X-ray induced grain boundary formation and grain rotation in Bi2Se3
Optimizing grain boundary characteristics in polycrystalline materials can improve their properties. Many processing methods have been developed for grain boundary manipulation, including the use of intense radiation in certain applications. In this work, we used X-ray free electron laser pulses to...
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| Published in | Scripta materialia Vol. 256; no. C; p. 116416 |
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| Main Authors | , , , , , , , , , , , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Ltd
01.02.2025
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Optimizing grain boundary characteristics in polycrystalline materials can improve their properties. Many processing methods have been developed for grain boundary manipulation, including the use of intense radiation in certain applications. In this work, we used X-ray free electron laser pulses to irradiate single-crystalline bismuth selenide (Bi2Se3) and observed grain boundary formation and subsequent grain rotation in response to the X-ray radiation. Our observations with simultaneous transmission X-ray microscopy and X-ray diffraction demonstrate how intense X-ray radiation can rapidly change size and texture of grains.
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| AbstractList | Optimizing grain boundary characteristics in polycrystalline materials can improve their properties. Many processing methods have been developed for grain boundary manipulation, including the use of intense radiation in certain applications. In this work, we used X-ray free electron laser pulses to irradiate single-crystalline bismuth selenide (Bi2Se3) and observed grain boundary formation and subsequent grain rotation in response to the X-ray radiation. Our observations with simultaneous transmission X-ray microscopy and X-ray diffraction demonstrate how intense X-ray radiation can rapidly change size and texture of grains.
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| ArticleNumber | 116416 |
| Author | Katagiri, Kento Preston, Thomas R. Appel, Karen Cook, Philip K. Seiboth, Frank Yang, Wenge Eggert, Jon Wang, Bihan Zastrau, Ulf Chalise, Darshan Makita, Mikako Schwinkendorf, Jan-Patrick Simons, Hugh Nielsen, Martin M. Kim, Sungwon Pelka, Alexander Kim, Hyunjung Dresselhaus-Marais, Leora E. Nakatsutsumi, Motoaki Kozioziemski, Bernard Folsom, Eric Poulsen, Henning F. Göde, Sebastian Howard, Marylesa Konôpková, Zuzana Wang, Yifan Reddy, Tharun |
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| Keywords | Thermoelectric materials Grain boundary engineering Dislocation dynamics Bismuth selenide (Bi2Se3) |
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| Title | X-ray induced grain boundary formation and grain rotation in Bi2Se3 |
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