Advanced photocatalysts for uranium extraction: Elaborate design and future perspectives

[Display omitted] •The influencing factors on photocatalytic uranium extraction was evaluated.•The design strategy of photocatalysts for uranium extraction was summarized.•The rational design was provided from band structure and surface coordination.•The technical methods for identificating uranium...

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Published in	Coordination chemistry reviews Vol. 467; p. 214615
Main Authors	Chen, Tao, Yu, Kaifu, Dong, Changxue, Yuan, Xin, Gong, Xiang, Lian, Jie, Cao, Xin, Li, Mingzhe, Zhou, Li, Hu, Baowei, He, Rong, Zhu, Wenkun, Wang, Xiangke
Format	Journal Article
Language	English
Published	Elsevier B.V 15.09.2022
Subjects	Heterogeneous catalysis Photocatalysts Photoreduction Uranium extraction Uranium extraction Photoreduction Heterogeneous catalysis Photocatalysts
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Abstract	[Display omitted] •The influencing factors on photocatalytic uranium extraction was evaluated.•The design strategy of photocatalysts for uranium extraction was summarized.•The rational design was provided from band structure and surface coordination.•The technical methods for identificating uranium reduction species were summarized.•The challenges and prospects of photocatalytic uranium reduction were pointed out. Nuclear energy has been regarded as one of the promising energy sources to replace traditional fossil fuels due to its advantages of high energy density and carbon-free emission. Unfortunately, the limited storage of uranium ore restricted the sustainable development of nuclear energy, together with the generation of uranium-containing wastewater resulting in the problems of environmental pollution. Therefore, extracting and recycling uranium from seawater and radioactive uranium-containing wastewater is necessary for the sustainable development of nuclear energy and environmental protection. The light-driven heterogeneous photocatalytic technology is an appealing strategy to significantly promote the kinetics, capacity, and selectivity during uranium extraction. However, the recovery of uranium from radioactive wastewater/seawater is restricted by various factors, such as abundant competing ions, low uranium concentration, coexisting organic matter, and strong acidity or alkalinity in special environmental in the process of practical application. In this review, we described the general background of uranium extraction, followed by a brief discussion of the several possible reduction paths for photocatalytic reduction of uranium. Then, the effects of experimental conditions, photocatalyst stability and environmental adaptability on the performance of photocatalytic uranium reduction were systematically discussed. After having some fundamental understanding on photocatalytic uranium reduction, we summarized the design guidelines of photocatalysts for uranium reduction, and further discussed the corresponding advantages and disadvantages in photocatalytic uranium reduction. In addition, we concluded the current available characterization techniques for identifying uranium species after reduction, which is critical to the mechanistic study. Finally, we end this review with an outlook into the remaining challenges and future perspectives of photocatalytic uranium reduction.
AbstractList	[Display omitted] •The influencing factors on photocatalytic uranium extraction was evaluated.•The design strategy of photocatalysts for uranium extraction was summarized.•The rational design was provided from band structure and surface coordination.•The technical methods for identificating uranium reduction species were summarized.•The challenges and prospects of photocatalytic uranium reduction were pointed out. Nuclear energy has been regarded as one of the promising energy sources to replace traditional fossil fuels due to its advantages of high energy density and carbon-free emission. Unfortunately, the limited storage of uranium ore restricted the sustainable development of nuclear energy, together with the generation of uranium-containing wastewater resulting in the problems of environmental pollution. Therefore, extracting and recycling uranium from seawater and radioactive uranium-containing wastewater is necessary for the sustainable development of nuclear energy and environmental protection. The light-driven heterogeneous photocatalytic technology is an appealing strategy to significantly promote the kinetics, capacity, and selectivity during uranium extraction. However, the recovery of uranium from radioactive wastewater/seawater is restricted by various factors, such as abundant competing ions, low uranium concentration, coexisting organic matter, and strong acidity or alkalinity in special environmental in the process of practical application. In this review, we described the general background of uranium extraction, followed by a brief discussion of the several possible reduction paths for photocatalytic reduction of uranium. Then, the effects of experimental conditions, photocatalyst stability and environmental adaptability on the performance of photocatalytic uranium reduction were systematically discussed. After having some fundamental understanding on photocatalytic uranium reduction, we summarized the design guidelines of photocatalysts for uranium reduction, and further discussed the corresponding advantages and disadvantages in photocatalytic uranium reduction. In addition, we concluded the current available characterization techniques for identifying uranium species after reduction, which is critical to the mechanistic study. Finally, we end this review with an outlook into the remaining challenges and future perspectives of photocatalytic uranium reduction.
ArticleNumber	214615
Author	Wang, Xiangke Yuan, Xin Zhou, Li Gong, Xiang Zhu, Wenkun Chen, Tao Cao, Xin Li, Mingzhe He, Rong Dong, Changxue Lian, Jie Hu, Baowei Yu, Kaifu
Author_xml	– sequence: 1 givenname: Tao surname: Chen fullname: Chen, Tao organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 2 givenname: Kaifu surname: Yu fullname: Yu, Kaifu organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 3 givenname: Changxue surname: Dong fullname: Dong, Changxue organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 4 givenname: Xin surname: Yuan fullname: Yuan, Xin organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 5 givenname: Xiang surname: Gong fullname: Gong, Xiang organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 6 givenname: Jie surname: Lian fullname: Lian, Jie organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 7 givenname: Xin surname: Cao fullname: Cao, Xin organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 8 givenname: Mingzhe surname: Li fullname: Li, Mingzhe organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 9 givenname: Li surname: Zhou fullname: Zhou, Li organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 10 givenname: Baowei surname: Hu fullname: Hu, Baowei organization: School of Life Science, Shaoxing University, Shaoxing 312000, PR China – sequence: 11 givenname: Rong surname: He fullname: He, Rong email: her@swust.edu.cn organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 12 givenname: Wenkun surname: Zhu fullname: Zhu, Wenkun email: zhuwenkun@swust.edu.cn organization: State Key Laboratory of Environmentally Friendly Energy Materials, Sichuan Civil-military Integration Institute, National Collaborative Innovation Center for Nuclear Waste and Environmental Safety, School of National Defence Science & Technology, Southwest University of Science and Technology, Mianyang 621010, PR China – sequence: 13 givenname: Xiangke surname: Wang fullname: Wang, Xiangke email: xkwang@ncepu.edu.cn organization: School of Life Science, Shaoxing University, Shaoxing 312000, PR China
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Snippet	[Display omitted] •The influencing factors on photocatalytic uranium extraction was evaluated.•The design strategy of photocatalysts for uranium extraction was...
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SubjectTerms	Heterogeneous catalysis Photocatalysts Photoreduction Uranium extraction
Title	Advanced photocatalysts for uranium extraction: Elaborate design and future perspectives
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