Anion receptors based on ureidocalix[4]arenes immobilised in the partial cone conformation
A novel method enabling the synthesis of receptors based on the calix[4]arenes immobilized in the partial cone conformation is reported. The application of a protection/deprotection strategy using nosyl groups enables the regioselective introduction of functional groups (NO2 and NH2) into the upper...
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| Published in | New journal of chemistry Vol. 37; no. 1; pp. 220 - 227 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Royal Soc Chemistry
01.01.2013
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| Abstract | A novel method enabling the synthesis of receptors based on the calix[4]arenes immobilized in the partial cone conformation is reported. The application of a protection/deprotection strategy using nosyl groups enables the regioselective introduction of functional groups (NO2 and NH2) into the upper rim of calix[4] arenes, leading finally to the substitution pattern so far inaccessible to calixarene chemistry. The introduction of two ureido functions at the para positions of the partial cone conformer yields a novel type of receptor which can bind anions even in a highly competitive solvent (DMSO). This revealed that the partial cone conformation, so far rather ignored in supramolecular chemistry, can be also very useful in design of novel anion receptors. |
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| AbstractList | A novel method enabling the synthesis of receptors based on the calix[4]arenes immobilized in the partial cone conformation is reported. The application of a protection/deprotection strategy using nosyl groups enables the regioselective introduction of functional groups (NO2 and NH2) into the upper rim of calix[4] arenes, leading finally to the substitution pattern so far inaccessible to calixarene chemistry. The introduction of two ureido functions at the para positions of the partial cone conformer yields a novel type of receptor which can bind anions even in a highly competitive solvent (DMSO). This revealed that the partial cone conformation, so far rather ignored in supramolecular chemistry, can be also very useful in design of novel anion receptors. |
| Author | Curinova, Petra Cisarova, Ivana Budka, Jan Hudecek, Oldrich Dvorakova, Hana Lhotak, Pavel |
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| CitedBy_id | crossref_primary_10_1002_elsa_202100221 crossref_primary_10_3390_ma15020692 crossref_primary_10_1039_C4CE01240B crossref_primary_10_1016_j_snb_2020_129151 crossref_primary_10_1039_C6NJ01271J |
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| Keywords | RECOGNITION 1,3-ALTERNATE COMPLEXATION BINDING |
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| Title | Anion receptors based on ureidocalix[4]arenes immobilised in the partial cone conformation |
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