Catalytic activity of cerium-doped Ru/Al2O3 during ozonation of dimethyl phthalate
In this paper, factors influencing the mineralization of dimethyl phthalate (DMP) during catalytic ozonation with a cerium-doped Ru/Al 2 O 3 catalyst were studied. The catalytic contribution was calculated through the results of a comparison experiment. It showed that doping cerium significantly enh...
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Published in | Frontiers of environmental science & engineering Vol. 2; no. 3; pp. 354 - 357 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
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SP Higher Education Press
01.09.2008
Springer Nature B.V |
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Abstract | In this paper, factors influencing the mineralization of dimethyl phthalate (DMP) during catalytic ozonation with a cerium-doped Ru/Al
2
O
3
catalyst were studied. The catalytic contribution was calculated through the results of a comparison experiment. It showed that doping cerium significantly enhanced catalytic activity. The total organic carbon (TOC) removal over the doped catalyst at 100 min reached 75.1%, 61.3% using Ru/Al
2
O
3
catalyst and only 14.0% using ozone alone. Catalytic activity reached the maximum when 0.2% of ruthenium and 1.0% of cerium were simultaneously loaded onto Al
2
O
3
support. Results of experiments on oxidation by ozone alone, adsorption of the catalyst, Ce ion’s and heterogeneous catalytic ozonation confirmed that the contribution of heterogeneous catalytic ozonation was about 50%, which showed the obvious effect of Ru-Ce/Al
2
O
3
on catalytic activity. |
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AbstractList | In this paper, factors influencing the mineralization of dimethyl phthalate (DMP) during catalytic ozonation with a cerium-doped Ru/Al
2
O
3
catalyst were studied. The catalytic contribution was calculated through the results of a comparison experiment. It showed that doping cerium significantly enhanced catalytic activity. The total organic carbon (TOC) removal over the doped catalyst at 100 min reached 75.1%, 61.3% using Ru/Al
2
O
3
catalyst and only 14.0% using ozone alone. Catalytic activity reached the maximum when 0.2% of ruthenium and 1.0% of cerium were simultaneously loaded onto Al
2
O
3
support. Results of experiments on oxidation by ozone alone, adsorption of the catalyst, Ce ion’s and heterogeneous catalytic ozonation confirmed that the contribution of heterogeneous catalytic ozonation was about 50%, which showed the obvious effect of Ru-Ce/Al
2
O
3
on catalytic activity. In this paper, factors influencing the mineralization of dimethyl phthalate (DMP) during catalytic ozonation with a cerium-doped Ru/Al2O3 catalyst were studied. The catalytic contribution was calculated through the results of a comparison experiment. It showed that doping cerium significantly enhanced catalytic activity. The total organic carbon (TOC) removal over the doped catalyst at 100 min reached 75.1%, 61.3% using Ru/Al2O3 catalyst and only 14.0% using ozone alone. Catalytic activity reached the maximum when 0.2% of ruthenium and 1.0% of cerium were simultaneously loaded onto Al2O3 support. Results of experiments on oxidation by ozone alone, adsorption of the catalyst, Ce ion’s and heterogeneous catalytic ozonation confirmed that the contribution of heterogeneous catalytic ozonation was about 50%, which showed the obvious effect of Ru-Ce/Al2O3 on catalytic activity. |
Author | Zhou, Yunrui Chen, Xun Zhu, Wanpeng |
Author_xml | – sequence: 1 givenname: Yunrui surname: Zhou fullname: Zhou, Yunrui email: zhou.yunrui@mepfeco.org.cn organization: Department of Environmental Science and Engineering, Tsinghua University – sequence: 2 givenname: Wanpeng surname: Zhu fullname: Zhu, Wanpeng organization: Department of Environmental Science and Engineering, Tsinghua University – sequence: 3 givenname: Xun surname: Chen fullname: Chen, Xun organization: Department of Chemical and Environmental Engineering, China University of Mining and Technology (Beijing) |
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Keywords | ozonation Ru-Ce/Al doped cerium catalytic oxidation ozone O |
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Snippet | In this paper, factors influencing the mineralization of dimethyl phthalate (DMP) during catalytic ozonation with a cerium-doped Ru/Al
2
O
3
catalyst were... In this paper, factors influencing the mineralization of dimethyl phthalate (DMP) during catalytic ozonation with a cerium-doped Ru/Al2O3 catalyst were... |
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StartPage | 354 |
SubjectTerms | Aluminum oxide Catalysts Catalytic activity Cerium Earth and Environmental Science Environment Mineralization Organic carbon Oxidation Ozonation Ozone Phthalates Research Article Ruthenium Total organic carbon |
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Title | Catalytic activity of cerium-doped Ru/Al2O3 during ozonation of dimethyl phthalate |
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