NaLa2SbO6:Mn4+ far-red phosphor: Synthesis, luminescence properties and emission enhancement by Al3+ ions

A novel far-red emission NaLa2SbO6(NLSO):Mn4+ phosphor was prepared by traditional high temperature solid state reaction method. In the range of 200–600 nm, NLSO:Mn4+ phosphors exhibit broad excitation band centered at 322 nm and 498 nm. Under the excitation of 322 nm, the phosphor exhibits a far-re...

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Published inJournal of luminescence Vol. 219; p. 116865
Main Authors Shi, Lei, Han, Ya-jie, Wang, Shuang, Ma, Di, Mao, Zhi-yong, Wang, Da-jian, Li, Xi-ze, Zhang, Lu, Zhang, Zhi-wei, Lu, Xu-lin
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.03.2020
Subjects
NLSO:Mn4
Photoluminescence
Plant cultivation and growth LEDs
Red phosphors
Plant cultivation and growth LEDs
Red phosphors
Photoluminescence
NLSO:Mn4
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Abstract A novel far-red emission NaLa2SbO6(NLSO):Mn4+ phosphor was prepared by traditional high temperature solid state reaction method. In the range of 200–600 nm, NLSO:Mn4+ phosphors exhibit broad excitation band centered at 322 nm and 498 nm. Under the excitation of 322 nm, the phosphor exhibits a far-red emission band centered at 707 nm in the range of 600–800 nm. In NLSO:Mn4+ phosphors, the optimum doping concentration is x = 0.003. In addition, the effect of Al3+-doped on the luminescent properties of the materials was also studied. The optimum doping concentration of Al3+ is x = 0.004, and the luminescence intensity of Mn4+ can be increased by 53%. In addition, NLSO:0.003Mn4+, 0.004Al3+ phosphors have high internal quantum efficiency and good thermal stability. The CIE chromaticity coordinates of NLSO:0.003Mn4+, yAl3+ phosphors are calculated, and which are located in the far-red region. All the results show that the synthesized phosphors have great application prospects in plant cultivation. •Novel-type far-red emit phosphors NaLa2SbO6(NLSO):Mn4+ were synthesized by solid state reaction.•When the doping concentration of Al3+ is 0.4%, the PL intensity of NaLa2SbO6:Mn4+, Al3+ reaches the maximum.•At 423 K, the PL intensity of NaLa2SbO6:0.003Mn4+ decreased to 42.75% of the initial PL intensity.•The activation energy (Ea) of NaLa2SbO6:0.003Mn4+ and NaLa2SbO6:0.003Mn4+, 0.004Al3+ are 0.355 eV and 0.392 eV, respectively.
AbstractList A novel far-red emission NaLa2SbO6(NLSO):Mn4+ phosphor was prepared by traditional high temperature solid state reaction method. In the range of 200–600 nm, NLSO:Mn4+ phosphors exhibit broad excitation band centered at 322 nm and 498 nm. Under the excitation of 322 nm, the phosphor exhibits a far-red emission band centered at 707 nm in the range of 600–800 nm. In NLSO:Mn4+ phosphors, the optimum doping concentration is x = 0.003. In addition, the effect of Al3+-doped on the luminescent properties of the materials was also studied. The optimum doping concentration of Al3+ is x = 0.004, and the luminescence intensity of Mn4+ can be increased by 53%. In addition, NLSO:0.003Mn4+, 0.004Al3+ phosphors have high internal quantum efficiency and good thermal stability. The CIE chromaticity coordinates of NLSO:0.003Mn4+, yAl3+ phosphors are calculated, and which are located in the far-red region. All the results show that the synthesized phosphors have great application prospects in plant cultivation. •Novel-type far-red emit phosphors NaLa2SbO6(NLSO):Mn4+ were synthesized by solid state reaction.•When the doping concentration of Al3+ is 0.4%, the PL intensity of NaLa2SbO6:Mn4+, Al3+ reaches the maximum.•At 423 K, the PL intensity of NaLa2SbO6:0.003Mn4+ decreased to 42.75% of the initial PL intensity.•The activation energy (Ea) of NaLa2SbO6:0.003Mn4+ and NaLa2SbO6:0.003Mn4+, 0.004Al3+ are 0.355 eV and 0.392 eV, respectively.
ArticleNumber 116865
Author Mao, Zhi-yong
Zhang, Lu
Li, Xi-ze
Shi, Lei
Wang, Shuang
Zhang, Zhi-wei
Ma, Di
Lu, Xu-lin
Han, Ya-jie
Wang, Da-jian
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Keywords Plant cultivation and growth LEDs
Red phosphors
Photoluminescence
NLSO:Mn4
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Snippet A novel far-red emission NaLa2SbO6(NLSO):Mn4+ phosphor was prepared by traditional high temperature solid state reaction method. In the range of 200–600 nm,...
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SubjectTerms NLSO:Mn4
Photoluminescence
Plant cultivation and growth LEDs
Red phosphors
Title NaLa2SbO6:Mn4+ far-red phosphor: Synthesis, luminescence properties and emission enhancement by Al3+ ions
URI https://dx.doi.org/10.1016/j.jlumin.2019.116865
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