Excess molar enthalpies for binary carbon dioxide+diethyl carbonate system at 298.15–308.15K and 5.0–6.5MPa
The excess molar enthalpies of the carbon dioxide+diethyl carbonate system were determined using a flow-type isothermal microcalorimeter at temperatures from 298DDT15 to 308DDT15K and pressures from 5DDT0 to 6DDT5MPa. Mixtures shows strong exothermic behavior in these regions. In addition, a strong...
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Published in | Fluid phase equilibria Vol. 236; no. 1-2; pp. 146 - 155 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
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20.09.2005
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Abstract | The excess molar enthalpies of the carbon dioxide+diethyl carbonate system were determined using a flow-type isothermal microcalorimeter at temperatures from 298DDT15 to 308DDT15K and pressures from 5DDT0 to 6DDT5MPa. Mixtures shows strong exothermic behavior in these regions. In addition, a strong pressure dependency of the excess molar enthalpies was observed, and the excess molar enthalpy values decreased with increasing pressure. The experimental results were correlated using a composition-dependent equation and the Peng-Robinson equation of state with the conventional mixing rule. Finally, the prediction of excess molar enthalpies using three mixing rules (MHV1, MHV2, and Wong-Sandler) was also tested on the basis of the vapor-liquid equilibrium data. |
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AbstractList | The excess molar enthalpies of the carbon dioxide+diethyl carbonate system were determined using a flow-type isothermal microcalorimeter at temperatures from 298DDT15 to 308DDT15K and pressures from 5DDT0 to 6DDT5MPa. Mixtures shows strong exothermic behavior in these regions. In addition, a strong pressure dependency of the excess molar enthalpies was observed, and the excess molar enthalpy values decreased with increasing pressure. The experimental results were correlated using a composition-dependent equation and the Peng-Robinson equation of state with the conventional mixing rule. Finally, the prediction of excess molar enthalpies using three mixing rules (MHV1, MHV2, and Wong-Sandler) was also tested on the basis of the vapor-liquid equilibrium data. |
Author | Nagashima, Akinori Ochi, Kenji Kurihara, Kiyofumi Matsuda, Hiroyuki Yoshii, Shigetaka |
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