Redox regulation of photocatalytic nitrogen reduction reaction by gadolinium doping in two-dimensional bismuth molybdate nanosheets
In-built Gd3+ redox centers can effectively promote the separation and transfer of photocarriers to regulate photocatalytic nitrogen reduction reaction of 2D Bi2MoO6 nanosheets. [Display omitted] •Gd doping can boost nitrogen fixation activity of 2D Bi2MoO6 (300.15 μmol g−1 h−1).•The Gd3+ redox cent...
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Published in | Applied surface science Vol. 600; p. 154105 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
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Elsevier B.V
30.10.2022
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Abstract | In-built Gd3+ redox centers can effectively promote the separation and transfer of photocarriers to regulate photocatalytic nitrogen reduction reaction of 2D Bi2MoO6 nanosheets.
[Display omitted]
•Gd doping can boost nitrogen fixation activity of 2D Bi2MoO6 (300.15 μmol g−1 h−1).•The Gd3+ redox centers can promote the separation and transfer of photocarriers.•The AQE of Gd-doped 2D Bi2MoO6 reached 4.9% at 375 nm, about 5.8 times of Bi2MoO6.•Gd doping promotes the formation of *NHNH to regulate nitrogen reduction reaction.
Photocatalytic nitrogen reduction can achieve sustainable NH3 synthesis at room temperature and pressure, which is a more sustainable technology than the classical Haber-Bosch process. Herein, based on the ability of Gd3+ ions to capture and release electrons, a novel Gd-doped 2D Bi2MoO6 nanosheet photocatalyst for nitrogen reduction with in-built Gd3+ redox center was designed and prepared. The results showed that Gd3+ doping can increase the number of reaction sites by increasing the specific surface area of 2D Bi2MoO6, and promote the separation and transfer of photogenerated carriers by forming in-built Gd3+ redox centers. The visible-light-driven nitrogen reduction performance of Gd-Bi2MoO6 was obviously improved, and the average yield of NH3 was 300.15 μmol g-1 h−1, which was about 5.8 times that of pure Bi2MoO6. Theoretical calculations showed that the Gd3+ redox centers can also control the formation of *NHNH to regulate the nitrogen reduction reaction, which greatly reduces the free energy of the whole nitrogen reduction reaction, thus effectively accelerating the conversion of N2 to NH3. The significance of this work is to prove that the lanthanide ion Gd3+ can be used to regulate the nitrogen reduction reaction of 2D catalyst and enhance the performance of nitrogen reduction reaction. |
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AbstractList | In-built Gd3+ redox centers can effectively promote the separation and transfer of photocarriers to regulate photocatalytic nitrogen reduction reaction of 2D Bi2MoO6 nanosheets.
[Display omitted]
•Gd doping can boost nitrogen fixation activity of 2D Bi2MoO6 (300.15 μmol g−1 h−1).•The Gd3+ redox centers can promote the separation and transfer of photocarriers.•The AQE of Gd-doped 2D Bi2MoO6 reached 4.9% at 375 nm, about 5.8 times of Bi2MoO6.•Gd doping promotes the formation of *NHNH to regulate nitrogen reduction reaction.
Photocatalytic nitrogen reduction can achieve sustainable NH3 synthesis at room temperature and pressure, which is a more sustainable technology than the classical Haber-Bosch process. Herein, based on the ability of Gd3+ ions to capture and release electrons, a novel Gd-doped 2D Bi2MoO6 nanosheet photocatalyst for nitrogen reduction with in-built Gd3+ redox center was designed and prepared. The results showed that Gd3+ doping can increase the number of reaction sites by increasing the specific surface area of 2D Bi2MoO6, and promote the separation and transfer of photogenerated carriers by forming in-built Gd3+ redox centers. The visible-light-driven nitrogen reduction performance of Gd-Bi2MoO6 was obviously improved, and the average yield of NH3 was 300.15 μmol g-1 h−1, which was about 5.8 times that of pure Bi2MoO6. Theoretical calculations showed that the Gd3+ redox centers can also control the formation of *NHNH to regulate the nitrogen reduction reaction, which greatly reduces the free energy of the whole nitrogen reduction reaction, thus effectively accelerating the conversion of N2 to NH3. The significance of this work is to prove that the lanthanide ion Gd3+ can be used to regulate the nitrogen reduction reaction of 2D catalyst and enhance the performance of nitrogen reduction reaction. |
ArticleNumber | 154105 |
Author | Li, Baiqing Tao, Boran Wang, Guofu Chang, Haixin Li, Hongda Gu, Shaonan Li, Chenpu Zhao, Hao |
Author_xml | – sequence: 1 givenname: Hongda surname: Li fullname: Li, Hongda organization: Liuzhou Key Laboratory for New Energy Vehicle Power Lithium Battery, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Liuzhou 545006, China – sequence: 2 givenname: Hao surname: Zhao fullname: Zhao, Hao organization: Liuzhou Key Laboratory for New Energy Vehicle Power Lithium Battery, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Liuzhou 545006, China – sequence: 3 givenname: Chenpu surname: Li fullname: Li, Chenpu organization: Liuzhou Key Laboratory for New Energy Vehicle Power Lithium Battery, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Liuzhou 545006, China – sequence: 4 givenname: Baiqing surname: Li fullname: Li, Baiqing organization: Liuzhou Key Laboratory for New Energy Vehicle Power Lithium Battery, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Liuzhou 545006, China – sequence: 5 givenname: Boran surname: Tao fullname: Tao, Boran organization: Liuzhou Key Laboratory for New Energy Vehicle Power Lithium Battery, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Liuzhou 545006, China – sequence: 6 givenname: Shaonan surname: Gu fullname: Gu, Shaonan email: sngu@qlu.edu.cn organization: Key Laboratory of Fine Chemicals in Universities of Shandong, Jinan Engineering Laboratory for Multi–Scale Functional Materials, School of Chemistry and Chemical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China – sequence: 7 givenname: Guofu surname: Wang fullname: Wang, Guofu email: gfwang@guet.edu.cn organization: Liuzhou Key Laboratory for New Energy Vehicle Power Lithium Battery, School of Microelectronics and Materials Engineering, Guangxi University of Science and Technology, Liuzhou 545006, China – sequence: 8 givenname: Haixin surname: Chang fullname: Chang, Haixin email: hxchang@hust.edu.cn organization: Quantum–Nano Matter and Device Lab, State Key Laboratory of Material Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China |
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Cites_doi | 10.1016/j.apcatb.2021.120766 10.1021/acscatal.1c00072 10.1016/j.chempr.2020.11.002 10.1002/adma.202008180 10.1039/D2NR00198E 10.1002/adfm.202010901 10.1039/D0TA04251J 10.1016/j.jcis.2021.09.069 10.1016/j.jallcom.2020.156935 10.1002/advs.202104579 10.1002/admi.202102031 10.1016/j.apsusc.2021.149753 10.1016/j.jcis.2021.07.111 10.1021/acsami.6b08129 10.1016/j.nanoen.2021.106333 10.1002/aenm.202003294 10.1021/acscatal.9b04925 10.1002/aenm.201801357 10.1039/C4CS00085D 10.1016/j.jmst.2020.04.023 10.1039/C9CC02291K 10.1016/j.jtice.2021.08.027 10.1016/j.cej.2020.127115 10.1016/j.jallcom.2021.161757 10.1016/j.cej.2020.125944 10.1016/j.jcis.2021.09.078 10.1016/j.apcatb.2020.119580 10.1002/cctc.202001775 10.1021/jp500645p 10.1002/jcc.20495 10.1007/BF00549096 10.1016/j.jcis.2020.08.083 10.1126/science.1186120 10.1002/aenm.201901973 10.1039/D1TA03339E 10.1016/j.apcatb.2019.117781 10.1021/acscatal.9b03246 10.1002/ange.202012357 10.1021/acsnano.1c06017 10.1039/D1QI00878A 10.1016/j.apsusc.2018.08.254 |
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Keywords | Bismuth molybdate Gadolinium doping Photocatalytic nitrogen reduction Redox regulation Two-dimensional |
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References | Li, Li, Liu, Ren, Miao, Li (b0125) 2019; 463 Yang, Zhao, Liu, Wang, Feng, Hu, Xue (b0080) 2022; 2022 Zhao, Hong, Yan, Choi, Jung, Liu, Liu, Li, Qiu, Sun (b0175) 2019; 55 Guan, Wang, Zhang, Liu, Xu, Wang, Zhao, Feng, Shang, Sun (b0030) 2021; 282 Zhang, Ran, Zhang, Zhai, Wu, Gao, Li, Zhang, Wang, Fan, Zhang, Cao, Jin, Sun, Hou (b0090) 2021; 15 Ma, Ren, Li, Liu, Li, Han, Li, Zhan, Khan, Chang, Sun, Zhou (b0185) 2021; 582 Y. Bai, L. Ye, T. Chen, L.i. Wang, X. Shi, X. Zhang, D. Chen, Facet-dependent photocatalytic N Li, Li, Gu, Liu, Li, Ren, Ma, Zhou (b0105) 2021; 851 Li, Li, Tao, Gu, Xie, Wu, Zhang, Wang, Zhang, Chang (b0070) 2021; 31 Liu, Han, Liang, Xue, Zhou, Zhang, Cui, Tian (b0085) 2022; 605 O fixation of bismuth-rich Bi Li, Li, Liu, Fan, Geng, Ma, Dong, Liu (b0120) 2021; 889 Liu, Gu, Zhao, Zhou, Li (b0135) 2020; 56 Li, Zhang, Feng, Bai, Ren (b0075) 2022; 607 Li, Li, Ma, Wei, Qiu, Guo, Shi, Zhang, Asiri, Chen, Tang, Sun (b0180) 2018; 8 Wu, Chen, Yue, Mine, Toyao, Matsuoka, Xi, Wang, Zhang (b0055) 2021; 11 Zhang, Zhao, Shi (b0100) 2020; 10 Hirshfeld (b0155) 1977; 44 Qiu, Huang, Dong, Chen, Zhao, Yu, Liu, Li, Wang (b0095) 2021; 9 I nanosheets. ACS Appl. Mater. Interf. 8 (2016) 27661–27668. Han, Wu, Jiao, Xu, Wang, Xie, Guo, Tang (b0020) 2021; 33 Li, Yang, Gao, Shen, Xue, Chen, Li (b0140) 2021; 404 Li, Liu, Tang, Huang, Cui, Mei, Zhong (b0205) 2020; 10 Zhang, Song, Ping, Du, Sun, Zhang, Qi, Miao, Li (b0170) 2021; 8 Canfield, Glazer, Falkowski (b0005) 2010; 330 He, Li, Qiu, Chen, Lu, Cui (b0050) 2021; 556 Li, Deng, Gu, Li, Tao, Chen, He, Wang, Zhang, Chang (b0190) 2022; 607 Wei, Jiang, Liu, Bai, Hao, Ni (b0035) 2022; 14 Meng, Li, Tung, Wu (b0025) 2021; 7 Van der Ham, Koper, Hetterscheid (b0010) 2014; 43 Liu, Luo, Ling, Shi, Zhan, Li, Gu, Wei, Guo, Ai, Zhang (b0040) 2022; 301 Zhang, Li, He, Ren, Zhang, Mi (b0065) 2021; 11 Fan, Jin, Liu, Liu (b0115) 2022; 2022 Grimme (b0150) 2006; 27 Li, Li, Liu, Li, Ren, Fan, Ma, Dong (b0110) 2021; 127 Liu, Xue, Hui, Yu, Fang, He, Li (b0060) 2021; 89 Wu, Xie, Ling, Si, Li, Wang, Ye, Zhao, Li, Zhao, Hou (b0130) 2020; 400 Fang, Xue, Hui, Yu, Li (b0045) 2021; 133 Tian, Zhang, Huang, He, Guo (b0165) 2014; 118 Li, Gu, Sun, Guo, Xie, Tao, He, Zhang, Chang (b0195) 2020; 8 Meng, Lv, Sun, Hong, Xing, Qiang, Chen, Jin (b0145) 2019; 256 Guo, Qiu, Li, Xu, Langford, Sun (b0160) 2021; 13 Shi, Zhao, Waterhouse, Zhang, Zhang (b0015) 2019; 9 Han (10.1016/j.apsusc.2022.154105_b0020) 2021; 33 Guan (10.1016/j.apsusc.2022.154105_b0030) 2021; 282 Li (10.1016/j.apsusc.2022.154105_b0070) 2021; 31 Liu (10.1016/j.apsusc.2022.154105_b0040) 2022; 301 Canfield (10.1016/j.apsusc.2022.154105_b0005) 2010; 330 Zhang (10.1016/j.apsusc.2022.154105_b0170) 2021; 8 Li (10.1016/j.apsusc.2022.154105_b0110) 2021; 127 Li (10.1016/j.apsusc.2022.154105_b0075) 2022; 607 Zhao (10.1016/j.apsusc.2022.154105_b0175) 2019; 55 Zhang (10.1016/j.apsusc.2022.154105_b0100) 2020; 10 Wu (10.1016/j.apsusc.2022.154105_b0130) 2020; 400 Li (10.1016/j.apsusc.2022.154105_b0120) 2021; 889 Meng (10.1016/j.apsusc.2022.154105_b0145) 2019; 256 Liu (10.1016/j.apsusc.2022.154105_b0135) 2020; 56 Li (10.1016/j.apsusc.2022.154105_b0140) 2021; 404 Tian (10.1016/j.apsusc.2022.154105_b0165) 2014; 118 Meng (10.1016/j.apsusc.2022.154105_b0025) 2021; 7 Wei (10.1016/j.apsusc.2022.154105_b0035) 2022; 14 Yang (10.1016/j.apsusc.2022.154105_b0080) 2022; 2022 Liu (10.1016/j.apsusc.2022.154105_b0085) 2022; 605 Hirshfeld (10.1016/j.apsusc.2022.154105_b0155) 1977; 44 Li (10.1016/j.apsusc.2022.154105_b0125) 2019; 463 Guo (10.1016/j.apsusc.2022.154105_b0160) 2021; 13 Van der Ham (10.1016/j.apsusc.2022.154105_b0010) 2014; 43 Fang (10.1016/j.apsusc.2022.154105_b0045) 2021; 133 Li (10.1016/j.apsusc.2022.154105_b0180) 2018; 8 Zhang (10.1016/j.apsusc.2022.154105_b0090) 2021; 15 Wu (10.1016/j.apsusc.2022.154105_b0055) 2021; 11 Zhang (10.1016/j.apsusc.2022.154105_b0065) 2021; 11 Fan (10.1016/j.apsusc.2022.154105_b0115) 2022; 2022 He (10.1016/j.apsusc.2022.154105_b0050) 2021; 556 Li (10.1016/j.apsusc.2022.154105_b0105) 2021; 851 Grimme (10.1016/j.apsusc.2022.154105_b0150) 2006; 27 Ma (10.1016/j.apsusc.2022.154105_b0185) 2021; 582 10.1016/j.apsusc.2022.154105_b0200 Qiu (10.1016/j.apsusc.2022.154105_b0095) 2021; 9 Li (10.1016/j.apsusc.2022.154105_b0190) 2022; 607 Li (10.1016/j.apsusc.2022.154105_b0205) 2020; 10 Liu (10.1016/j.apsusc.2022.154105_b0060) 2021; 89 Li (10.1016/j.apsusc.2022.154105_b0195) 2020; 8 Shi (10.1016/j.apsusc.2022.154105_b0015) 2019; 9 |
References_xml | – volume: 2022 start-page: 2102031 year: 2022 ident: b0080 article-title: Designing “Core–Shell” insoluble-SiW publication-title: Adv. Mater. Interf. contributor: fullname: Xue – volume: 8 start-page: 1801357 year: 2018 ident: b0180 article-title: Boosted electrocatalytic N publication-title: Adv. Energy Mater. contributor: fullname: Sun – volume: 301 start-page: 120766 year: 2022 ident: b0040 article-title: Rare earth La single atoms supported MoO publication-title: Appl. Catal. B: Environ. contributor: fullname: Zhang – volume: 10 start-page: 1901973 year: 2020 ident: b0100 article-title: Efficient photocatalytic nitrogen fixation over Cu publication-title: Adv. Energy Mater. contributor: fullname: Shi – volume: 56 start-page: 45 year: 2020 end-page: 68 ident: b0135 article-title: BiVO publication-title: J. Mater. Sci. Tech. contributor: fullname: Li – volume: 55 start-page: 7171 year: 2019 end-page: 7174 ident: b0175 article-title: Efficient visible-light driven N publication-title: Chem. Commun. contributor: fullname: Sun – volume: 8 start-page: 13038 year: 2020 end-page: 13048 ident: b0195 article-title: In–built bionic ‘‘MoFe–cofactor” in Fe–doped two–dimensional MoTe publication-title: J. Mater. Chem. A contributor: fullname: Chang – volume: 44 start-page: 129 year: 1977 end-page: 138 ident: b0155 article-title: Bonded-atom fragments for describing molecular charge densities publication-title: Theor. Chim. Acta contributor: fullname: Hirshfeld – volume: 607 start-page: 1625 year: 2022 end-page: 1632 ident: b0190 article-title: Engineering of bionic Fe/Mo bimetallene for boosting the photocatalytic nitrogen reduction performance publication-title: J. Colloid Interf. Sci. contributor: fullname: Chang – volume: 607 start-page: 1323 year: 2022 end-page: 1332 ident: b0075 article-title: Electrostatic self-assembly to form unique LiNbO publication-title: J. Colloid Interf. Sci. contributor: fullname: Ren – volume: 27 start-page: 1787 year: 2006 end-page: 1799 ident: b0150 article-title: Semiempirical GGA-type density functional constructed with a long-range dispersion correction publication-title: J. Comput. Chem. contributor: fullname: Grimme – volume: 556 start-page: 149753 year: 2021 ident: b0050 article-title: Nonlinear optical polarization and heterostructure synergistically boosted the built-in electric field of CeF publication-title: Appl. Surf. Sci. contributor: fullname: Cui – volume: 8 start-page: 4720 year: 2021 end-page: 4729 ident: b0170 article-title: A biodegradable bismuth–gadolinium-based nano contrast agent for accurate identification and imaging of renal insufficiency in vivo publication-title: Inorg. Chem. Front. contributor: fullname: Li – volume: 89 start-page: 106333 year: 2021 ident: b0060 article-title: Porous graphdiyne loading CoO publication-title: Nano Energy contributor: fullname: Li – volume: 11 start-page: 4362 year: 2021 end-page: 4371 ident: b0055 article-title: Single-atom high-valent Fe (IV) for promoted photocatalytic nitrogen hydrogenation on porous TiO publication-title: ACS Catal. contributor: fullname: Zhang – volume: 31 start-page: 2010901 year: 2021 ident: b0070 article-title: Two-dimensional metal telluride atomic crystals (2D MTACs): preparation, physical properties and applications publication-title: Adv. Funct. Mater. contributor: fullname: Chang – volume: 2022 start-page: 2104579 year: 2022 ident: b0115 article-title: One-step MOF-templated strategy to fabrication of Ce-doped ZnIn publication-title: Adv. Sci. contributor: fullname: Liu – volume: 9 start-page: 9739 year: 2019 end-page: 9750 ident: b0015 article-title: Defect engineering in photocatalytic nitrogen fixation publication-title: ACS Catal. contributor: fullname: Zhang – volume: 118 start-page: 15640 year: 2014 end-page: 15648 ident: b0165 article-title: Influences of Gd substitution on the crystal structure and visible-light-driven photocatalytic performance of Bi publication-title: J. Phys. Chem. C contributor: fullname: Guo – volume: 10 start-page: 2431 year: 2020 end-page: 2442 ident: b0205 article-title: Single-atom Pt−N publication-title: ACS Catal. contributor: fullname: Zhong – volume: 11 start-page: 2003294 year: 2021 ident: b0065 article-title: Recent progress in 2D catalysts for photocatalytic and electrocatalytic artificial nitrogen reduction to ammonia publication-title: Adv. Energy Mater. contributor: fullname: Mi – volume: 256 start-page: 117781 year: 2019 ident: b0145 article-title: High-efficiency Fe-mediated Bi publication-title: Appl. Catal. B: Environ. contributor: fullname: Jin – volume: 851 start-page: 156935 year: 2021 ident: b0105 article-title: Efficient ytterbium-doped Bi publication-title: J. Alloy. Compd. contributor: fullname: Zhou – volume: 605 start-page: 320 year: 2022 end-page: 329 ident: b0085 article-title: Phosphorous-doped 1T-MoS publication-title: J. Colloid Interf. Sci. contributor: fullname: Tian – volume: 15 start-page: 17820 year: 2021 end-page: 17830 ident: b0090 article-title: Two-dimensional defective boron-doped niobic acid nanosheets for robust nitrogen photofixation publication-title: ACS nano contributor: fullname: Hou – volume: 404 start-page: 127115 year: 2021 ident: b0140 article-title: Creation of rich oxygen vacancies in bismuth molybdate nanosheets to boost the photocatalytic nitrogen fixation performance under visible light illumination publication-title: Chem. Eng. J. contributor: fullname: Li – volume: 43 start-page: 5183 year: 2014 end-page: 5191 ident: b0010 article-title: Challenges in reduction of dinitrogen by proton and electron transfer publication-title: Chem. Soc. Rev. contributor: fullname: Hetterscheid – volume: 889 start-page: 161757 year: 2021 ident: b0120 article-title: Novel Yb publication-title: J. Alloy. Compd. contributor: fullname: Liu – volume: 463 start-page: 556 year: 2019 end-page: 565 ident: b0125 article-title: Engineering of Gd/Er/Lu triple-doped Bi publication-title: Appl. Surf. Sci. contributor: fullname: Li – volume: 330 start-page: 192 year: 2010 end-page: 196 ident: b0005 article-title: The evolution and future of Earth’s nitrogen cycle publication-title: Science contributor: fullname: Falkowski – volume: 14 start-page: 2990 year: 2022 end-page: 2997 ident: b0035 article-title: Recent advances in photocatalytic nitrogen fixation and beyond publication-title: Nanoscale contributor: fullname: Ni – volume: 582 start-page: 488 year: 2021 end-page: 495 ident: b0185 article-title: A novel noble-metal-free Mo publication-title: J. Colloid Interf. Sci. contributor: fullname: Zhou – volume: 9 start-page: 14459 year: 2021 end-page: 14465 ident: b0095 article-title: Plasmonic gold nanocrystals simulated efficient photocatalytic nitrogen fixation over Mo doped W publication-title: J. Mater. Chem. A contributor: fullname: Wang – volume: 7 start-page: 1431 year: 2021 end-page: 1450 ident: b0025 article-title: Nitrogenase inspired artificial photosynthetic nitrogen fixation publication-title: Chem contributor: fullname: Wu – volume: 133 start-page: 3207 year: 2021 end-page: 3211 ident: b0045 article-title: Graphdiyne@Janus magnetite for photocatalytic nitrogen fixation publication-title: Angew. Chem. contributor: fullname: Li – volume: 282 start-page: 119580 year: 2021 ident: b0030 article-title: Enhanced photocatalytic N publication-title: Appl. Catal. B: Environ. contributor: fullname: Sun – volume: 400 start-page: 125944 year: 2020 ident: b0130 article-title: One-step synthesis and Gd publication-title: Chem. Eng. J. contributor: fullname: Hou – volume: 13 start-page: 1239 year: 2021 end-page: 1245 ident: b0160 article-title: Electrocatalytic nitrogen reduction performance of Si-doped 2D nanosheets of boron nitride evaluated via density functional theory publication-title: ChemCatChem contributor: fullname: Sun – volume: 33 start-page: 2008180 year: 2021 ident: b0020 article-title: Rational design of high-concentration Ti publication-title: Adv. Mater. contributor: fullname: Tang – volume: 127 start-page: 265 year: 2021 end-page: 275 ident: b0110 article-title: Insights into the in-built Tb publication-title: J. Taiwan Inst. Chem. E. contributor: fullname: Dong – volume: 301 start-page: 120766 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0040 article-title: Rare earth La single atoms supported MoO3-x for efficient photocatalytic nitrogen fixation publication-title: Appl. Catal. B: Environ. doi: 10.1016/j.apcatb.2021.120766 contributor: fullname: Liu – volume: 11 start-page: 4362 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0055 article-title: Single-atom high-valent Fe (IV) for promoted photocatalytic nitrogen hydrogenation on porous TiO2-SiO2 publication-title: ACS Catal. doi: 10.1021/acscatal.1c00072 contributor: fullname: Wu – volume: 7 start-page: 1431 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0025 article-title: Nitrogenase inspired artificial photosynthetic nitrogen fixation publication-title: Chem doi: 10.1016/j.chempr.2020.11.002 contributor: fullname: Meng – volume: 33 start-page: 2008180 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0020 article-title: Rational design of high-concentration Ti3+ in porous carbon-doped TiO2 nanosheets for efficient photocatalytic ammonia synthesis publication-title: Adv. Mater. doi: 10.1002/adma.202008180 contributor: fullname: Han – volume: 14 start-page: 2990 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0035 article-title: Recent advances in photocatalytic nitrogen fixation and beyond publication-title: Nanoscale doi: 10.1039/D2NR00198E contributor: fullname: Wei – volume: 31 start-page: 2010901 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0070 article-title: Two-dimensional metal telluride atomic crystals (2D MTACs): preparation, physical properties and applications publication-title: Adv. Funct. Mater. doi: 10.1002/adfm.202010901 contributor: fullname: Li – volume: 8 start-page: 13038 year: 2020 ident: 10.1016/j.apsusc.2022.154105_b0195 article-title: In–built bionic ‘‘MoFe–cofactor” in Fe–doped two–dimensional MoTe2 nanosheets for boosting the photocatalytic nitrogen reduction performance publication-title: J. Mater. Chem. A doi: 10.1039/D0TA04251J contributor: fullname: Li – volume: 607 start-page: 1323 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0075 article-title: Electrostatic self-assembly to form unique LiNbO3/ZnS core-shell structure for photocatalytic nitrate reduction enhancement publication-title: J. Colloid Interf. Sci. doi: 10.1016/j.jcis.2021.09.069 contributor: fullname: Li – volume: 851 start-page: 156935 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0105 article-title: Efficient ytterbium-doped Bi2WO6 photocatalysts: synthesis, the formation of oxygen vacancies and boosted superoxide yield for enhanced visible-light photocatalytic activity publication-title: J. Alloy. Compd. doi: 10.1016/j.jallcom.2020.156935 contributor: fullname: Li – volume: 2022 start-page: 2104579 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0115 article-title: One-step MOF-templated strategy to fabrication of Ce-doped ZnIn2S4 tetrakaidecahedron hollow nanocages as an efficient photocatalyst for hydrogen evolution publication-title: Adv. Sci. doi: 10.1002/advs.202104579 contributor: fullname: Fan – volume: 2022 start-page: 2102031 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0080 article-title: Designing “Core–Shell” insoluble-SiW11Fe@δ-Bi2O3 Z-scheme heterojunction for photo-driven nitrogen reduction reaction and evaluating the impact of oxygen toward nitrogen reduction publication-title: Adv. Mater. Interf. doi: 10.1002/admi.202102031 contributor: fullname: Yang – volume: 556 start-page: 149753 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0050 article-title: Nonlinear optical polarization and heterostructure synergistically boosted the built-in electric field of CeF3/LiNbO3 for a higher photocatalytic nitrogen reduction activity publication-title: Appl. Surf. Sci. doi: 10.1016/j.apsusc.2021.149753 contributor: fullname: He – volume: 605 start-page: 320 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0085 article-title: Phosphorous-doped 1T-MoS2 decorated nitrogen-doped g-C3N4 nanosheets for enhanced photocatalytic nitrogen fixation publication-title: J. Colloid Interf. Sci. doi: 10.1016/j.jcis.2021.07.111 contributor: fullname: Liu – ident: 10.1016/j.apsusc.2022.154105_b0200 doi: 10.1021/acsami.6b08129 – volume: 89 start-page: 106333 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0060 article-title: Porous graphdiyne loading CoOx quantum dots for fixation nitrogen reaction publication-title: Nano Energy doi: 10.1016/j.nanoen.2021.106333 contributor: fullname: Liu – volume: 11 start-page: 2003294 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0065 article-title: Recent progress in 2D catalysts for photocatalytic and electrocatalytic artificial nitrogen reduction to ammonia publication-title: Adv. Energy Mater. doi: 10.1002/aenm.202003294 contributor: fullname: Zhang – volume: 10 start-page: 2431 year: 2020 ident: 10.1016/j.apsusc.2022.154105_b0205 article-title: Single-atom Pt−N3 sites on the stable covalent triazine framework nanosheets for photocatalytic N2 fixation publication-title: ACS Catal. doi: 10.1021/acscatal.9b04925 contributor: fullname: Li – volume: 8 start-page: 1801357 year: 2018 ident: 10.1016/j.apsusc.2022.154105_b0180 article-title: Boosted electrocatalytic N2 reduction to NH3 by defect-rich MoS2 nanoflower publication-title: Adv. Energy Mater. doi: 10.1002/aenm.201801357 contributor: fullname: Li – volume: 43 start-page: 5183 year: 2014 ident: 10.1016/j.apsusc.2022.154105_b0010 article-title: Challenges in reduction of dinitrogen by proton and electron transfer publication-title: Chem. Soc. Rev. doi: 10.1039/C4CS00085D contributor: fullname: Van der Ham – volume: 56 start-page: 45 year: 2020 ident: 10.1016/j.apsusc.2022.154105_b0135 article-title: BiVO4, Bi2WO6 and Bi2MoO6 photocatalysis: a brief review publication-title: J. Mater. Sci. Tech. doi: 10.1016/j.jmst.2020.04.023 contributor: fullname: Liu – volume: 55 start-page: 7171 issue: 50 year: 2019 ident: 10.1016/j.apsusc.2022.154105_b0175 article-title: Efficient visible-light driven N2 fixation over two-dimensional Sb/TiO2 composites publication-title: Chem. Commun. doi: 10.1039/C9CC02291K contributor: fullname: Zhao – volume: 127 start-page: 265 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0110 article-title: Insights into the in-built Tb4+/Tb3+ redox centers for boosted hydroxyl radical yield and superior separation of charge carriers by investigating Tb2O3/g-C3N4 composite photocatalysts publication-title: J. Taiwan Inst. Chem. E. doi: 10.1016/j.jtice.2021.08.027 contributor: fullname: Li – volume: 404 start-page: 127115 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0140 article-title: Creation of rich oxygen vacancies in bismuth molybdate nanosheets to boost the photocatalytic nitrogen fixation performance under visible light illumination publication-title: Chem. Eng. J. doi: 10.1016/j.cej.2020.127115 contributor: fullname: Li – volume: 889 start-page: 161757 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0120 article-title: Novel Yb3+/Nd3+ co-doped bismuth tungstate for excellent photocatalytic performance: construction and synergistic effect of oxygen vacancies and in-built Yb3+/Yb2+ redox center publication-title: J. Alloy. Compd. doi: 10.1016/j.jallcom.2021.161757 contributor: fullname: Li – volume: 400 start-page: 125944 year: 2020 ident: 10.1016/j.apsusc.2022.154105_b0130 article-title: One-step synthesis and Gd3+ decoration of BiOBr microspheres consisting of nanosheets toward improving photocatalytic reduction of CO2 into hydrocarbon fuel publication-title: Chem. Eng. J. doi: 10.1016/j.cej.2020.125944 contributor: fullname: Wu – volume: 607 start-page: 1625 year: 2022 ident: 10.1016/j.apsusc.2022.154105_b0190 article-title: Engineering of bionic Fe/Mo bimetallene for boosting the photocatalytic nitrogen reduction performance publication-title: J. Colloid Interf. Sci. doi: 10.1016/j.jcis.2021.09.078 contributor: fullname: Li – volume: 282 start-page: 119580 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0030 article-title: Enhanced photocatalytic N2 fixation via defective and fluoride modified TiO2 surface publication-title: Appl. Catal. B: Environ. doi: 10.1016/j.apcatb.2020.119580 contributor: fullname: Guan – volume: 13 start-page: 1239 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0160 article-title: Electrocatalytic nitrogen reduction performance of Si-doped 2D nanosheets of boron nitride evaluated via density functional theory publication-title: ChemCatChem doi: 10.1002/cctc.202001775 contributor: fullname: Guo – volume: 118 start-page: 15640 year: 2014 ident: 10.1016/j.apsusc.2022.154105_b0165 article-title: Influences of Gd substitution on the crystal structure and visible-light-driven photocatalytic performance of Bi2WO6 publication-title: J. Phys. Chem. C doi: 10.1021/jp500645p contributor: fullname: Tian – volume: 27 start-page: 1787 year: 2006 ident: 10.1016/j.apsusc.2022.154105_b0150 article-title: Semiempirical GGA-type density functional constructed with a long-range dispersion correction publication-title: J. Comput. Chem. doi: 10.1002/jcc.20495 contributor: fullname: Grimme – volume: 44 start-page: 129 year: 1977 ident: 10.1016/j.apsusc.2022.154105_b0155 article-title: Bonded-atom fragments for describing molecular charge densities publication-title: Theor. Chim. Acta doi: 10.1007/BF00549096 contributor: fullname: Hirshfeld – volume: 582 start-page: 488 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0185 article-title: A novel noble-metal-free Mo2C-In2S3 heterojunction photocatalyst with efficient charge separation for enhanced photocatalytic H2 evolution under visible light publication-title: J. Colloid Interf. Sci. doi: 10.1016/j.jcis.2020.08.083 contributor: fullname: Ma – volume: 330 start-page: 192 year: 2010 ident: 10.1016/j.apsusc.2022.154105_b0005 article-title: The evolution and future of Earth’s nitrogen cycle publication-title: Science doi: 10.1126/science.1186120 contributor: fullname: Canfield – volume: 10 start-page: 1901973 year: 2020 ident: 10.1016/j.apsusc.2022.154105_b0100 article-title: Efficient photocatalytic nitrogen fixation over Cuδ+-modified defective ZnAl-layered double hydroxide nanosheets publication-title: Adv. Energy Mater. doi: 10.1002/aenm.201901973 contributor: fullname: Zhang – volume: 9 start-page: 14459 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0095 article-title: Plasmonic gold nanocrystals simulated efficient photocatalytic nitrogen fixation over Mo doped W18O49 nanowires publication-title: J. Mater. Chem. A doi: 10.1039/D1TA03339E contributor: fullname: Qiu – volume: 256 start-page: 117781 year: 2019 ident: 10.1016/j.apsusc.2022.154105_b0145 article-title: High-efficiency Fe-mediated Bi2MoO6 nitrogen–fixing photocatalyst: reduced surface work function and ameliorated surface reaction publication-title: Appl. Catal. B: Environ. doi: 10.1016/j.apcatb.2019.117781 contributor: fullname: Meng – volume: 9 start-page: 9739 year: 2019 ident: 10.1016/j.apsusc.2022.154105_b0015 article-title: Defect engineering in photocatalytic nitrogen fixation publication-title: ACS Catal. doi: 10.1021/acscatal.9b03246 contributor: fullname: Shi – volume: 133 start-page: 3207 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0045 article-title: Graphdiyne@Janus magnetite for photocatalytic nitrogen fixation publication-title: Angew. Chem. doi: 10.1002/ange.202012357 contributor: fullname: Fang – volume: 15 start-page: 17820 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0090 article-title: Two-dimensional defective boron-doped niobic acid nanosheets for robust nitrogen photofixation publication-title: ACS nano doi: 10.1021/acsnano.1c06017 contributor: fullname: Zhang – volume: 8 start-page: 4720 year: 2021 ident: 10.1016/j.apsusc.2022.154105_b0170 article-title: A biodegradable bismuth–gadolinium-based nano contrast agent for accurate identification and imaging of renal insufficiency in vivo publication-title: Inorg. Chem. Front. doi: 10.1039/D1QI00878A contributor: fullname: Zhang – volume: 463 start-page: 556 year: 2019 ident: 10.1016/j.apsusc.2022.154105_b0125 article-title: Engineering of Gd/Er/Lu triple-doped Bi2MoO6 to synergistically boost the photocatalytic performance in three different aspects: oxidizability, light absorption and charge separation publication-title: Appl. Surf. Sci. doi: 10.1016/j.apsusc.2018.08.254 contributor: fullname: Li |
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