Effects of Fe on Oxidation of Ni-20Cr and Ni-30Cr Alloys at 800 °C in Wet CO2 Gas
The oxidation behaviour of model alloys Ni-(20, 30)Cr (wt.%) with (0, 1, 5, 15%) Fe was investigated at 800 °C in Ar-20%CO 2 -20%H 2 O gas. All 20Cr alloys developed a multilayered scale, and the outer scale layers on alloys containing iron were subject to spallation. However, all 30Cr alloys develo...
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| Published in | High temperature corrosion of materials Vol. 94; no. 3-4; pp. 219 - 233 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
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01.10.2020
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| Abstract | The oxidation behaviour of model alloys Ni-(20, 30)Cr (wt.%) with (0, 1, 5, 15%) Fe was investigated at 800 °C in Ar-20%CO
2
-20%H
2
O gas. All 20Cr alloys developed a multilayered scale, and the outer scale layers on alloys containing iron were subject to spallation. However, all 30Cr alloys developed a scale which was predominantly chromia scale and resisted spallation. These effects are discussed in terms of Fe alloying effects on oxide scale development in the presence of water vapour. Differences between scaling behaviour in wet and dry CO
2
are shown to be explained by changed oxide transport properties. |
|---|---|
| AbstractList | The oxidation behaviour of model alloys Ni-(20, 30)Cr (wt.%) with (0, 1, 5, 15%) Fe was investigated at 800 °C in Ar-20%CO
2
-20%H
2
O gas. All 20Cr alloys developed a multilayered scale, and the outer scale layers on alloys containing iron were subject to spallation. However, all 30Cr alloys developed a scale which was predominantly chromia scale and resisted spallation. These effects are discussed in terms of Fe alloying effects on oxide scale development in the presence of water vapour. Differences between scaling behaviour in wet and dry CO
2
are shown to be explained by changed oxide transport properties. The oxidation behaviour of model alloys Ni-(20, 30)Cr (wt.%) with (0, 1, 5, 15%) Fe was investigated at 800 °C in Ar-20%CO2-20%H2O gas. All 20Cr alloys developed a multilayered scale, and the outer scale layers on alloys containing iron were subject to spallation. However, all 30Cr alloys developed a scale which was predominantly chromia scale and resisted spallation. These effects are discussed in terms of Fe alloying effects on oxide scale development in the presence of water vapour. Differences between scaling behaviour in wet and dry CO2 are shown to be explained by changed oxide transport properties. |
| Author | Zhang, Jianqiang Young, David J. Xie, Yun |
| Author_xml | – sequence: 1 givenname: Yun surname: Xie fullname: Xie, Yun organization: School of Materials Science and Engineering, University of New South Wales – sequence: 2 givenname: Jianqiang orcidid: 0000-0002-9331-4601 surname: Zhang fullname: Zhang, Jianqiang email: j.q.zhang@unsw.edu.au organization: School of Materials Science and Engineering, University of New South Wales – sequence: 3 givenname: David J. surname: Young fullname: Young, David J. organization: School of Materials Science and Engineering, University of New South Wales |
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| Cites_doi | 10.15302/J-ENG-2015031 10.3184/096034009X438185 10.1002/bbpc.19590630713 10.3184/096034005782744443 10.1007/s11085-010-9215-5 10.1179/mht.2000.17.2.008 10.1016/j.corsci.2020.108777 10.1016/S0010-938X(65)90500-7 10.4028/www.scientific.net/MSF.696.200 10.1016/j.corsci.2006.02.002 10.1016/j.corsci.2019.04.007 10.3139/146.110271 10.1016/S0364-5916(02)00037-8 10.1179/0960340914Z.000000000108 10.1149/1.2779605 10.1016/j.scriptamat.2007.06.050 10.1016/j.msea.2007.05.035 10.4028/www.scientific.net/MSF.595-598.1189 10.1149/1.2425624 10.1007/s11085-018-9873-2 10.1016/j.corsci.2018.02.022 10.1016/j.corsci.2017.08.003 10.1007/BF00665448 10.4028/www.scientific.net/MSF.369-372.231 10.1016/j.corsci.2011.03.015 10.1016/j.corsci.2018.10.029 10.1361/10599490524039 10.1016/j.corsci.2018.03.023 |
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| References | J. Ehlers, D. J. Young, E. J. Smaardijk, A. K. Tyagi, H. J. Penkalla, L. Singheiser and W. J. Quadakkers, Enhanced oxidation of the 9%Cr steel P91 in water vapour containing environments, Corrosion Science48, 3428–3454 (2006). M.-C. Demizieux, C. Desgranges, L. Martinelli, J. Favergeon and K. Ginestar, Morphology and buckling of the oxide scale after Fe-9Cr steel oxidation in water vapor environment, Oxidation of Metals91, 191–212 (2019). E. A. Polman, T. Fransen and P. J. Gellings, Oxidation kinetics of chromium and morphological phenomena, Oxidation of Metals32, 433–447 (1989). C. T. Fujii and R. A. Meussner, Oxide structures produced on iron-chromium alloys by a dissociative mechanism, Journal of the Electrochemical Society110, 1195–1204 (1963). Y.-X. Xu, W.-Y. Li and X.-W. Yang, Influence of alloyed Fe on corrosion of Ni-Cr alloys in molten silicates and the effects of pre-oxidation treatment, Corrosion Science134, 179–188 (2018). D. Huenert and A. Kranzmann, Impact of oxyfuel atmospheres H2O/CO2/O2 and H2O/CO2 on the oxidation of ferritic-martensitic and austenitic steels, Corrosion Science53, 2306–2317 (2011). R. Viswanathan, J. F. Henry, J. Tanzosh, G. Stanko, J. Shingledecker, B. Vitalis and R. Purgert, U.S. program on materials technology for ultra-supercritical coal power plants, Journal of Materials Engineering and Performance14, 281–292 (2005). C. Wagner, Reaktionstypen bei der oxydation von legierungen, Zeitschrift für Elektrochemie63, 772–782 (1959). J. O. Andersson, T. Helander, L. Höglund, P. Shi and B. Sundman, Thermo-Calc & DICTRA, computational tools for materials science, CALPHAD26, 273–312 (2002). A. Galerie, J. P. Petit, Y. Wouters, J. Mougin, A. Srisrual and P. Y. Hou, Water vapour effects on the oxidation of chromia-forming alloys, Materials Science Forum696, 200–205 (2011). J. Zurek, D. J. Young, E. Essuman, M. Hänsel, H. J. Penkalla, L. Niewolak and W. J. Quadakkers, Growth and adherence of chromia based surface scales on Ni-base alloys in high- and low-pO2 gases, Materials Science and Engineering, A477, 259–270 (2008). C. Wagner, Theoretical analysis of the diffusion processes determining the oxidation rate of alloys, Journal of the Electrochemical Society99, 369–380 (1952). F. Abe, Research and development of heat-resistant materials for advanced USC power plants with steam temperatures of 700°C and above, Engineering1, 211–224 (2015). G. H. Meier, K. Jung, N. Mu, N. M. Yanar, F. S. Pettit, J. Pirón Abellán, T. Olszewski, L. Nieto Hierro, W. J. Quadakkers and G. R. Holcomb, Effect of alloy composition and exposure conditions on the selective oxidation behavior of ferritic Fe-Cr and Fe-Cr-X alloys, Oxidation of Metals74, 319–340 (2010). Y. Xie, T. D. Nguyen, J. Zhang and D. J. Young, Corrosion behaviour of Ni-Cr alloys in wet CO2 atmosphere at 700 and 800°C, Corrosion Science146, 28–43 (2019). A. Rahmel and J. Tobolski, Einfluss von wasserdampf und kohlendioxyd auf die oxydation von eisen in sauerstoff bei hohen temperaturen, Corrosion Science5, 333–346 (1965). J. P. Abellán, T. Olszewski, G. H. Meier, L. Singheiser and W. J. Quadakkers, The oxidation behaviour of the 9%Cr steel P92 in CO2- and H2O-rich gases relevant to oxyfuel environments, International Journal of Materials Research101, 287–299 (2010). A. Galerie, Y. Wouters and M. Caillet, The kinetic behaviour of metals in water vapour at high temperatures: can general rules be proposed? Materials Science Forum369–372, 231–238 (2001). Y. Xie, T. Liang, J. Zhang and D. J. Young, Effects of Fe on oxidation of Ni-20Cr and Ni-30Cr alloys at 800°C in dry CO2 gas, Corrosion Science 173, 108777 (2020). Y. Xie, J. Zhang and D. J. Young, Water vapour effects on corrosion of Ni-Cr alloys in CO2 gas at 650°C, Corrosion Science136, 311–325 (2018). G. Bamba, Y. Wouters, A. Galerie, G. Borchardt, S. Shimada, O. Heintz and S. Chevalier, Inverse growth transport in thermal chromia scales on Fe-15Cr steels in oxygen and in water vapour and its effect on scale adhesion, Scripta Materialia57, 671–674 (2007). J. Pirón Abellán, T. Olszewski, H. J. Penkalla, G. H. Meier, L. Singheiser and W. J. Quadakkers, Scale formation mechanisms of martensitic steels in high CO2/H2O-containing gases simulating oxyfuel environments, Materials at High Temperatures26, 63–72 (2009). M. Michalik, M. Hänsel, J. Zurek, L. Singheiser and W. J. Quadakkers, Effect of water vapour on growth and adherence of chromia scales formed on Cr in high and low pO2-environments at 1000 and 1050°C, Materials at High Temperatures22, 213–221 (2005). Y.-X. Xu, J.-T. Lu, X.-W. Yang, J.-B. Yan and W.-Y. Li, Effect and role of alloyed Nb on the air oxidation behaviour of Ni-Cr-Fe alloys at 1000 °C, Corrosion Science127, 10–20 (2017). S. Henry, J. Mougin, Y. Wouters, J. P. Petit and A. Galerie, Characterization of chromia scales grown on pure chromium in different oxidizing atmospheres, Materials at High Temperatures17, 231–234 (2000). Y. Xie, J. Zhang, D. J. Young and W. Zheng, Effect of Fe on corrosion of Ni-20Cr and Ni-30Cr alloys in wet CO2 gas at 650 and 700 °C, Corrosion Science154, 129–143 (2019). D. Simon, B. Gorr, M. Hänsel, V. Shemet, H. J. Christ and W. J. Quadakkers, Effect of in situ gas changes on thermally grown chromia scales formed on Ni-25Cr alloy at 1000°C in atmospheres with and without water vapour, Materials at High Temperatures32, 238–247 (2015). D. J. Young, Effects of water vapour on the oxidation of chromia formers, Materials Science Forum595, 1189–1197 (2008). 9987_CR13 9987_CR12 9987_CR15 9987_CR14 9987_CR17 9987_CR16 9987_CR19 9987_CR18 9987_CR11 9987_CR10 9987_CR7 9987_CR24 9987_CR8 9987_CR23 9987_CR9 9987_CR26 9987_CR25 9987_CR28 9987_CR27 9987_CR1 9987_CR2 9987_CR3 9987_CR4 9987_CR5 9987_CR6 9987_CR20 9987_CR22 9987_CR21 |
| References_xml | – reference: C. Wagner, Theoretical analysis of the diffusion processes determining the oxidation rate of alloys, Journal of the Electrochemical Society99, 369–380 (1952). – reference: Y. Xie, T. Liang, J. Zhang and D. J. Young, Effects of Fe on oxidation of Ni-20Cr and Ni-30Cr alloys at 800°C in dry CO2 gas, Corrosion Science 173, 108777 (2020). – reference: J. Zurek, D. J. Young, E. Essuman, M. Hänsel, H. J. Penkalla, L. Niewolak and W. J. Quadakkers, Growth and adherence of chromia based surface scales on Ni-base alloys in high- and low-pO2 gases, Materials Science and Engineering, A477, 259–270 (2008). – reference: S. Henry, J. Mougin, Y. Wouters, J. P. Petit and A. Galerie, Characterization of chromia scales grown on pure chromium in different oxidizing atmospheres, Materials at High Temperatures17, 231–234 (2000). – reference: E. A. Polman, T. Fransen and P. J. Gellings, Oxidation kinetics of chromium and morphological phenomena, Oxidation of Metals32, 433–447 (1989). – reference: M.-C. Demizieux, C. Desgranges, L. Martinelli, J. Favergeon and K. Ginestar, Morphology and buckling of the oxide scale after Fe-9Cr steel oxidation in water vapor environment, Oxidation of Metals91, 191–212 (2019). – reference: A. Rahmel and J. Tobolski, Einfluss von wasserdampf und kohlendioxyd auf die oxydation von eisen in sauerstoff bei hohen temperaturen, Corrosion Science5, 333–346 (1965). – reference: Y.-X. Xu, J.-T. Lu, X.-W. Yang, J.-B. Yan and W.-Y. Li, Effect and role of alloyed Nb on the air oxidation behaviour of Ni-Cr-Fe alloys at 1000 °C, Corrosion Science127, 10–20 (2017). – reference: G. H. Meier, K. Jung, N. Mu, N. M. Yanar, F. S. Pettit, J. Pirón Abellán, T. Olszewski, L. Nieto Hierro, W. J. Quadakkers and G. R. Holcomb, Effect of alloy composition and exposure conditions on the selective oxidation behavior of ferritic Fe-Cr and Fe-Cr-X alloys, Oxidation of Metals74, 319–340 (2010). – reference: D. Simon, B. Gorr, M. Hänsel, V. Shemet, H. J. Christ and W. J. Quadakkers, Effect of in situ gas changes on thermally grown chromia scales formed on Ni-25Cr alloy at 1000°C in atmospheres with and without water vapour, Materials at High Temperatures32, 238–247 (2015). – reference: R. Viswanathan, J. F. Henry, J. Tanzosh, G. Stanko, J. Shingledecker, B. Vitalis and R. Purgert, U.S. program on materials technology for ultra-supercritical coal power plants, Journal of Materials Engineering and Performance14, 281–292 (2005). – reference: Y. Xie, T. D. Nguyen, J. Zhang and D. J. Young, Corrosion behaviour of Ni-Cr alloys in wet CO2 atmosphere at 700 and 800°C, Corrosion Science146, 28–43 (2019). – reference: A. Galerie, J. P. Petit, Y. Wouters, J. Mougin, A. Srisrual and P. Y. Hou, Water vapour effects on the oxidation of chromia-forming alloys, Materials Science Forum696, 200–205 (2011). – reference: J. Pirón Abellán, T. Olszewski, H. J. Penkalla, G. H. Meier, L. Singheiser and W. J. Quadakkers, Scale formation mechanisms of martensitic steels in high CO2/H2O-containing gases simulating oxyfuel environments, Materials at High Temperatures26, 63–72 (2009). – reference: J. Ehlers, D. J. Young, E. J. Smaardijk, A. K. Tyagi, H. J. Penkalla, L. Singheiser and W. J. Quadakkers, Enhanced oxidation of the 9%Cr steel P91 in water vapour containing environments, Corrosion Science48, 3428–3454 (2006). – reference: Y.-X. Xu, W.-Y. Li and X.-W. Yang, Influence of alloyed Fe on corrosion of Ni-Cr alloys in molten silicates and the effects of pre-oxidation treatment, Corrosion Science134, 179–188 (2018). – reference: Y. Xie, J. Zhang and D. J. Young, Water vapour effects on corrosion of Ni-Cr alloys in CO2 gas at 650°C, Corrosion Science136, 311–325 (2018). – reference: C. Wagner, Reaktionstypen bei der oxydation von legierungen, Zeitschrift für Elektrochemie63, 772–782 (1959). – reference: J. O. Andersson, T. Helander, L. Höglund, P. Shi and B. Sundman, Thermo-Calc & DICTRA, computational tools for materials science, CALPHAD26, 273–312 (2002). – reference: A. Galerie, Y. Wouters and M. Caillet, The kinetic behaviour of metals in water vapour at high temperatures: can general rules be proposed? Materials Science Forum369–372, 231–238 (2001). – reference: J. P. Abellán, T. Olszewski, G. H. Meier, L. Singheiser and W. J. Quadakkers, The oxidation behaviour of the 9%Cr steel P92 in CO2- and H2O-rich gases relevant to oxyfuel environments, International Journal of Materials Research101, 287–299 (2010). – reference: F. Abe, Research and development of heat-resistant materials for advanced USC power plants with steam temperatures of 700°C and above, Engineering1, 211–224 (2015). – reference: Y. Xie, J. Zhang, D. J. Young and W. Zheng, Effect of Fe on corrosion of Ni-20Cr and Ni-30Cr alloys in wet CO2 gas at 650 and 700 °C, Corrosion Science154, 129–143 (2019). – reference: D. J. Young, Effects of water vapour on the oxidation of chromia formers, Materials Science Forum595, 1189–1197 (2008). – reference: D. Huenert and A. Kranzmann, Impact of oxyfuel atmospheres H2O/CO2/O2 and H2O/CO2 on the oxidation of ferritic-martensitic and austenitic steels, Corrosion Science53, 2306–2317 (2011). – reference: C. T. Fujii and R. A. Meussner, Oxide structures produced on iron-chromium alloys by a dissociative mechanism, Journal of the Electrochemical Society110, 1195–1204 (1963). – reference: M. Michalik, M. Hänsel, J. Zurek, L. Singheiser and W. J. Quadakkers, Effect of water vapour on growth and adherence of chromia scales formed on Cr in high and low pO2-environments at 1000 and 1050°C, Materials at High Temperatures22, 213–221 (2005). – reference: G. Bamba, Y. Wouters, A. Galerie, G. Borchardt, S. Shimada, O. Heintz and S. Chevalier, Inverse growth transport in thermal chromia scales on Fe-15Cr steels in oxygen and in water vapour and its effect on scale adhesion, Scripta Materialia57, 671–674 (2007). – ident: 9987_CR3 doi: 10.15302/J-ENG-2015031 – ident: 9987_CR10 doi: 10.3184/096034009X438185 – ident: 9987_CR18 doi: 10.1002/bbpc.19590630713 – ident: 9987_CR12 doi: 10.3184/096034005782744443 – ident: 9987_CR5 doi: 10.1007/s11085-010-9215-5 – ident: 9987_CR13 doi: 10.1179/mht.2000.17.2.008 – ident: 9987_CR9 doi: 10.1016/j.corsci.2020.108777 – ident: 9987_CR20 doi: 10.1016/S0010-938X(65)90500-7 – ident: 9987_CR27 doi: 10.4028/www.scientific.net/MSF.696.200 – ident: 9987_CR22 doi: 10.1016/j.corsci.2006.02.002 – ident: 9987_CR8 doi: 10.1016/j.corsci.2019.04.007 – ident: 9987_CR7 doi: 10.3139/146.110271 – ident: 9987_CR17 doi: 10.1016/S0364-5916(02)00037-8 – ident: 9987_CR15 doi: 10.1179/0960340914Z.000000000108 – ident: 9987_CR19 doi: 10.1149/1.2779605 – ident: 9987_CR26 doi: 10.1016/j.scriptamat.2007.06.050 – ident: 9987_CR14 doi: 10.1016/j.msea.2007.05.035 – ident: 9987_CR16 doi: 10.4028/www.scientific.net/MSF.595-598.1189 – ident: 9987_CR21 doi: 10.1149/1.2425624 – ident: 9987_CR25 doi: 10.1007/s11085-018-9873-2 – ident: 9987_CR2 doi: 10.1016/j.corsci.2018.02.022 – ident: 9987_CR4 doi: 10.1016/j.corsci.2017.08.003 – ident: 9987_CR28 doi: 10.1007/BF00665448 – ident: 9987_CR23 doi: 10.4028/www.scientific.net/MSF.369-372.231 – ident: 9987_CR6 doi: 10.1016/j.corsci.2011.03.015 – ident: 9987_CR11 doi: 10.1016/j.corsci.2018.10.029 – ident: 9987_CR1 doi: 10.1361/10599490524039 – ident: 9987_CR24 doi: 10.1016/j.corsci.2018.03.023 |
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| Snippet | The oxidation behaviour of model alloys Ni-(20, 30)Cr (wt.%) with (0, 1, 5, 15%) Fe was investigated at 800 °C in Ar-20%CO
2
-20%H
2
O gas. All 20Cr alloys... The oxidation behaviour of model alloys Ni-(20, 30)Cr (wt.%) with (0, 1, 5, 15%) Fe was investigated at 800 °C in Ar-20%CO2-20%H2O gas. All 20Cr alloys... |
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| SubjectTerms | Alloy development Alloying effects Carbon dioxide Chemistry and Materials Science Chromium oxides Corrosion and Coatings Inorganic Chemistry Iron Materials Science Metallic Materials Nickel chromium alloys Original Paper Oxidation Scale (corrosion) Spallation Transport properties Tribology Water vapor |
| Title | Effects of Fe on Oxidation of Ni-20Cr and Ni-30Cr Alloys at 800 °C in Wet CO2 Gas |
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