Heterogeneous junctions of magnetic Ni core@binary dielectric shells toward high-efficiency microwave attenuation
•Ni@C@PEDOT spheres with multilayer heterogeneous interfaces are synthesized.•The spheres are constructed by magnetic Ni core and binary dielectric shells.•The multilayer heterogeneous interfaces trigger strong interfacial polarization.•The final absorption performance is sensitive to the dielectric...
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| Published in | Journal of materials science & technology Vol. 115; pp. 71 - 80 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
10.07.2022
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1005-0302 |
| DOI | 10.1016/j.jmst.2021.10.035 |
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| Abstract | •Ni@C@PEDOT spheres with multilayer heterogeneous interfaces are synthesized.•The spheres are constructed by magnetic Ni core and binary dielectric shells.•The multilayer heterogeneous interfaces trigger strong interfacial polarization.•The final absorption performance is sensitive to the dielectric PEDOT layer.•A strong RL value of −72.4 dB and wide bandwidth of 6.4 GHz are achieved.
Metal-organic-frameworks (MOFs) derived carbon-based composites with balanced impedance matching and synergistic dielectric/magnetic loss are considered as promising microwave absorbers. With the aim to promote interfacial polarization, herein, heterogeneous junctions composed of magnetic Ni core and binary dielectric shells (C and PEDOT) are synthesized by annealing Ni-MOFs precursors and an in-situ polymerization strategy, forming Ni@C@PEDOT spheres with multilayer heterogeneous interfaces. The results indicate that the final absorption attenuation is sensitive to the thickness of the dielectric PEDOT layer, when the thickness of the PEDOT layer is 224 nm, an optimal reflection loss of -72.4 dB is achieved at 2 mm and the effective absorption bandwidth reaches 6.4 GHz with a thickness of only 1.85 mm, the excellent absorption attenuation is accredited to the promoted impedance matching, enhanced conduction loss as well as the synergistic interfacial polarization induced by magnetic core and binary dielectric shells. Meanwhile, this work offers a simple and significant strategy in preparation for ideal microwave absorbers by rational design of multilayer heterogeneous interfaces. |
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| AbstractList | •Ni@C@PEDOT spheres with multilayer heterogeneous interfaces are synthesized.•The spheres are constructed by magnetic Ni core and binary dielectric shells.•The multilayer heterogeneous interfaces trigger strong interfacial polarization.•The final absorption performance is sensitive to the dielectric PEDOT layer.•A strong RL value of −72.4 dB and wide bandwidth of 6.4 GHz are achieved.
Metal-organic-frameworks (MOFs) derived carbon-based composites with balanced impedance matching and synergistic dielectric/magnetic loss are considered as promising microwave absorbers. With the aim to promote interfacial polarization, herein, heterogeneous junctions composed of magnetic Ni core and binary dielectric shells (C and PEDOT) are synthesized by annealing Ni-MOFs precursors and an in-situ polymerization strategy, forming Ni@C@PEDOT spheres with multilayer heterogeneous interfaces. The results indicate that the final absorption attenuation is sensitive to the thickness of the dielectric PEDOT layer, when the thickness of the PEDOT layer is 224 nm, an optimal reflection loss of -72.4 dB is achieved at 2 mm and the effective absorption bandwidth reaches 6.4 GHz with a thickness of only 1.85 mm, the excellent absorption attenuation is accredited to the promoted impedance matching, enhanced conduction loss as well as the synergistic interfacial polarization induced by magnetic core and binary dielectric shells. Meanwhile, this work offers a simple and significant strategy in preparation for ideal microwave absorbers by rational design of multilayer heterogeneous interfaces. |
| Author | Wu, Qingqing Li, Fangyuan Wang, Jijun Liu, Panbo Yu, Songlin Li, Bingzhen Li, Yan Chen, Yuhua Zhou, Xiao |
| Author_xml | – sequence: 1 givenname: Jijun surname: Wang fullname: Wang, Jijun organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 2 givenname: Songlin surname: Yu fullname: Yu, Songlin organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 3 givenname: Qingqing surname: Wu fullname: Wu, Qingqing organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 4 givenname: Yan surname: Li fullname: Li, Yan organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 5 givenname: Fangyuan surname: Li fullname: Li, Fangyuan organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 6 givenname: Xiao surname: Zhou fullname: Zhou, Xiao organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 7 givenname: Yuhua surname: Chen fullname: Chen, Yuhua email: cyhcst@sina.com organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 8 givenname: Bingzhen surname: Li fullname: Li, Bingzhen email: tylerlibz@hotmail.com organization: Institute of Defense Engineering, Academy of Military Sciences, Beijing 100036, China – sequence: 9 givenname: Panbo surname: Liu fullname: Liu, Panbo email: liupanbo@nwpu.edu.cn organization: School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710129, China |
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| Snippet | •Ni@C@PEDOT spheres with multilayer heterogeneous interfaces are synthesized.•The spheres are constructed by magnetic Ni core and binary dielectric shells.•The... |
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| SubjectTerms | Conductive polymer Core-shell structure Metal-organic-frameworks Microwave absorption |
| Title | Heterogeneous junctions of magnetic Ni core@binary dielectric shells toward high-efficiency microwave attenuation |
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