Efficient electron transfer in CdSe quantum dots-decorated reduced graphene oxide for electromagnetic interference shielding application
Effective charge separation and use of hot charge carriers are considered to be the most essential factors affecting the activity of an excellent energy harvester. Herein, we have successfully decorated 3 nm of CdSe quantum dots (QDs) on the surface of reduced graphene oxide (rGO) using solvothermal...
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| Published in | Bulletin of materials science Vol. 47; no. 2; p. 119 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Bangalore
Indian Academy of Sciences
04.06.2024
Springer Nature B.V |
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| Abstract | Effective charge separation and use of hot charge carriers are considered to be the most essential factors affecting the activity of an excellent energy harvester. Herein, we have successfully decorated 3 nm of CdSe quantum dots (QDs) on the surface of reduced graphene oxide (rGO) using solvothermal method. Formation of CdSe–rGO nanocomposite (NC) has been confirmed by X-ray diffraction pattern, transmission electron microscopy and Raman analysis. Further, the emission spectrum of CdSe–rGO NC shows quenching of emission of CdSe QDs on the surface of rGO nanosheet. To elucidate this phenomenon, we have carried out time-correlated single-photon counting (TCSPC) measurements, which reveal efficient electron transfer, as the exciton lifetime of CdSe QDs in the NC is significantly reduced compared to bare CdSe QDs. Owing to the efficient electron transfer, this NC showed big boost in total shielding effectiveness (
SE
T
= 29 dB) when compared to graphene (
SE
T
= 23 dB) in electromagnetic interference shielding application.
Graphical abstract |
|---|---|
| AbstractList | Effective charge separation and use of hot charge carriers are considered to be the most essential factors affecting the activity of an excellent energy harvester. Herein, we have successfully decorated 3 nm of CdSe quantum dots (QDs) on the surface of reduced graphene oxide (rGO) using solvothermal method. Formation of CdSe–rGO nanocomposite (NC) has been confirmed by X-ray diffraction pattern, transmission electron microscopy and Raman analysis. Further, the emission spectrum of CdSe–rGO NC shows quenching of emission of CdSe QDs on the surface of rGO nanosheet. To elucidate this phenomenon, we have carried out time-correlated single-photon counting (TCSPC) measurements, which reveal efficient electron transfer, as the exciton lifetime of CdSe QDs in the NC is significantly reduced compared to bare CdSe QDs. Owing to the efficient electron transfer, this NC showed big boost in total shielding effectiveness (SET = 29 dB) when compared to graphene (SET = 23 dB) in electromagnetic interference shielding application. Effective charge separation and use of hot charge carriers are considered to be the most essential factors affecting the activity of an excellent energy harvester. Herein, we have successfully decorated 3 nm of CdSe quantum dots (QDs) on the surface of reduced graphene oxide (rGO) using solvothermal method. Formation of CdSe–rGO nanocomposite (NC) has been confirmed by X-ray diffraction pattern, transmission electron microscopy and Raman analysis. Further, the emission spectrum of CdSe–rGO NC shows quenching of emission of CdSe QDs on the surface of rGO nanosheet. To elucidate this phenomenon, we have carried out time-correlated single-photon counting (TCSPC) measurements, which reveal efficient electron transfer, as the exciton lifetime of CdSe QDs in the NC is significantly reduced compared to bare CdSe QDs. Owing to the efficient electron transfer, this NC showed big boost in total shielding effectiveness ( SE T = 29 dB) when compared to graphene ( SE T = 23 dB) in electromagnetic interference shielding application. Graphical abstract |
| ArticleNumber | 119 |
| Author | Singh, Ashwani Kumar Yadav, Amar Nath Upadhyay, Shiva Singh, Kedar |
| Author_xml | – sequence: 1 givenname: Amar Nath orcidid: 0000-0003-4500-3304 surname: Yadav fullname: Yadav, Amar Nath email: amar22892@gmail.com organization: School of Physical Sciences, Jawaharlal Nehru University, Division of Materials Science and Engineering, Hanyang University – sequence: 2 givenname: Shiva surname: Upadhyay fullname: Upadhyay, Shiva organization: Department of Physics, Swami Shraddhanand College, University of Delhi – sequence: 3 givenname: Ashwani Kumar surname: Singh fullname: Singh, Ashwani Kumar organization: Department of Physics, Deshbandhu College, University of Delhi – sequence: 4 givenname: Kedar surname: Singh fullname: Singh, Kedar organization: School of Physical Sciences, Jawaharlal Nehru University |
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| ContentType | Journal Article |
| Copyright | Indian Academy of Sciences 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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| SubjectTerms | Cadmium selenides Chemistry and Materials Science Composite materials Current carriers Diffraction patterns Electromagnetic interference Electromagnetic shielding Electron transfer Electrons Emission Energy harvesting Engineering Excitons Graphene Graphite Materials Science Nanocomposites Photovoltaic cells Potassium Quantum dots Raman spectroscopy Sulfuric acid This article is part of the Special issue on “Materials for Energy and Sustainable Development” Time correlation functions |
| Title | Efficient electron transfer in CdSe quantum dots-decorated reduced graphene oxide for electromagnetic interference shielding application |
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