Investigations on energy transfer mechanism and tunable luminescent properties of Co-doped Ca9La(PO4)7:Dy3+,Eu3+ phosphors
The synthesized Ca 9 La(PO 4 ) 7 :Dy 3+ ,Eu 3+ (CLPO:Dy 3+ ,Eu 3+ ) phosphors were analyzed by phase structure, optical performance, thermal stability and lifetime. The XRD pattern indicated that both the matrix and rare earth ion-doped phosphors were pure phases, and the crystal structure was confi...
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Published in | Applied physics. A, Materials science & processing Vol. 126; no. 5 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
2020
Springer Nature B.V |
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Abstract | The synthesized Ca
9
La(PO
4
)
7
:Dy
3+
,Eu
3+
(CLPO:Dy
3+
,Eu
3+
) phosphors were analyzed by phase structure, optical performance, thermal stability and lifetime. The XRD pattern indicated that both the matrix and rare earth ion-doped phosphors were pure phases, and the crystal structure was confirmed as trigonal system. Upon 351 nm excitation, Dy
3+
-doped CLPO phosphors performed two strong emission peaks at 481 nm and 573 nm. The energy transfer phenomenon from Dy
3+
to Eu
3+
can be found in the Dy
3+
, Eu
3+
co-doped CLPO phosphors, and the color was tuned from red to blue upon 395 nm excitation with Eu
3+
concentration decreasing. The energy transfer characteristic was evidenced by the excitation spectra, emission spectrum and decay time of the synthesized phosphors, and the mechanism of energy transfer from Dy
3+
to Eu
3+
was evaluated as a dipole–quadrupole interaction. In addition, temperature-dependent spectra were performed and the activation energy was further evaluated about 0.1902 eV. The results indicate the potential application of CLPO:Dy
3+
,Eu
3+
phosphors in white LEDs. |
---|---|
AbstractList | The synthesized Ca9La(PO4)7:Dy3+,Eu3+(CLPO:Dy3+,Eu3+) phosphors were analyzed by phase structure, optical performance, thermal stability and lifetime. The XRD pattern indicated that both the matrix and rare earth ion-doped phosphors were pure phases, and the crystal structure was confirmed as trigonal system. Upon 351 nm excitation, Dy3+-doped CLPO phosphors performed two strong emission peaks at 481 nm and 573 nm. The energy transfer phenomenon from Dy3+ to Eu3+ can be found in the Dy3+, Eu3+ co-doped CLPO phosphors, and the color was tuned from red to blue upon 395 nm excitation with Eu3+ concentration decreasing. The energy transfer characteristic was evidenced by the excitation spectra, emission spectrum and decay time of the synthesized phosphors, and the mechanism of energy transfer from Dy3+ to Eu3+ was evaluated as a dipole–quadrupole interaction. In addition, temperature-dependent spectra were performed and the activation energy was further evaluated about 0.1902 eV. The results indicate the potential application of CLPO:Dy3+,Eu3+ phosphors in white LEDs. The synthesized Ca 9 La(PO 4 ) 7 :Dy 3+ ,Eu 3+ (CLPO:Dy 3+ ,Eu 3+ ) phosphors were analyzed by phase structure, optical performance, thermal stability and lifetime. The XRD pattern indicated that both the matrix and rare earth ion-doped phosphors were pure phases, and the crystal structure was confirmed as trigonal system. Upon 351 nm excitation, Dy 3+ -doped CLPO phosphors performed two strong emission peaks at 481 nm and 573 nm. The energy transfer phenomenon from Dy 3+ to Eu 3+ can be found in the Dy 3+ , Eu 3+ co-doped CLPO phosphors, and the color was tuned from red to blue upon 395 nm excitation with Eu 3+ concentration decreasing. The energy transfer characteristic was evidenced by the excitation spectra, emission spectrum and decay time of the synthesized phosphors, and the mechanism of energy transfer from Dy 3+ to Eu 3+ was evaluated as a dipole–quadrupole interaction. In addition, temperature-dependent spectra were performed and the activation energy was further evaluated about 0.1902 eV. The results indicate the potential application of CLPO:Dy 3+ ,Eu 3+ phosphors in white LEDs. |
ArticleNumber | 378 |
Author | Ding, Heping Zhang, Ze Niu, Jialiang Bai, Dongsheng Zhou, Wei Wang, Xinrui |
Author_xml | – sequence: 1 givenname: Jialiang surname: Niu fullname: Niu, Jialiang organization: Department of Chemistry, School of Science, Beijing Technology and Business University – sequence: 2 givenname: Heping surname: Ding fullname: Ding, Heping organization: Department of Chemistry, School of Science, Beijing Technology and Business University – sequence: 3 givenname: Wei surname: Zhou fullname: Zhou, Wei email: zhouw@th.btbu.edu.cn organization: Department of Chemistry, School of Science, Beijing Technology and Business University – sequence: 4 givenname: Ze surname: Zhang fullname: Zhang, Ze organization: Department of Chemistry, School of Science, Beijing Technology and Business University – sequence: 5 givenname: Dongsheng surname: Bai fullname: Bai, Dongsheng organization: Beijing Key Lab of Plant Resource Research and Development, Beijing Technology and Business University – sequence: 6 givenname: Xinrui surname: Wang fullname: Wang, Xinrui organization: Beijing Key Lab of Plant Resource Research and Development, Beijing Technology and Business University |
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CitedBy_id | crossref_primary_10_1016_j_optmat_2024_115033 crossref_primary_10_1039_D1DT04124J crossref_primary_10_1016_j_jlumin_2021_118423 crossref_primary_10_1016_j_ceramint_2021_01_049 crossref_primary_10_1016_j_ceramint_2023_05_126 crossref_primary_10_1016_j_jallcom_2021_162758 crossref_primary_10_1016_j_molstruc_2024_137622 crossref_primary_10_1016_j_optmat_2024_115769 crossref_primary_10_1007_s10854_022_09602_x |
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Snippet | The synthesized Ca
9
La(PO
4
)
7
:Dy
3+
,Eu
3+
(CLPO:Dy
3+
,Eu
3+
) phosphors were analyzed by phase structure, optical performance, thermal stability and... The synthesized Ca9La(PO4)7:Dy3+,Eu3+(CLPO:Dy3+,Eu3+) phosphors were analyzed by phase structure, optical performance, thermal stability and lifetime. The XRD... |
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SubjectTerms | Applied physics Characterization and Evaluation of Materials Condensed Matter Physics Crystal structure Dipoles Dysprosium Emission spectra Energy transfer Europium Excitation spectra Machines Manufacturing Materials science Metal ions Nanotechnology Optical and Electronic Materials Optical properties Phosphors Physics Physics and Astronomy Processes Quadrupole interaction Quadrupoles Solid phases Stability analysis Surfaces and Interfaces Synthesis Temperature dependence Thermal stability Thin Films |
Title | Investigations on energy transfer mechanism and tunable luminescent properties of Co-doped Ca9La(PO4)7:Dy3+,Eu3+ phosphors |
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