Quantum Electric Dipole Lattice Water Molecules Confined to Nanocavities in Beryl
Water is subject to intense investigations due to its importance in biological matter but keeps many of its secrets. Here, we unveil an even other aspect by confining H 2 O molecules to nanosize cages. Our THz and infrared spectra of water in the gemstone beryl evidence quantum tunneling of H 2 O mo...
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| Published in | Journal of infrared, millimeter and terahertz waves Vol. 39; no. 9; pp. 799 - 815 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Springer US
01.09.2018
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| Abstract | Water is subject to intense investigations due to its importance in biological matter but keeps many of its secrets. Here, we unveil an even other aspect by confining H
2
O molecules to nanosize cages. Our THz and infrared spectra of water in the gemstone beryl evidence quantum tunneling of H
2
O molecules in the crystal lattice. The water molecules are spread out when confined in a nanocage. In combination with low-frequency dielectric measurements, we were also able to show that dipolar coupling among the H
2
O molecules leads towards a ferroelectric state at low temperatures. Upon cooling, a ferroelectric soft mode shifts through the THz range. Only quantum fluctuations prevent perfect macroscopic order to be fully achieved. Beside the significance to life science and possible application, nanoconfined water may become the prime example of a quantum electric dipolar lattice. |
|---|---|
| AbstractList | Water is subject to intense investigations due to its importance in biological matter but keeps many of its secrets. Here, we unveil an even other aspect by confining H
2
O molecules to nanosize cages. Our THz and infrared spectra of water in the gemstone beryl evidence quantum tunneling of H
2
O molecules in the crystal lattice. The water molecules are spread out when confined in a nanocage. In combination with low-frequency dielectric measurements, we were also able to show that dipolar coupling among the H
2
O molecules leads towards a ferroelectric state at low temperatures. Upon cooling, a ferroelectric soft mode shifts through the THz range. Only quantum fluctuations prevent perfect macroscopic order to be fully achieved. Beside the significance to life science and possible application, nanoconfined water may become the prime example of a quantum electric dipolar lattice. |
| Author | Dressel, Martin Thomas, Victor G. Gorshunov, Boris P. Zhukova, Elena S. |
| Author_xml | – sequence: 1 givenname: Martin orcidid: 0000-0003-1907-052X surname: Dressel fullname: Dressel, Martin email: dressel@pi1.physik.uni-stuttgart.de organization: 1. Physikalisches Institut, Universität Stuttgart – sequence: 2 givenname: Elena S. surname: Zhukova fullname: Zhukova, Elena S. organization: Moscow Institute of Physics and Technology (State University) – sequence: 3 givenname: Victor G. surname: Thomas fullname: Thomas, Victor G. organization: Sobolev Institute of Geology and Mineralogy, SB RAS, Novosibirsk State University – sequence: 4 givenname: Boris P. surname: Gorshunov fullname: Gorshunov, Boris P. organization: Moscow Institute of Physics and Technology (State University) |
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| CitedBy_id | crossref_primary_10_1038_s41467_020_17832_y crossref_primary_10_1103_PhysRevB_108_064101 crossref_primary_10_3367_UFNe_2020_01_038721 crossref_primary_10_1063_5_0131510 crossref_primary_10_2139_ssrn_4196997 crossref_primary_10_3367_UFNr_2020_01_038721 crossref_primary_10_1039_D1CP05338H |
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| Keywords | Water Dipolar interaction THz spectroscopy Quantum tunneling Dielectric spectroscopy Ferroelectricity Fourier transform infrared spectroscopy |
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| Subtitle | Water Molecules Confined to Nanocavities in Beryl |
| Title | Quantum Electric Dipole Lattice |
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