Remediation of antimony-contaminated soil with composite materials of Fe/Fe2+-fly ash-concrete additive in seasonal freezing regions
Antimony (Sb) finds its wide application in industries, however, the research on Sb solidification/stabilization (S/S) in the Sb-contaminated soil is currently insufficient, particularly in seasonal freezing regions. Here six composite materials of Fe/Fe2+-fly ash-concrete additive (Fe-FA-CA) were e...
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| Published in | Process safety and environmental protection Vol. 167; pp. 247 - 256 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.11.2022
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| Subjects | |
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| Abstract | Antimony (Sb) finds its wide application in industries, however, the research on Sb solidification/stabilization (S/S) in the Sb-contaminated soil is currently insufficient, particularly in seasonal freezing regions. Here six composite materials of Fe/Fe2+-fly ash-concrete additive (Fe-FA-CA) were employed and optimized to remediate the Sb-contaminated soil subject to 40 freezing-thawing (F-T) cycles. After remediation, FeSO4-fly ash-calcium lignosulfonate (FFC) exhibited the best resistance performance to F-T. The stabilization efficiency was evaluated with TCLP at 92.92%. Meanwhile, Sb concentration met the criteria of landfill for inert waste assessed with the compliance test for leaching (CT) of European Standard. The S/S efficiency of Sb dropped slightly from 92.68% to 88.22% (TCLP) and from 97.18% to 93.37% (CT), respectively, after aging 40 F-T cycles. The fraction of residual Sb in the soil treated by FFC was increased by 10.41%, and the strength of the S/S soil was much higher than 350 kPa, the requirement of landfills in the U.S. during F-T cycles. Additionally, the poorly crystalline Fe in the soil remediated by FFC was increased by 4.54 g/kg, suppressing Sb migration. The feasibility and effectiveness of FFC in S/S of Sb demonstrated its potential to remediate Sb-contaminated soil in seasonal freezing regions.
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| AbstractList | Antimony (Sb) finds its wide application in industries, however, the research on Sb solidification/stabilization (S/S) in the Sb-contaminated soil is currently insufficient, particularly in seasonal freezing regions. Here six composite materials of Fe/Fe2+-fly ash-concrete additive (Fe-FA-CA) were employed and optimized to remediate the Sb-contaminated soil subject to 40 freezing-thawing (F-T) cycles. After remediation, FeSO4-fly ash-calcium lignosulfonate (FFC) exhibited the best resistance performance to F-T. The stabilization efficiency was evaluated with TCLP at 92.92%. Meanwhile, Sb concentration met the criteria of landfill for inert waste assessed with the compliance test for leaching (CT) of European Standard. The S/S efficiency of Sb dropped slightly from 92.68% to 88.22% (TCLP) and from 97.18% to 93.37% (CT), respectively, after aging 40 F-T cycles. The fraction of residual Sb in the soil treated by FFC was increased by 10.41%, and the strength of the S/S soil was much higher than 350 kPa, the requirement of landfills in the U.S. during F-T cycles. Additionally, the poorly crystalline Fe in the soil remediated by FFC was increased by 4.54 g/kg, suppressing Sb migration. The feasibility and effectiveness of FFC in S/S of Sb demonstrated its potential to remediate Sb-contaminated soil in seasonal freezing regions.
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| Author | Jiang, Miao Zhao, Qingliang Wang, Long Wang, Weiye Ding, Jing Xue, Ruiyuan Wang, Kun |
| Author_xml | – sequence: 1 givenname: Miao surname: Jiang fullname: Jiang, Miao organization: State Key Laboratory of Urban Water Resources and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China – sequence: 2 givenname: Kun surname: Wang fullname: Wang, Kun organization: State Key Laboratory of Urban Water Resources and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China – sequence: 3 givenname: Ruiyuan surname: Xue fullname: Xue, Ruiyuan organization: State Key Laboratory of Urban Water Resources and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China – sequence: 4 givenname: Qingliang surname: Zhao fullname: Zhao, Qingliang email: zhql1962@163.com organization: State Key Laboratory of Urban Water Resources and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China – sequence: 5 givenname: Long surname: Wang fullname: Wang, Long organization: Beijing General Municipal Engineering Design & Research Institute Co., Ltd., Beijing 100082, China – sequence: 6 givenname: Weiye surname: Wang fullname: Wang, Weiye organization: State Key Laboratory of Urban Water Resources and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China – sequence: 7 givenname: Jing surname: Ding fullname: Ding, Jing organization: State Key Laboratory of Urban Water Resources and Environment, School of Environment, Harbin Institute of Technology, Harbin 150090, China |
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| Keywords | C-S-H RES UCS XANES S-A XRD F-T EXAFS Fe/Fe2+-fly ash-concrete additive AFT W-D SE TCLP ANOVA S/S CA OM Unconfined compressive strength Ca-L SDS Leaching concentration Fe-FA-CA BDAT Solidification/stabilization Mont USGS Freezing-thawing cycles CT EXC CAR Antimony-contaminated soil Fe/Mn SEM FA |
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| Snippet | Antimony (Sb) finds its wide application in industries, however, the research on Sb solidification/stabilization (S/S) in the Sb-contaminated soil is currently... |
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| SourceType | Enrichment Source Index Database Publisher |
| StartPage | 247 |
| SubjectTerms | Antimony-contaminated soil Fe/Fe2+-fly ash-concrete additive Freezing-thawing cycles Leaching concentration Solidification/stabilization Unconfined compressive strength |
| Title | Remediation of antimony-contaminated soil with composite materials of Fe/Fe2+-fly ash-concrete additive in seasonal freezing regions |
| URI | https://dx.doi.org/10.1016/j.psep.2022.09.018 |
| Volume | 167 |
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