated emission cross-sections (σλp, 10−22 cm2) and optical gain (σλp × τcal, 10−25 cm2 s) for 5D3→7FJ and 5D4→7FJ (J = 0 ÷ 6) transitions. The dominant interaction mechanism and energy transfer parameters between Tb3+ ions have been found by fitting the decay curves of 5D3 level to the Inokuti-Hirayama model. In addition, the quantum cutting process based on energy transfer between Tb3+ ions has also been studied for K2YF5:Tb3+ crystal. •Quantum cutting luminescence in K2YF2:Tb3+ occurs under excitation at 245 nm.•Spectroscopic properties of K2YF2:Tb3+ crystal is analyzed by Judd-Ofelt theory.•Luminescence from 5D4 level is enhanced with the increase of Tb3+ concentration.•The 5D4.→7F5 transition has application ability for laser and optical amplifier.•Energy transfer between Tb3+ ions is studied through Inokuti-Hirayama model.
ArticleNumber 109939
Author Thanh, Luong Duy
Tuyen, Vu Phi
Van Do, Phan
Quang, Vu Xuan
Ca, Nguyen Xuan
Van Hao, Nguyen
Van Nghia, Nguyen
Khaidukov, Nicholas M.
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Snippet Tb3+ doped K2YF5 single crystal was synthesized by the hydrothermal technique. Structure of material was analyzed by X-ray diffraction pattern and Raman...
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SubjectTerms Judd-ofelt theory
K2YF5 single Crystal
Quantum cutting
Title K2YF5:Tb3+ single crystal: An in-depth study of spectroscopic properties, energy transfer and quantum cutting
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