Excitation‐Dependent Multicolour Luminescence of Organic Materials: Internal Mechanism and Potential Applications
Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such multicolour luminescence is a characteristic exception to the ubiquitously accepted Kasha's rule. This phenomenon has been increasingly presented in som...
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Published in | Angewandte Chemie Vol. 135; no. 6 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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01.02.2023
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Abstract | Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such multicolour luminescence is a characteristic exception to the ubiquitously accepted Kasha's rule. This phenomenon has been increasingly presented in some studies on different luminescence systems; however, a systematic overview of the mechanisms underlying this phenomenon is currently absent. Herein, we resolve this issue by classifying multicolour luminescence from single chromophores and dual/ternary chromophores, as well as multiple emitting species. The underlying processes are described based on electronic and/or geometrical conditions under which the phenomenon occurs. Before we present it in categories, related photophysical and photochemical foundations are introduced. This systematic overview will provide a clear approach to designing multicolour luminescence materials for special applications.
According to Kasha's rule for luminescent materials, the emitting electronic level of a given multiplicity is the lowest excited level of that multiplicity. A characteristic exception, excitation‐dependent multicolour emission, is presented systemically, with the aim of enriching fundamental photophysics and potential applications. This Minireview will serve as a timely summary of the scattered reports of multicolour phenomena and their underlying mechanisms. |
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AbstractList | Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such multicolour luminescence is a characteristic exception to the ubiquitously accepted Kasha's rule. This phenomenon has been increasingly presented in some studies on different luminescence systems; however, a systematic overview of the mechanisms underlying this phenomenon is currently absent. Herein, we resolve this issue by classifying multicolour luminescence from single chromophores and dual/ternary chromophores, as well as multiple emitting species. The underlying processes are described based on electronic and/or geometrical conditions under which the phenomenon occurs. Before we present it in categories, related photophysical and photochemical foundations are introduced. This systematic overview will provide a clear approach to designing multicolour luminescence materials for special applications. Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such multicolour luminescence is a characteristic exception to the ubiquitously accepted Kasha's rule. This phenomenon has been increasingly presented in some studies on different luminescence systems; however, a systematic overview of the mechanisms underlying this phenomenon is currently absent. Herein, we resolve this issue by classifying multicolour luminescence from single chromophores and dual/ternary chromophores, as well as multiple emitting species. The underlying processes are described based on electronic and/or geometrical conditions under which the phenomenon occurs. Before we present it in categories, related photophysical and photochemical foundations are introduced. This systematic overview will provide a clear approach to designing multicolour luminescence materials for special applications. According to Kasha's rule for luminescent materials, the emitting electronic level of a given multiplicity is the lowest excited level of that multiplicity. A characteristic exception, excitation‐dependent multicolour emission, is presented systemically, with the aim of enriching fundamental photophysics and potential applications. This Minireview will serve as a timely summary of the scattered reports of multicolour phenomena and their underlying mechanisms. Abstract Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such multicolour luminescence is a characteristic exception to the ubiquitously accepted Kasha's rule. This phenomenon has been increasingly presented in some studies on different luminescence systems; however, a systematic overview of the mechanisms underlying this phenomenon is currently absent. Herein, we resolve this issue by classifying multicolour luminescence from single chromophores and dual/ternary chromophores, as well as multiple emitting species. The underlying processes are described based on electronic and/or geometrical conditions under which the phenomenon occurs. Before we present it in categories, related photophysical and photochemical foundations are introduced. This systematic overview will provide a clear approach to designing multicolour luminescence materials for special applications. |
Author | Shen, Yunxia An, Zhongfu Yang, Bing Liu, Haichao Zhang, Yujian |
Author_xml | – sequence: 1 givenname: Yunxia surname: Shen fullname: Shen, Yunxia organization: Zhejiang Normal University – sequence: 2 givenname: Zhongfu orcidid: 0000-0002-6522-2654 surname: An fullname: An, Zhongfu organization: Nanjing Tech University (NanjingTech) – sequence: 3 givenname: Haichao surname: Liu fullname: Liu, Haichao email: hcliu@jlu.edu.cn organization: Jilin University – sequence: 4 givenname: Bing orcidid: 0000-0003-4827-0926 surname: Yang fullname: Yang, Bing organization: Jilin University – sequence: 5 givenname: Yujian orcidid: 0000-0003-4638-0056 surname: Zhang fullname: Zhang, Yujian email: sciencezyj@foxmail.com organization: Zhejiang Normal University |
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Snippet | Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such multicolour... Abstract Excitation‐dependent emission (Ex‐de) materials have been of considerable academic interest and have potential applications in real life. Such... |
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SubjectTerms | Chemistry Chromophores Excitation Excitation-Dependent Emission Information Encryption Kasha's Rule Luminescence Multicolour Emission Organic materials Photochemicals |
Title | Excitation‐Dependent Multicolour Luminescence of Organic Materials: Internal Mechanism and Potential Applications |
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