Water Effect on Amine-Modification of Adsorbents for Separation of CO2/N2
The adsorption of CO2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO2 from other gases is promoted. Water plays an important role in this process. Water increases both the adsorption amount of CO2 and the separation coefficient with N2 for all amines loaded. Ho...
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| Published in | Transactions of Tianjin University Vol. 19; no. 5; pp. 313 - 318 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.10.2013
School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China%School of Sciences, Tianjin University, Tianjin 300072, China |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1006-4982 1995-8196 |
| DOI | 10.1007/s12209-013-2002-z |
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| Abstract | The adsorption of CO2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO2 from other gases is promoted. Water plays an important role in this process. Water increases both the adsorption amount of CO2 and the separation coefficient with N2 for all amines loaded. However, the effect of loading trialkylamines is not remarkable in the absence of water. The effect of loading dialkylamine does not depend on water, but the adsorbent cannot be regenerated at ambient temperature. In comparison, an adsorbent loading trialkylamine can be regenerated at ambient temperature even in the presence of water with fairly good stability. |
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| AbstractList | The adsorption of CO2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO2 from other gases is promoted. Water plays an important role in this process. Water increases both the adsorption amount of CO2 and the separation coefficient with N2 for all amines loaded. However, the effect of loading trialkylamines is not remarkable in the absence of water. The effect of loading dialkylamine does not depend on water, but the adsorbent cannot be regenerated at ambient temperature. In comparison, an adsorbent loading trialkylamine can be regenerated at ambient temperature even in the presence of water with fairly good stability. The adsorption of CO 2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO 2 from other gases is promoted. Water plays an important role in this process. Water increases both the adsorption amount of CO 2 and the separation coefficient with N 2 for all amines loaded. However, the effect of loading trialkylamines is not remarkable in the absence of water. The effect of loading dialkylamine does not depend on water, but the adsorbent cannot be regenerated at ambient temperature. In comparison, an adsorbent loading trialkylamine can be regenerated at ambient temperature even in the presence of water with fairly good stability. |
| Author | 张中正 汤娇娣 孙艳 苏伟 |
| AuthorAffiliation | School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China School of Sciences, Tianjin University, Tianjin 300072, China |
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| CitedBy_id | crossref_primary_10_1021_acs_jced_8b00798 crossref_primary_10_1007_s12209_020_00245_9 crossref_primary_10_1007_s10450_015_9651_2 |
| Cites_doi | 10.1016/j.enconman.2007.06.007 10.1021/ie070685c 10.1016/S1004-9541(11)60050-5 10.1021/ie060774+ 10.1021/ef000241s 10.1021/ja01269a023 10.1021/je0201267 10.1016/S1001-0742(08)60002-9 10.1016/j.fuel.2005.04.003 10.1021/es072085a 10.1627/jpi.48.29 10.1016/j.apsusc.2011.12.046 10.1016/j.ces.2004.11.058 10.1016/j.fuel.2007.06.001 10.1016/j.fuel.2009.02.025 10.1016/0020-1693(95)04534-1 10.1002/chem.200701467 10.1016/j.fuproc.2005.01.014 10.1021/la702466d 10.1016/j.fuel.2006.07.003 10.1002/cssc.200900036 10.1021/ja01145a126 10.1021/ie051286p 10.1016/S1003-9953(06)60030-3 10.1246/cl.2004.510 10.1016/j.ces.2006.11.005 |
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| Keywords | adsorption separation of CO water effect amine-modification separation of CO2 |
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| Notes | 12-1248/T separation of CO2; adsorption; amine-modification; water effect The adsorption of CO2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO2 from other gases is promoted. Water plays an important role in this process. Water increases both the adsorption amount of CO2 and the separation coefficient with N2 for all amines loaded. However, the effect of loading trialkylamines is not remarkable in the absence of water. The effect of loading dialkylamine does not depend on water, but the adsorbent cannot be regenerated at ambient temperature. In comparison, an adsorbent loading trialkylamine can be regenerated at ambient temperature even in the presence of water with fairly good stability. |
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| References | MetzBDavidsonOBoschPMitigation of Climate Change[M]2007New YorkCambridge University Press MetzBDavidsonOConinckH DCarbon Dioxide Capture and Storage [M]2005New YorkCambridge University Press DouglasACostasTSeparation of CO2 from flue gas: A review [J]Separation Science and Technology2005401–3321348 ArenillasASmithK MDrageT CCO2 capture using some fly ash-derived carbon materials[J]Fuel200584172204221010.1016/j.fuel.2005.04.003 YangHXuZFanMProgress in carbon dioxide separation and capture: A review [J]Journal of Environmental Science2008201142710.1016/S1001-0742(08)60002-9 PlazaM GPevidaCArenillasACO2 capture by adsorption with nitrogen enriched carbons [J]Fuel200786142204221210.1016/j.fuel.2007.06.001 BarrettE PJoynerL GHalendaP PThe determination of pore volume and area distributions in porous substances (I): Computations from nitrogen isotherms [J]Journal of the American Chemical Society195173137338010.1021/ja01145a126 XueQ MWuDZhouY PImprovement of aminemodification with piperazine for the adsorption of CO2[J]Applied Surface Science201225883859386310.1016/j.apsusc.2011.12.046 ZhouLWuJ QLiMPrediction of multicomponent adsorption equilibrium of gas mixtures including supercritical components [J]Chemical Engineering Science200560112833284410.1016/j.ces.2004.11.058 IEA.Key World Energy Statistics [M]2008ParisOECD/IEA Publishing DíazEMuñozEVegaAEnhancement of the CO2 retention capacity of Y zeolites by Na and Cs treatments: Effects of adsorption temperature and water treatment [J]Industrial & Engineering Chemistry Research200847241241810.1021/ie070685c XuX CSongC SAndersenJ MPreparation and characterization of novel CO2 ‘molecular basket’ adsorbents based on polymer-modified mesoporous molecular sieve MCM-41 [J]Microporous and Mesoporous Materials2003621/2294510.1016/S1387-1811(03)00388-3 ChoiSDreseJ HJonesC WAdsorbent materials for carbon dioxide capture from large anthropogenic point sources [J]ChemSusChem20092979685410.1002/cssc.200900036 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exceptional CO2 dynamic and equilibrium adsorption performance [J]Industrial & Engineering Chemistry Research200746244645810.1021/ie060774 SiriwardaneR VShenMFisherE PAdsorption of CO2 on molecular sieves and activated carbon [J]Energy Fuels200115227928410.1021/ef000241s IEA.Tracking Industrial Energy Efficiency and CO2 Emissions [M]2007ParisOECD/IEA Publishing WangX PYuJ JChengJHigh temperature adsorption of carbon dioxide on mixed oxides derived hydrotalcite-like compounds [J]Environmental Science and Technology2008422614618243572910.1021/es072085a DrageT CArenillasASmithK MPreparation of carbon dioxide adsorbents from the chemical activation of urea-formaldehyde and melamine-formaldehyde resins [J]Fuel2007861/2223110.1016/j.fuel.2006.07.003 YangR TGas Separation by Adsorption Process[M]1987BostonButter Worths HarlickP J ESayariAApplications of pore-expanded mesoporous silicas(3): Triamine silane grafting for enhanced CO2 adsorption [J]Industrial & Engineering Chemistry Research20064593248325510.1021/ie051286p ZhangJWebleyP AXiaoPEffect of process parameters on power requirements of vacuum swing adsorption technology for CO2 capture from flue gas [J]Energy Conversion and Management200849234635610.1016/j.enconman.2007.06.007 LiuX WZhouLFuXAdsorption and regeneration study of the mesoporous adsorbent SBA-15 adapted to the capture/separation of CO2 and CH4 [J]Chemical Engineering Science20076241101111010.1016/j.ces.2006.11.005 RuthvenD MPrinciples of Adsorption and Adsorption Process[M]1984New YorkWiley LealOBolivarCOvallesCReversible adsorption of carbon dioxide on amine surface-bonded silica gel [J]Inorganica Chimica Acta19952401/218318910.1016/0020-1693(95)04534-1 NorihitoHKatsunoriYTatsuakiYAdsorption characteristics of carbon dioxide on organically functionalized SBA-15 [J]Microporous and Mesoporous Materials2005841–3357365 YueM BSunL BCaoYEfficient CO2 capturer derived from as-synthesized MCM-41 modified with amine [J]Chemistry — A European 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| References_xml | – reference: ZhangZ ZRuanH ZZhouY PA research note on the adsorption of CO2 and N2[J]Chinese Journal of Chemical Engineering201119573373710.1016/S1004-9541(11)60050-5 – reference: MetzBDavidsonOConinckH DCarbon Dioxide Capture and Storage [M]2005New YorkCambridge University Press – reference: JadhavP DRayaluS SBiniwaleR BCO2 emission and its mitigation by adsorption on zeolites and activated carbon [J]Current Science2007926724726 – reference: PlazaM GPevidaCAriasBDevelopment of lowcost biomass-based adsorbents for postcombustion CO2 capture [J]Fuel200988122442244710.1016/j.fuel.2009.02.025 – reference: NorihitoHKatsunoriYTatsuakiYAdsorption characteristics of carbon dioxide on organically functionalized SBA-15 [J]Microporous and Mesoporous Materials2005841–3357365 – reference: KnowlesG PGrahamJ VDelaneyS WAminopropyl-functionalized mesoporous silicas as CO2 adsorbents [J]Fuel Processing Technology20058614/151435144810.1016/j.fuproc.2005.01.014 – reference: HarlickP J ESayariAApplications of pore-expanded mesoporous silicas(3): Triamine silane grafting for enhanced CO2 adsorption [J]Industrial & Engineering Chemistry Research20064593248325510.1021/ie051286p – reference: ZhouLWuJ QLiMPrediction of multicomponent adsorption equilibrium of gas mixtures including supercritical components [J]Chemical Engineering Science200560112833284410.1016/j.ces.2004.11.058 – reference: YueM BSunL BCaoYEfficient CO2 capturer derived from as-synthesized MCM-41 modified with amine [J]Chemistry — A European Journal200814113442345110.1002/chem.200701467 – reference: YangR TGas Separation by Adsorption Process[M]1987BostonButter Worths – reference: LiuX WZhouLFuXAdsorption and regeneration study of the mesoporous adsorbent SBA-15 adapted to the capture/separation of CO2 and CH4 [J]Chemical Engineering Science20076241101111010.1016/j.ces.2006.11.005 – reference: DíazEMuñozEVegaAEnhancement of the CO2 retention capacity of Y zeolites by Na and Cs treatments: Effects of adsorption temperature and water treatment [J]Industrial & Engineering Chemistry Research200847241241810.1021/ie070685c – reference: ChoiSDreseJ HJonesC WAdsorbent materials for carbon dioxide capture from large anthropogenic point sources [J]ChemSusChem20092979685410.1002/cssc.200900036 – reference: MetzBDavidsonOBoschPMitigation of Climate Change[M]2007New YorkCambridge University Press – reference: WangX PYuJ JChengJHigh temperature adsorption of carbon dioxide on mixed oxides derived hydrotalcite-like compounds [J]Environmental Science and Technology2008422614618243572910.1021/es072085a – reference: IEA.Key World Energy Statistics [M]2008ParisOECD/IEA Publishing – reference: DouglasACostasTSeparation of CO2 from flue gas: A review [J]Separation Science and Technology2005401–3321348 – reference: LealOBolivarCOvallesCReversible adsorption of carbon dioxide on amine surface-bonded silica gel [J]Inorganica Chimica Acta19952401/218318910.1016/0020-1693(95)04534-1 – reference: ArenillasASmithK MDrageT CCO2 capture using some fly ash-derived carbon materials[J]Fuel200584172204221010.1016/j.fuel.2005.04.003 – reference: XuX CSongC SAndersenJ MPreparation and characterization of novel CO2 ‘molecular basket’ adsorbents based on polymer-modified mesoporous molecular sieve MCM-41 [J]Microporous and Mesoporous Materials2003621/2294510.1016/S1387-1811(03)00388-3 – reference: HarlickP J ESayariAApplications of pore-expanded mesoporous silica(5): Triamine grafted material with exceptional CO2 dynamic and equilibrium adsorption performance [J]Industrial & Engineering Chemistry Research200746244645810.1021/ie060774+ – reference: DrageT CArenillasASmithK MPreparation of carbon dioxide adsorbents from the chemical activation of urea-formaldehyde and melamine-formaldehyde resins [J]Fuel2007861/2223110.1016/j.fuel.2006.07.003 – reference: BrunauerSEmmettP HTellermE JAdsorption of gases in multimolecular layers [J]Journal of the American Chemical Society193860230931910.1021/ja01269a023 – reference: ZhangJWebleyP AXiaoPEffect of process parameters on power requirements of vacuum swing adsorption technology for CO2 capture from flue gas [J]Energy Conversion and Management200849234635610.1016/j.enconman.2007.06.007 – reference: HiyoshiNYogoKYashimaTAdsorption of carbon dioxide on amine modified SBA-15 in the presence of water vapor [J]Chemistry Letters200433551051110.1246/cl.2004.510 – reference: RuthvenD MPrinciples of Adsorption and Adsorption Process[M]1984New YorkWiley – reference: YangHXuZFanMProgress in carbon dioxide separation and capture: A review [J]Journal of Environmental Science2008201142710.1016/S1001-0742(08)60002-9 – reference: KimJ HLeeC HKimW SAdsorption equilibria of water vapor on alumina, zeolite 13X, and a zeolite X/activated carbon composite [J]Journal of Chemical & Engineering Data200348113714110.1021/je0201267 – reference: PlazaM GPevidaCArenillasACO2 capture by adsorption with nitrogen enriched carbons [J]Fuel200786142204221210.1016/j.fuel.2007.06.001 – reference: IEA.Tracking Industrial Energy Efficiency and CO2 Emissions [M]2007ParisOECD/IEA Publishing – reference: GuoBChangL PXieK CAdsorption of carbon dioxide on activated carbon [J]Journal of Natural Gas Chemistry200615322322910.1016/S1003-9953(06)60030-3 – reference: BarrettE PJoynerL GHalendaP PThe determination of pore volume and area distributions in porous substances (I): Computations from nitrogen isotherms [J]Journal of the American Chemical Society195173137338010.1021/ja01145a126 – reference: LiYYangR TGas adsorption and storage in metalorganic framework MOF-177 [J]Langmuir20072326129371294410.1021/la702466d – reference: HiyoshiNYogoKYashimaTAdsorption of carbon di-oxide on aminosilane-modified mesoporous silica [J]J Jpn Pet Inst2005481293610.1627/jpi.48.29 – reference: XueQ MWuDZhouY PImprovement of aminemodification with piperazine for the adsorption of CO2[J]Applied Surface 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| Snippet | The adsorption of CO2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO2 from other gases is promoted. Water plays an... The adsorption of CO 2 can be enhanced through loading amines on adsorbents, therefore, the separation of CO 2 from other gases is promoted. Water plays an... |
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| SubjectTerms | Engineering Humanities and Social Sciences Mechanical Engineering multidisciplinary Science 三烷基胺 二氧化碳 分离系数 加载 改性吸附剂 气体分离 水 环境温度 |
| Title | Water Effect on Amine-Modification of Adsorbents for Separation of CO2/N2 |
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