Thermodynamic modeling of aqueous Na+–K+–Mg2+–SO42− quaternary system

A comprehensive thermodynamic model based on the electrolyte non-random two-liquid (eNRTL) theory is developed for aqueous Na+–K+–Mg2+–SO42− quaternary system. The model accounts for the liquid phase nonideality by two binary interaction parameters per water-electrolyte and electrolyte–electrolyte p...

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Published inFluid phase equilibria Vol. 404; pp. 141 - 149
Main Authors Bhattacharia, Sanjoy K., Tanveer, Sheik, Hossain, Nazir, Chen, Chau-Chyun
Format Journal Article
LanguageEnglish
Published Elsevier B.V 25.10.2015
Subjects
Aqueous electrolytes
Electrolyte NRTL model
Magnesium sulfate
Solubility
Thermodynamic properties
Aqueous electrolytes
Magnesium sulfate
Thermodynamic properties
Electrolyte NRTL model
Solubility
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Abstract A comprehensive thermodynamic model based on the electrolyte non-random two-liquid (eNRTL) theory is developed for aqueous Na+–K+–Mg2+–SO42− quaternary system. The model accounts for the liquid phase nonideality by two binary interaction parameters per water-electrolyte and electrolyte–electrolyte pair. The temperature dependence of the binary interaction parameters is further correlated with three temperature coefficients associated with a Gibbs Helmholtz type expression. We obtain the binary interaction parameters for the H2O:(Mg2+ SO42−) pair, the (Na+ SO42−):(Mg2+ SO42−) pair and the (K+ SO42−):(Mg2+ SO42−) pair by regressing appropriate thermodynamic data. Integrated with other eNRTL binary interaction parameters in the literature, the eNRTL model accurately represents various thermodynamic properties of aqueous Na+–K+–Mg2+–SO42− quaternary system and its subsystems with temperatures up to 473.15K and electrolyte concentrations up to saturation.
AbstractList A comprehensive thermodynamic model based on the electrolyte non-random two-liquid (eNRTL) theory is developed for aqueous Na+–K+–Mg2+–SO42− quaternary system. The model accounts for the liquid phase nonideality by two binary interaction parameters per water-electrolyte and electrolyte–electrolyte pair. The temperature dependence of the binary interaction parameters is further correlated with three temperature coefficients associated with a Gibbs Helmholtz type expression. We obtain the binary interaction parameters for the H2O:(Mg2+ SO42−) pair, the (Na+ SO42−):(Mg2+ SO42−) pair and the (K+ SO42−):(Mg2+ SO42−) pair by regressing appropriate thermodynamic data. Integrated with other eNRTL binary interaction parameters in the literature, the eNRTL model accurately represents various thermodynamic properties of aqueous Na+–K+–Mg2+–SO42− quaternary system and its subsystems with temperatures up to 473.15K and electrolyte concentrations up to saturation.
Author Hossain, Nazir
Chen, Chau-Chyun
Tanveer, Sheik
Bhattacharia, Sanjoy K.
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Keywords Aqueous electrolytes
Magnesium sulfate
Thermodynamic properties
Electrolyte NRTL model
Solubility
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Snippet A comprehensive thermodynamic model based on the electrolyte non-random two-liquid (eNRTL) theory is developed for aqueous Na+–K+–Mg2+–SO42− quaternary system....
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SubjectTerms Aqueous electrolytes
Electrolyte NRTL model
Magnesium sulfate
Solubility
Thermodynamic properties
Title Thermodynamic modeling of aqueous Na+–K+–Mg2+–SO42− quaternary system
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