Mixed Alkali-zinc Effects on Thermo-mechanical Properties in Borosilicate Glasses
A series of mixed alkali-zinc borosilicate glasses with various r values ( r = molar ratio of [ZnO] / ([R 2 O]+[ZnO])) from 0.00 to 1.00 were fabricated to probe the mixed alkali-zinc effects on thermo-mechanical properties. The nonlinear evolution of glass transition temperature ( T g ) with the ad...
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| Published in | Journal of Wuhan University of Technology. Materials science edition Vol. 39; no. 5; pp. 1093 - 1099 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Wuhan
Wuhan University of Technology
01.10.2024
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| Abstract | A series of mixed alkali-zinc borosilicate glasses with various
r
values (
r
= molar ratio of [ZnO] / ([R
2
O]+[ZnO])) from 0.00 to 1.00 were fabricated to probe the mixed alkali-zinc effects on thermo-mechanical properties. The nonlinear evolution of glass transition temperature (
T
g
) with the addition of ZnO is ascribed to the competition of two converse factors,
i e
, the
T
g
depression as one of the colligative properties for a solution, on the one hand, and the enhancement of
T
g
due to the higher field strength of zinc cations compared to that of alkali ions. However, the nonlinear evolution of elastic moduli and coefficients of thermal expansion with
r
is attributed to the variance of intermediate-range clusters, which is confirmed by infrared and Raman scattering spectra. These findings are very helpful in tailoring the performance of borosilicate glasses. |
|---|---|
| AbstractList | A series of mixed alkali-zinc borosilicate glasses with various
r
values (
r
= molar ratio of [ZnO] / ([R
2
O]+[ZnO])) from 0.00 to 1.00 were fabricated to probe the mixed alkali-zinc effects on thermo-mechanical properties. The nonlinear evolution of glass transition temperature (
T
g
) with the addition of ZnO is ascribed to the competition of two converse factors,
i e
, the
T
g
depression as one of the colligative properties for a solution, on the one hand, and the enhancement of
T
g
due to the higher field strength of zinc cations compared to that of alkali ions. However, the nonlinear evolution of elastic moduli and coefficients of thermal expansion with
r
is attributed to the variance of intermediate-range clusters, which is confirmed by infrared and Raman scattering spectra. These findings are very helpful in tailoring the performance of borosilicate glasses. |
| Author | Zhou, Hemin Xiao, Guanzhou Zheng, Qingshuang Qiao, Ang Tao, Haizheng Tao, Yunhang |
| Author_xml | – sequence: 1 givenname: Guanzhou surname: Xiao fullname: Xiao, Guanzhou organization: State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology – sequence: 2 givenname: Yunhang surname: Tao fullname: Tao, Yunhang organization: State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology – sequence: 3 givenname: Hemin surname: Zhou fullname: Zhou, Hemin organization: State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology – sequence: 4 givenname: Qingshuang surname: Zheng fullname: Zheng, Qingshuang organization: State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology – sequence: 5 givenname: Ang surname: Qiao fullname: Qiao, Ang organization: Wuhan University of Technology Advanced Engineering Technology Research Institute of Zhongshan City – sequence: 6 givenname: Haizheng surname: Tao fullname: Tao, Haizheng email: thz@whut.edu.cn organization: State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology |
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r
values (
r
= molar ratio of [ZnO] / ([R
2
O]+[ZnO])) from 0.00 to 1.00 were fabricated to... |
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| Title | Mixed Alkali-zinc Effects on Thermo-mechanical Properties in Borosilicate Glasses |
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