Structure and dielectric properties of (1-x)Bi 0.5 Na 0.5 TiO 3-x BaTiO 3 piezoceramics prepared using hydrothermally synthesized powders
The influence of different processing parameters and various Ba addition (up to 10 mol%) on the structure and dielectric properties of Bi Na TiO -BaTiO (BNT-BT) ceramics was investigated. The powders were hydrothermally synthesized in the alkaline environment at 180°C for different time periods. X-r...
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Published in | Royal Society open science Vol. 8; no. 7; p. 202365 |
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Main Authors | , , , , , , , |
Format | Journal Article |
Language | English |
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01.07.2021
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Abstract | The influence of different processing parameters and various Ba
addition (up to 10 mol%) on the structure and dielectric properties of Bi
Na
TiO
-BaTiO
(BNT-BT) ceramics was investigated. The powders were hydrothermally synthesized in the alkaline environment at 180°C for different time periods. X-ray diffraction confirmed the presence of dominant rhombohedral Bi
Na
TiO
phase and a small amount of secondary pyrochlore Bi
Ti
O
phase in the pure BNT powders. In addition, one-dimensional Na
Ti
O
structure was also observed in the powder hydrothermally treated for a long time (i.e. 48 h). The amount of secondary pyrochlore phase in the BNT-BT powders increases with the increase of Ba
content. The synthesized powders were pressed into pellets and finally sintered at various temperatures up to 1150°C. High density (more than 90%TD) was obtained in all BNT-BT sintered samples. Optimal sintering parameters were chosen in order to obtain dense ceramics with the optimal phase composition. The temperature dependence of dielectric properties for the BNT-BT ceramics was also studied. Relaxor behaviour of BNT-based ceramics and broad transition peaks are evident in all samples. Dielectric constant up to 400 as well as an acceptable low dielectric loss at temperatures lower than 200°C were obtained in BNT-BT ceramics. |
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AbstractList | The influence of different processing parameters and various Ba
2+
addition (up to 10 mol%) on the structure and dielectric properties of Bi
0.5
Na
0.5
TiO
3
-BaTiO
3
(BNT-BT) ceramics was investigated. The powders were hydrothermally synthesized in the alkaline environment at 180°C for different time periods. X-ray diffraction confirmed the presence of dominant rhombohedral Bi
0.5
Na
0.5
TiO
3
phase and a small amount of secondary pyrochlore Bi
2
Ti
2
O
7
phase in the pure BNT powders. In addition, one-dimensional Na
2
Ti
2
O
7
structure was also observed in the powder hydrothermally treated for a long time (i.e. 48 h). The amount of secondary pyrochlore phase in the BNT-BT powders increases with the increase of Ba
2+
content. The synthesized powders were pressed into pellets and finally sintered at various temperatures up to 1150°C. High density (more than 90%TD) was obtained in all BNT-BT sintered samples. Optimal sintering parameters were chosen in order to obtain dense ceramics with the optimal phase composition. The temperature dependence of dielectric properties for the BNT-BT ceramics was also studied. Relaxor behaviour of BNT-based ceramics and broad transition peaks are evident in all samples. Dielectric constant up to 400 as well as an acceptable low dielectric loss at temperatures lower than 200°C were obtained in BNT-BT ceramics. The influence of different processing parameters and various Ba addition (up to 10 mol%) on the structure and dielectric properties of Bi Na TiO -BaTiO (BNT-BT) ceramics was investigated. The powders were hydrothermally synthesized in the alkaline environment at 180°C for different time periods. X-ray diffraction confirmed the presence of dominant rhombohedral Bi Na TiO phase and a small amount of secondary pyrochlore Bi Ti O phase in the pure BNT powders. In addition, one-dimensional Na Ti O structure was also observed in the powder hydrothermally treated for a long time (i.e. 48 h). The amount of secondary pyrochlore phase in the BNT-BT powders increases with the increase of Ba content. The synthesized powders were pressed into pellets and finally sintered at various temperatures up to 1150°C. High density (more than 90%TD) was obtained in all BNT-BT sintered samples. Optimal sintering parameters were chosen in order to obtain dense ceramics with the optimal phase composition. The temperature dependence of dielectric properties for the BNT-BT ceramics was also studied. Relaxor behaviour of BNT-based ceramics and broad transition peaks are evident in all samples. Dielectric constant up to 400 as well as an acceptable low dielectric loss at temperatures lower than 200°C were obtained in BNT-BT ceramics. |
Author | Nesterović, Andrea Vukmirović, Jelena Stijepović, Ivan Milanović, Marija Tóth, Elvira Bajac, Branimir Srdić, Vladimir V Cvejić, Željka |
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BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34350012$$D View this record in MEDLINE/PubMed |
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CitedBy_id | crossref_primary_10_1016_j_ceramint_2024_02_203 crossref_primary_10_1016_j_matchemphys_2023_127457 crossref_primary_10_15251_DJNB_2023_184_1409 crossref_primary_10_1007_s11664_023_10407_9 crossref_primary_10_1080_21870764_2022_2076362 crossref_primary_10_1007_s10854_022_08187_9 crossref_primary_10_1007_s10854_023_10308_x crossref_primary_10_1007_s11664_023_10486_8 crossref_primary_10_1007_s00339_023_06990_7 crossref_primary_10_1016_j_ceramint_2023_09_210 crossref_primary_10_1016_j_jssc_2022_122940 crossref_primary_10_1080_21870764_2024_2314340 |
Cites_doi | 10.1143/JJAP.30.2236 10.1515/ehs-2016-0028 10.1039/C7RA01293D 10.1063/1.4804940 10.1007/s10854-017-8054-4 10.1107/S0108768101020845 10.1002/jrs.5603 10.2298/PAC0802109N 10.2320/matertrans.MRA2007043 10.4028/www.scientific.net/AMR.482-484.2573 10.1016/j.jeurceramsoc.2011.04.025 10.1039/C7TC03812G 10.1016/j.ceramint.2013.01.015 10.1016/j.jeurceramsoc.2007.02.156 10.1007/s10853-007-2246-x 10.1016/S0921-5107(02)00515-9 10.1007/s10853-007-1853-x 10.1016/j.jallcom.2011.07.034 10.1016/j.ceramint.2015.11.162 10.1142/S2010135X17500199 10.1134/S0020168520010136 10.1142/S1793604710000919 10.1016/j.jallcom.2011.11.129 10.1039/c3ce40139a 10.1088/0953-8984/23/5/055901 10.1016/j.ceramint.2017.05.115 10.1111/j.1551-2916.2009.03061.x 10.1016/j.cap.2012.01.016 10.1016/j.jeurceramsoc.2014.12.036 10.1021/cm9906654 10.1002/jrs.1032 10.1016/j.jallcom.2011.06.085 10.1007/s10832-007-9047-0 10.4028/www.scientific.net/AMR.763.135 |
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References | e_1_3_7_20_2 Nesterović A (e_1_3_7_38_2) 2021 e_1_3_7_22_2 e_1_3_7_21_2 e_1_3_7_24_2 e_1_3_7_23_2 e_1_3_7_26_2 e_1_3_7_25_2 Mendez-González Y (e_1_3_7_30_2) 2019; 50 Jaffe B (e_1_3_7_9_2) 1971 e_1_3_7_28_2 e_1_3_7_27_2 e_1_3_7_29_2 Smolenskii GA (e_1_3_7_6_2) 1961; 2 e_1_3_7_31_2 e_1_3_7_10_2 e_1_3_7_33_2 e_1_3_7_11_2 e_1_3_7_32_2 e_1_3_7_12_2 e_1_3_7_35_2 e_1_3_7_13_2 e_1_3_7_34_2 e_1_3_7_14_2 e_1_3_7_37_2 e_1_3_7_15_2 e_1_3_7_36_2 e_1_3_7_16_2 e_1_3_7_17_2 e_1_3_7_18_2 e_1_3_7_19_2 e_1_3_7_2_2 e_1_3_7_4_2 e_1_3_7_3_2 e_1_3_7_5_2 e_1_3_7_8_2 e_1_3_7_7_2 |
References_xml | – ident: e_1_3_7_10_2 doi: 10.1143/JJAP.30.2236 – ident: e_1_3_7_3_2 doi: 10.1515/ehs-2016-0028 – ident: e_1_3_7_16_2 doi: 10.1039/C7RA01293D – ident: e_1_3_7_31_2 doi: 10.1063/1.4804940 – ident: e_1_3_7_36_2 doi: 10.1007/s10854-017-8054-4 – ident: e_1_3_7_7_2 doi: 10.1107/S0108768101020845 – volume: 50 start-page: 1044 year: 2019 ident: e_1_3_7_30_2 article-title: Raman spectroscopy study of the La-modified (Bi0.5Na0.5)0.92Ba0.08TiO3 lead-free ceramic system publication-title: J. Raman Spectrosc. doi: 10.1002/jrs.5603 contributor: fullname: Mendez-González Y – ident: e_1_3_7_27_2 doi: 10.2298/PAC0802109N – ident: e_1_3_7_26_2 doi: 10.2320/matertrans.MRA2007043 – ident: e_1_3_7_14_2 doi: 10.4028/www.scientific.net/AMR.482-484.2573 – ident: e_1_3_7_19_2 doi: 10.1016/j.jeurceramsoc.2011.04.025 – ident: e_1_3_7_21_2 doi: 10.1039/C7TC03812G – ident: e_1_3_7_24_2 doi: 10.1016/j.ceramint.2013.01.015 – ident: e_1_3_7_28_2 doi: 10.1016/j.jeurceramsoc.2007.02.156 – ident: e_1_3_7_8_2 doi: 10.1007/s10853-007-2246-x – ident: e_1_3_7_11_2 doi: 10.1016/S0921-5107(02)00515-9 – ident: e_1_3_7_12_2 doi: 10.1007/s10853-007-1853-x – ident: e_1_3_7_18_2 doi: 10.1016/j.jallcom.2011.07.034 – ident: e_1_3_7_32_2 doi: 10.1016/j.ceramint.2015.11.162 – volume: 2 start-page: 2651 year: 1961 ident: e_1_3_7_6_2 article-title: New ferroelectrics of complex composition publication-title: Sov. Phys. Solid State contributor: fullname: Smolenskii GA – ident: e_1_3_7_20_2 doi: 10.1142/S2010135X17500199 – ident: e_1_3_7_22_2 doi: 10.1134/S0020168520010136 – ident: e_1_3_7_5_2 doi: 10.1142/S1793604710000919 – ident: e_1_3_7_25_2 doi: 10.1016/j.jallcom.2011.11.129 – ident: e_1_3_7_15_2 doi: 10.1039/c3ce40139a – ident: e_1_3_7_33_2 doi: 10.1088/0953-8984/23/5/055901 – ident: e_1_3_7_17_2 doi: 10.1016/j.ceramint.2017.05.115 – ident: e_1_3_7_2_2 doi: 10.1111/j.1551-2916.2009.03061.x – ident: e_1_3_7_37_2 doi: 10.1016/j.cap.2012.01.016 – ident: e_1_3_7_34_2 doi: 10.1016/j.jeurceramsoc.2014.12.036 – year: 2021 ident: e_1_3_7_38_2 publication-title: Dryad Digital Repository contributor: fullname: Nesterović A – volume-title: Piezoeletric ceramics year: 1971 ident: e_1_3_7_9_2 contributor: fullname: Jaffe B – ident: e_1_3_7_13_2 doi: 10.1021/cm9906654 – ident: e_1_3_7_29_2 doi: 10.1002/jrs.1032 – ident: e_1_3_7_35_2 doi: 10.1016/j.jallcom.2011.06.085 – ident: e_1_3_7_4_2 doi: 10.1007/s10832-007-9047-0 – ident: e_1_3_7_23_2 doi: 10.4028/www.scientific.net/AMR.763.135 |
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Snippet | The influence of different processing parameters and various Ba
addition (up to 10 mol%) on the structure and dielectric properties of Bi
Na
TiO
-BaTiO... The influence of different processing parameters and various Ba 2+ addition (up to 10 mol%) on the structure and dielectric properties of Bi 0.5 Na 0.5 TiO 3... |
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Title | Structure and dielectric properties of (1-x)Bi 0.5 Na 0.5 TiO 3-x BaTiO 3 piezoceramics prepared using hydrothermally synthesized powders |
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