The influence of pH value on nitrate and nitrite formation in air-plasma-treated aqueous solutions
A DC air discharge plasma is operated over an aqueous solution of Na 2 SO 4 . Nitrate and nitrite are formed in the solution after the plasma treatment. In order to trace the origin of the nitrate and nitrite, we investigated the processes of the nitrate and nitrite formation as a function of the so...
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| Published in | Plasma science & technology Vol. 27; no. 9; pp. 95508 - 95512 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Plasma Science and Technology
01.09.2025
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1009-0630 2058-6272 |
| DOI | 10.1088/2058-6272/adf039 |
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| Abstract | A DC air discharge plasma is operated over an aqueous solution of Na 2 SO 4 . Nitrate and nitrite are formed in the solution after the plasma treatment. In order to trace the origin of the nitrate and nitrite, we investigated the processes of the nitrate and nitrite formation as a function of the solution’s pH value. We measured the nitrate with a nitrate ion selective electrode and the nitrite with Griess assay. The results show that air is activated to form nitrogen oxides by discharge plasma, and the dissolution of these nitrogen oxides leads to the formation of nitrate and nitrite. The total nitrogen content of the nitrate and nitrite in the solution is independent, while the nitrate and nitrite production rates are dependent on the solution’s pH value. A high pH environment is beneficial for nitrite formation, while a low pH environment is better for nitrate production. Moreover, the production rates of both nitrate and nitrite are greater in the solution cathode than those in the solution anode. |
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| AbstractList | A DC air discharge plasma is operated over an aqueous solution of Na 2 SO 4 . Nitrate and nitrite are formed in the solution after the plasma treatment. In order to trace the origin of the nitrate and nitrite, we investigated the processes of the nitrate and nitrite formation as a function of the solution’s pH value. We measured the nitrate with a nitrate ion selective electrode and the nitrite with Griess assay. The results show that air is activated to form nitrogen oxides by discharge plasma, and the dissolution of these nitrogen oxides leads to the formation of nitrate and nitrite. The total nitrogen content of the nitrate and nitrite in the solution is independent, while the nitrate and nitrite production rates are dependent on the solution’s pH value. A high pH environment is beneficial for nitrite formation, while a low pH environment is better for nitrate production. Moreover, the production rates of both nitrate and nitrite are greater in the solution cathode than those in the solution anode. |
| Author | ZHANG, Mingjia LIN, Taiyu CHEN, Qiang LIU, Guangchao WU, Binhong WANG, Xin |
| Author_xml | – sequence: 1 givenname: Mingjia surname: ZHANG fullname: ZHANG, Mingjia organization: Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, Fujian Provincial Key Laboratory of Electromagnetic Wave Science and Detection Technology, Xiamen Key Laboratory of Multiphysics Electronic Information, Institute of Electromagnetics and Acoustics, Xiamen University, Xiamen 361005, People’s Republic of China – sequence: 2 givenname: Taiyu surname: LIN fullname: LIN, Taiyu organization: Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, Fujian Provincial Key Laboratory of Electromagnetic Wave Science and Detection Technology, Xiamen Key Laboratory of Multiphysics Electronic Information, Institute of Electromagnetics and Acoustics, Xiamen University, Xiamen 361005, People’s Republic of China – sequence: 3 givenname: Guangchao surname: LIU fullname: LIU, Guangchao organization: Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, Fujian Provincial Key Laboratory of Electromagnetic Wave Science and Detection Technology, Xiamen Key Laboratory of Multiphysics Electronic Information, Institute of Electromagnetics and Acoustics, Xiamen University, Xiamen 361005, People’s Republic of China – sequence: 4 givenname: Binhong surname: WU fullname: WU, Binhong organization: Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, Fujian Provincial Key Laboratory of Electromagnetic Wave Science and Detection Technology, Xiamen Key Laboratory of Multiphysics Electronic Information, Institute of Electromagnetics and Acoustics, Xiamen University, Xiamen 361005, People’s Republic of China – sequence: 5 givenname: Xin surname: WANG fullname: WANG, Xin organization: Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, Fujian Provincial Key Laboratory of Electromagnetic Wave Science and Detection Technology, Xiamen Key Laboratory of Multiphysics Electronic Information, Institute of Electromagnetics and Acoustics, Xiamen University, Xiamen 361005, People’s Republic of China – sequence: 6 givenname: Qiang surname: CHEN fullname: CHEN, Qiang organization: Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, Fujian Provincial Key Laboratory of Electromagnetic Wave Science and Detection Technology, Xiamen Key Laboratory of Multiphysics Electronic Information, Institute of Electromagnetics and Acoustics, Xiamen University, Xiamen 361005, People’s Republic of China |
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| SubjectTerms | air discharge plasma nitrate nitrite pH value plasma-liquid interface |
| Title | The influence of pH value on nitrate and nitrite formation in air-plasma-treated aqueous solutions |
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